Effect of Reaction Pathway on the Extent and Mechanism of Uranium(VI) Immobilization with Calcium and Phosphate

Mehta, Vrajesh S.; Maillot, Fabien; Wang, Zheming; Catalano, Jeffrey G.; Giammar, Daniel E.

doi:10.1021/acs.est.5b06212

Effect of Reaction Pathway on the Extent and Mechanism of Uranium(VI) Immobilization with Calcium and Phosphate

Journal Article · Sun Feb 21 23:00:00 EST 2016 · Environmental Science and Technology

DOI:https://doi.org/10.1021/acs.est.5b06212· OSTI ID:1245508

Mehta, Vrajesh S. ^[1]; Maillot, Fabien ^[2]; Wang, Zheming ^[3]; Catalano, Jeffrey G. ^[2]; Giammar, Daniel E. ^[1]

Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, Missouri 63130, United States
Department of Earth and Planetary Sciences, Washington University in St. Louis, St. Louis, Missouri 63130, United States
Department of Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352, United States

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); National Science Foundation; USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23)

Grant/Contract Number:: AC05-76RL01830; SC0006857; AC02-06CH11357

OSTI ID:: 1245508

Journal Information:: Environmental Science and Technology, Journal Name: Environmental Science and Technology Journal Issue: 6 Vol. 50; ISSN 0013-936X

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

References (35)

Pore-scale evaluation of uranyl phosphate precipitation in a model groundwater system: PORE-SCALE URANYL PHOSPHATE PRECIPITATION Fanizza, Michael F.; Yoon, Hongkyu; Zhang, Changyong Water Resources Research, Vol. 49, Issue 2 https://doi.org/10.1002/wrcr.20088	journal	February 2013
Apparent solubilities of two amorphous calcium phosphates and of octacalcium phosphate in the temperature range 30–42°C Christoffersen, M. R.; Christoffersen, J.; Kibalczyc, W. Journal of Crystal Growth, Vol. 106, Issue 2-3 https://doi.org/10.1016/0022-0248(90)90079-Z	journal	November 1990
Theory of error for target factor analysis with applications to mass spectrometry and nuclear magnetic resonance spectrometry Malinowski, Edmund R. Analytica Chimica Acta, Vol. 103, Issue 4 https://doi.org/10.1016/S0003-2670(01)83099-3	journal	December 1978
Phosphate based immobilization of uranium in an oxidizing bedrock aquifer Jerden, James L.; Sinha, A. K. Applied Geochemistry, Vol. 18, Issue 6 https://doi.org/10.1016/S0883-2927(02)00179-8	journal	June 2003
Trace element-incorporating octacalcium phosphate porous beads via polypeptide-assisted nanocrystal self-assembly for potential applications in osteogenesis Yang, X.; Zhang, L.; Chen, X. Acta Biomaterialia, Vol. 8, Issue 4 https://doi.org/10.1016/j.actbio.2011.12.012	journal	April 2012
The formation of autunite (Ca(UO2)2(PO4)2nH2O) within the leached layer of dissolving apatite: incorporation mechanism of uranium by apatite Ohnuki, T.; Kozai, N.; Samadfam, M. Chemical Geology, Vol. 211, Issue 1-2 https://doi.org/10.1016/j.chemgeo.2004.03.004	journal	November 2004
The biogeochemistry and bioremediation of uranium and other priority radionuclides Newsome, Laura; Morris, Katherine; Lloyd, Jonathan R. Chemical Geology, Vol. 363 https://doi.org/10.1016/j.chemgeo.2013.10.034	journal	January 2014
Effect of co-solutes on the products and solubility of uranium(VI) precipitated with phosphate Mehta, Vrajesh S.; Maillot, Fabien; Wang, Zheming Chemical Geology, Vol. 364 https://doi.org/10.1016/j.chemgeo.2013.12.002	journal	January 2014
Impact of phosphate on U(VI) immobilization in the presence of goethite Singh, Abhas; Ulrich, Kai-Uwe; Giammar, Daniel E. Geochimica et Cosmochimica Acta, Vol. 74, Issue 22 https://doi.org/10.1016/j.gca.2010.08.031	journal	November 2010
Determining individual mineral contributions to U(VI) adsorption in a contaminated aquifer sediment: A fluorescence spectroscopy study Wang, Zheming; Zachara, John M.; Boily, Jean-François Geochimica et Cosmochimica Acta, Vol. 75, Issue 10 https://doi.org/10.1016/j.gca.2011.03.008	journal	May 2011
Optics upgrades at the APS beamline 20-BM Heald, Steve M. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 649, Issue 1 https://doi.org/10.1016/j.nima.2010.11.070	journal	September 2011
Detection of U(VI) on the surface of altered depleted uranium by time-resolved laser-induced fluorescence spectroscopy (TRLFS) Baumann, N.; Arnold, T.; Geipel, G. Science of The Total Environment, Vol. 366, Issue 2-3 https://doi.org/10.1016/j.scitotenv.2005.09.093	journal	August 2006
Determination of the number of factors and the experimental error in a data matrix Malinowski, Edmund R. Analytical Chemistry, Vol. 49, Issue 4 https://doi.org/10.1021/ac50012a027	journal	April 1977
Mechanisms of Uranium Interactions with Hydroxyapatite: Implications for Groundwater Remediation Fuller, C. C.; Bargar, J. R.; Davis, J. A. Environmental Science & Technology, Vol. 36, Issue 2 https://doi.org/10.1021/es0108483	journal	January 2002
Molecular-Scale Characterization of Uranium Sorption by Bone Apatite Materials for a Permeable Reactive Barrier Demonstration Fuller, C. C.; Bargar, J. R.; Davis, J. A. Environmental Science & Technology, Vol. 37, Issue 20 https://doi.org/10.1021/es0343959	journal	October 2003
Oxidative Dissolution of Biogenic Uraninite in Groundwater at Old Rifle, CO Campbell, Kate M.; Veeramani, Harish; Ulrich, Kai-Uwe Environmental Science & Technology, Vol. 45, Issue 20 https://doi.org/10.1021/es200482f	journal	October 2011
Contaminant Uranium Phases and Leaching at the Fernald Site in Ohio Buck, Edgar C.; Brown, Neil R.; Dietz, Nancy L. Environmental Science & Technology, Vol. 30, Issue 1 https://doi.org/10.1021/es9500825	journal	January 1996
Immobilization of Uranium in Contaminated Sediments by Hydroxyapatite Addition Arey, J. Samuel; Seaman, John C.; Bertsch, Paul M. Environmental Science & Technology, Vol. 33, Issue 2 https://doi.org/10.1021/es980425+	journal	December 1998
Comparative Analysis of Soluble Phosphate Amendments for the Remediation of Heavy Metal Contaminants: Effect on Sediment Hydraulic Conductivity Wellman, Dawn M.; Icenhower, Jonathan P.; Owen, Antoinette T. Environmental Chemistry, Vol. 3, Issue 3 https://doi.org/10.1071/EN05023	journal	January 2006
Sequestration and retention of uranium(VI) in the presence of hydroxylapatite under dynamic geochemical conditions Wellman, Dawn M.; Glovack, Julia N.; Parker, Kent Environmental Chemistry, Vol. 5, Issue 1 https://doi.org/10.1071/EN07060	journal	January 2008
Nonreductive Biomineralization of Uranium(VI) Phosphate Via Microbial Phosphatase Activity in Anaerobic Conditions Beazley, Melanie J.; Martinez, Robert J.; Sobecky, Patricia A. Geomicrobiology Journal, Vol. 26, Issue 7 https://doi.org/10.1080/01490450903060780	journal	September 2009
Polarized x-ray-absorption spectroscopy of the uranyl ion: Comparison of experiment and theory Hudson, E. A.; Allen, P. G.; Terminello, L. J. Physical Review B, Vol. 54, Issue 1 https://doi.org/10.1103/PhysRevB.54.156	journal	July 1996
Relativistic calculations of spin-dependent x-ray-absorption spectra Ankudinov, A. L.; Rehr, J. J. Physical Review B, Vol. 56, Issue 4 https://doi.org/10.1103/PhysRevB.56.R1712	journal	July 1997
IFEFFIT : interactive XAFS analysis and FEFF fitting Newville, Matthew Journal of Synchrotron Radiation, Vol. 8, Issue 2 https://doi.org/10.1107/S0909049500016964	journal	March 2001
ATHENA , ARTEMIS , HEPHAESTUS : data analysis for X-ray absorption spectroscopy using IFEFFIT Ravel, B.; Newville, M. Journal of Synchrotron Radiation, Vol. 12, Issue 4 https://doi.org/10.1107/S0909049505012719	journal	June 2005
XAFS and micro-XAFS at the PNC-CAT beamlines Heald, S. M.; Brewe, D. L.; Stern, E. A. Journal of Synchrotron Radiation, Vol. 6, Issue 3 https://doi.org/10.1107/S090904959801677X	journal	May 1999
EXAFS and principal component analysis: a new shell game Wasserman, S. R.; Allen, P. G.; Shuh, D. K. Journal of Synchrotron Radiation, Vol. 6, Issue 3 https://doi.org/10.1107/S0909049599000965	journal	May 1999
SIXPack a Graphical User Interface for XAS Analysis Using IFEFFIT Webb, S. M. Physica Scripta https://doi.org/10.1238/Physica.Topical.115a01011	journal	January 2005
Synthesis and characterization of sodium meta-autunite, Na[UO2PO4]·3H2O Wellman, D. M.; Catalano, J. G.; Icenhower, J. P. Radiochimica Acta, Vol. 93, Issue 7 https://doi.org/10.1524/ract.2005.93.7.393	journal	January 2005
XAFS spectroscopic study of uranyl coordination in solids and aqueous solution Thompson, Hillary A.; Brown, Gordon E.; Parks, George A. American Mineralogist, Vol. 82, Issue 5-6 https://doi.org/10.2138/am-1997-5-607	journal	June 1997
Mobility of uranium during weathering Murakami, Takashi; Ohnuki, Toshihiko; Isobe, Hiroshi American Mineralogist, Vol. 82, Issue 9-10 https://doi.org/10.2138/am-1997-9-1006	journal	October 1997
The crystal structure of synthetic autunite, Ca[(UO ₂ )(PO ₄ )] ₂ (H ₂ O) ₁₁ Locock, Andrew J.; Burns, Peter C. American Mineralogist, Vol. 88, Issue 1 https://doi.org/10.2138/am-2003-0128	journal	January 2003
Analysis of uranyl-bearing phases by EXAFS spectroscopy: Interferences, multiple scattering, accuracy of structural parameters, and spectral differences Catalano, Jeffrey G.; Brown, Gordon E. American Mineralogist, Vol. 89, Issue 7 https://doi.org/10.2138/am-2004-0711	journal	July 2004
Quantitative Speciation of Heavy Metals in Soils and Sediments by Synchrotron X-ray Techniques Manceau, A.; Marcus, M. A.; Tamura, N. Reviews in Mineralogy and Geochemistry, Vol. 49, Issue 1 https://doi.org/10.2138/gsrmg.49.1.341	journal	January 2002
300 Area Uranium Stabilization Through Polyphosphate Injection: Final Report Vermeul, Vincent R.; Bjornstad, Bruce N.; Fritz, Brad G. https://doi.org/10.2172/967237	report	June 2009

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Effect of Reaction Pathway on the Extent and Mechanism of Uranium(VI) Immobilization with Calcium and Phosphate

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