Publisher's Note: High-temperature superconductivity stabilized by electron-hole interband coupling in collapsed tetragonal phase of under high pressure [Phys. Rev. B 91 , 060508(R) (2015)]
- Univ. of Maryland, College Park, MD (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Here, we report a high-pressure study of simultaneous low-temperature electrical resistivity and Hall effect measurements on high quality single-crystalline KFe2As2 using designer diamond anvil cell techniques with applied pressures up to 33 GPa. In the low pressure regime, we show that the superconducting transition temperature Tc finds a maximum onset value of 7 K near 2 GPa, in contrast to previous reports that find a minimum Tc and reversal of pressure dependence at this pressure. Upon applying higher pressures, this Tc is diminished until a sudden drastic enhancement occurs coincident with a first-order structural phase transition into a collapsed tetragonal phase. The appearance of a distinct superconducting phase above 13 GPa is also accompanied by a sudden reversal of dominant charge carrier sign, from hole- to electron-like, which agrees with our band calculations predicting the emergence of an electron pocket and diminishment of hole pockets upon Fermi surface reconstruction. Our results suggest the high-temperature superconducting phase in KFe2As2 is substantially enhanced by the presence of nested electron and hole pockets, providing the key ingredient of high-Tc superconductivity in iron pnictide superconductors.
- Research Organization:
- Carnegie Institution of Washington, Washington, D.C. (United States)
- Sponsoring Organization:
- USDOE National Nuclear Security Administration (NNSA)
- Grant/Contract Number:
- NA0002006
- OSTI ID:
- 1335147
- Journal Information:
- Physical Review. B, Condensed Matter and Materials Physics, Vol. 91, Issue 9; ISSN 1098-0121
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
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