Diffractive imaging of coherent nuclear motion in isolated molecules

Yang, Jie; Guehr, Markus; Shen, Xiaozhe; Li, Renkai; Vecchione, Theodore; Coffee, Ryan; Corbett, Jeff; Fry, Alan; Hartmann, Nick; Hast, Carsten; Hegazy, Kareem; Jobe, Keith; Makasyuk, Igor; Robinson, Joseph; Robinson, Matthew S.; Vetter, Sharon; Weathersby, Stephen; Yoneda, Charles; Wang, Xijie; Centurion, Martin

doi:10.1103/PhysRevLett.117.153002

Title: Diffractive imaging of coherent nuclear motion in isolated molecules

Journal Article · Mon Oct 03 00:00:00 EDT 2016 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.117.153002· OSTI ID:1331204

Yang, Jie ^[1]; Guehr, Markus ^[2]; Shen, Xiaozhe ^[3]; Li, Renkai ^[3]; Vecchione, Theodore ^[3]; Coffee, Ryan ^[3]; Corbett, Jeff ^[3]; Fry, Alan ^[3]; Hartmann, Nick ^[3]; Hast, Carsten ^[3]; Hegazy, Kareem ^[3]; Jobe, Keith ^[3]; Makasyuk, Igor ^[3]; Robinson, Joseph ^[3]; Robinson, Matthew S. ^[1]; Vetter, Sharon ^[3]; Weathersby, Stephen ^[3]; Yoneda, Charles ^[3]; Wang, Xijie ^[3]; Centurion, Martin ^[1]

Univ. of Nebraska-Lincoln, Lincoln, NE (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Potsdam Univ., Potsdam (Germany)
SLAC National Accelerator Lab., Menlo Park, CA (United States)

Observing the motion of the nuclear wave packets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational wave packet in isolated iodine molecules using ultrafast electron diffraction with relativistic electrons. The time-varying interatomic distance was measured with a precision 0.07 Å and temporal resolution of 230 fs full width at half maximum. As a result, the method is not only sensitive to the position but also the shape of the nuclear wave packet.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-76SF00515; SC0014170; IIA-1430519

OSTI ID:: 1331204

Alternate ID(s):: OSTI ID: 1328470; OSTI ID: 1348858

Report Number(s):: SLAC-PUB-16860; PRLTAO; TRN: US1601861

Journal Information:: Physical Review Letters, Vol. 117, Issue 15; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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