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Electronic structure of the chiral helimagnet and 3d-intercalated transition metal dichalcogenide Cr1/3NbS2

Journal Article · · Physical Review B
 [1];  [2];  [3];  [4];  [3];  [1];  [1];  [5];  [6];  [7];  [3];  [1];  [1];  [1];  [8];  [9];  [1]
  1. Univ. of Tennessee, Knoxville, TN (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  3. Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy)
  4. Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy); Elettra Sincrotrone Trieste, Basovizza (Italy)
  5. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science (CNMS)
  6. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
  7. Institute of Materials Workshop (IOM), CNR Laboratory, Trieste (Italy); International Centre for Theoretical Physics, Strada Costiera, Trieste (Italy)
  8. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  9. Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
+ Show Author Affiliations
The electronic structure of the chiral helimagnet Cr1/3NbS2 has been studied with core level and angle-resolved photoemission spectroscopy (ARPES). Intercalated Cr atoms are found to be effective in donating electrons to the NbS2 layers but also cause significant modifications of the electronic structure of the host NbS2 material. Specifically, the data provide evidence that a description of the electronic structure of Cr1/3NbS2 on the basis of a simple rigid band picture is untenable. The data also reveal substantial inconsistencies with the predictions of standard density functional theory. In conclusion, the relevance of these results to the attainment of a correct description of the electronic structure of chiral helimagnets, magnetic thin films/multilayers, and transition metal dichalcogenides intercalated with 3d magnetic elements is discussed.
Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); National Science Foundation (NSF)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1311264
Alternate ID(s):
OSTI ID: 1298342
OSTI ID: 1393070
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 7 Vol. 94; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (2)

Critical phenomenon and phase diagram of Mn-intercalated layered MnNb 3 S 6 journal March 2019
Tricritical point and phase diagram based on critical scaling in the monoaxial chiral helimagnet Cr 1 / 3 NbS 2 journal September 2017

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