Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Ground state of underdoped cuprates in vicinity of superconductor-to-insulator transition

Journal Article · · Journal of Superconductivity and Novel Magnetism
 [1];  [1];  [2];  [3]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States); Chinese Academy of Sciences, Beijing (China)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States); Yale Univ., New Haven, CT (United States)
When an insulating underdoped cuprate is doped beyond a critical concentration (xc), high-temperature superconductivity emerges. We have synthesized a series of La2–xSrxCuO4 (LSCO) samples using the combinatorial spread technique that allows us to traverse the superconductor-to-insulator transition (SIT) in extremely fine doping steps, Δx≈0.00008. We have measured the Hall resistivity (ρH) as a function of temperature down to 300 mK in magnetic fields up to 9 T. At very low temperatures, ρH shows an erratic behavior, jumps and fluctuations exceeding 100%, hysteresis, and memory effects, indicating that the insulating ground state is a charge-cluster glass (CCG). Furthermore, based on the phase diagram depicted in our experiment, we propose a unified picture to account for the anomalous electric transport in the vicinity of the SIT, suggesting that the CCG is in fact a disordered and glassy version of the charge density wave.
Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI ID:
1324274
Report Number(s):
BNL--112538-2016-JA; KC0203020
Journal Information:
Journal of Superconductivity and Novel Magnetism, Journal Name: Journal of Superconductivity and Novel Magnetism; ISSN 1557-1939
Publisher:
SpringerCopyright Statement
Country of Publication:
United States
Language:
English

References (25)

Emergence of superconductivity from the dynamically heterogeneous insulating state in La2−xSrxCuO4 journal November 2012
Fluctuating charge-density waves in a cuprate superconductor journal February 2013
Anomalous independence of interface superconductivity from carrier density journal August 2013
Charge-density-wave origin of cuprate checkerboard visualized by scanning tunnelling microscopy journal July 2008
Direct observation of competition between superconductivity and charge density wave order in YBa2Cu3O6.67 journal October 2012
Inelastic X-ray scattering in YBa2Cu3O6.6 reveals giant phonon anomalies and elastic central peak due to charge-density-wave formation journal November 2013
Combinatorial measurements of Hall effect and resistivity in oxide films journal March 2008
Perspective: Extremely fine tuning of doping enabled by combinatorial molecular-beam epitaxy journal June 2015
Hall effect in quantum critical charge-cluster glass journal April 2016
Normal-state Hall effect and the insulating resistivity of high- T c cuprates at low temperatures journal October 1997
Spin-glass state of individual magnetic vortices in Y Ba 2 Cu 3 O y and La 2 − x Sr x Cu O 4 below the metal-to-insulator crossover journal August 2007
Photoinduced expansion of cuprate superconductors: Evidence of strong electron-lattice coupling journal March 2008
Magnetic phase diagram of low-doped La 2 − x Sr x CuO 4 thin films studied by low-energy muon-spin rotation journal August 2013
Evidence for Charge Glasslike Behavior in Lightly Doped La 2 − x Sr x CuO 4 at Low Temperatures journal October 2008
Electron-Phonon Interactions in Superconducting La 1.84 Sr 0.16 CuO 4 Films journal December 2008
Logarithmic Divergence of both In-Plane and Out-of-Plane Normal-State Resistivities of Superconducting La 2 − x Sr x Cu O 4 in the Zero-Temperature Limit journal December 1995
Charge Segregation, Cluster Spin Glass, and Superconductivity in La 1.94 Sr 0.06 CuO 4 journal July 1999
Metal-to-Insulator Crossover in the Low-Temperature Normal State of Bi 2 Sr 2 − x La x CuO 6 + δ journal July 2000
Unusual Magnetic Susceptibility Anisotropy in Untwinned La 2 − x Sr x CuO 4 Single Crystals in the Lightly Doped Region journal June 2001
Doping a Mott insulator: Physics of high-temperature superconductivity journal January 2006
Local Ordering in the Pseudogap State of the High-Tc Superconductor Bi2Sr2CaCu2O8+  journal March 2004
An Intrinsic Bond-Centered Electronic Glass with Unidirectional Domains in Underdoped Cuprates journal March 2007
Nonequilibrium Phase Transitions in Cuprates Observed by Ultrafast Electron Crystallography journal April 2007
Long-Range Incommensurate Charge Fluctuations in (Y,Nd)Ba2Cu3O6+x journal July 2012
Ubiquitous Interplay Between Charge Ordering and High-Temperature Superconductivity in Cuprates journal December 2013

Similar Records

Unusual Superconducting State of Underdoped Cuprates
Journal Article · Thu May 01 00:00:00 EDT 1997 · Physical Review Letters · OSTI ID:509069

Gapped commensurate antiferromagnetic response in a strongly underdoped model cuprate superconductor
Journal Article · Tue Aug 19 20:00:00 EDT 2025 · npj Quantum Materials · OSTI ID:2584516