Intrinsic quantum anomalous Hall effect in the kagome lattice Cs 2LiMn 3F 12
Abstract
In a kagome lattice, the time reversal symmetry can be broken by a staggered magnetic flux emerging from ferromagnetic ordering and intrinsic spin-orbit coupling, leading to several well-separated nontrivial Chern bands and intrinsic quantum anomalous Hall effect. Based on this idea and ab initio calculations, we propose the realization of the intrinsic quantum anomalous Hall effect in the single layer Cs 2Mn 3F 12 kagome lattice and on the (001) surface of a Cs 2LiMn 3F 12 single crystal by modifying the carrier coverage on it, where the band gap is around 20 meV. Furthermore, a simplified tight binding model based on the in-plane ddσ antibonding states is constructed to understand the topological band structures of the system.
- Authors:
-
- Stanford Univ., Stanford, CA (United States). Dept. of Physics
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1263391
- Alternate Identifier(s):
- OSTI ID: 1224374
- Report Number(s):
- SLAC-PUB-16645
Journal ID: ISSN 0031-9007; PRLTAO; arXiv:1507.04043
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 115; Journal Issue: 18; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; MATSCI
Citation Formats
Xu, Gang, Lian, Biao, and Zhang, Shou -Cheng. Intrinsic quantum anomalous Hall effect in the kagome lattice Cs2LiMn3F12. United States: N. p., 2015.
Web. doi:10.1103/PhysRevLett.115.186802.
Xu, Gang, Lian, Biao, & Zhang, Shou -Cheng. Intrinsic quantum anomalous Hall effect in the kagome lattice Cs2LiMn3F12. United States. doi:10.1103/PhysRevLett.115.186802.
Xu, Gang, Lian, Biao, and Zhang, Shou -Cheng. Tue .
"Intrinsic quantum anomalous Hall effect in the kagome lattice Cs2LiMn3F12". United States. doi:10.1103/PhysRevLett.115.186802. https://www.osti.gov/servlets/purl/1263391.
@article{osti_1263391,
title = {Intrinsic quantum anomalous Hall effect in the kagome lattice Cs2LiMn3F12},
author = {Xu, Gang and Lian, Biao and Zhang, Shou -Cheng},
abstractNote = {In a kagome lattice, the time reversal symmetry can be broken by a staggered magnetic flux emerging from ferromagnetic ordering and intrinsic spin-orbit coupling, leading to several well-separated nontrivial Chern bands and intrinsic quantum anomalous Hall effect. Based on this idea and ab initio calculations, we propose the realization of the intrinsic quantum anomalous Hall effect in the single layer Cs2Mn3F12 kagome lattice and on the (001) surface of a Cs2LiMn3F12 single crystal by modifying the carrier coverage on it, where the band gap is around 20 meV. Furthermore, a simplified tight binding model based on the in-plane ddσ antibonding states is constructed to understand the topological band structures of the system.},
doi = {10.1103/PhysRevLett.115.186802},
journal = {Physical Review Letters},
issn = {0031-9007},
number = 18,
volume = 115,
place = {United States},
year = {2015},
month = {10}
}
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Works referenced in this record:
Metal-Insulator Transition of Fermions on a Kagome Lattice at 1/3 Filling
journal, May 2010
- Nishimoto, Satoshi; Nakamura, Masaaki; O’Brien, Aroon
- Physical Review Letters, Vol. 104, Issue 19
Zur Elektronentheorie der Metalle. I
journal, January 1931
- Nordheim, Lothar
- Annalen der Physik, Vol. 401, Issue 5
Soft self-consistent pseudopotentials in a generalized eigenvalue formalism
journal, April 1990
- Vanderbilt, David
- Physical Review B, Vol. 41, Issue 11, p. 7892-7895
Dynamical axion field in topological magnetic insulators
journal, March 2010
- Li, Rundong; Wang, Jing; Qi, Xiao-Liang
- Nature Physics, Vol. 6, Issue 4
Scale-Invariant Quantum Anomalous Hall Effect in Magnetic Topological Insulators beyond the Two-Dimensional Limit
journal, September 2014
- Kou, Xufeng; Guo, Shih-Ting; Fan, Yabin
- Physical Review Letters, Vol. 113, Issue 13
Quantum anomalous Hall effect in graphene from Rashba and exchange effects
journal, October 2010
- Qiao, Zhenhua; Yang, Shengyuan A.; Feng, Wanxiang
- Physical Review B, Vol. 82, Issue 16
Chern Semimetal and the Quantized Anomalous Hall Effect in
journal, October 2011
- Xu, Gang; Weng, Hongming; Wang, Zhijun
- Physical Review Letters, Vol. 107, Issue 18
Chern insulator at a magnetic rocksalt interface
journal, September 2014
- Garrity, Kevin F.; Vanderbilt, David
- Physical Review B, Vol. 90, Issue 12
Topological insulators from complex orbital order in transition-metal oxides heterostructures
journal, November 2011
- Rüegg, Andreas; Fiete, Gregory A.
- Physical Review B, Vol. 84, Issue 20
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996
- Kresse, G.; Furthmüller, J.
- Physical Review B, Vol. 54, Issue 16, p. 11169-11186
Observation of the Zero Hall Plateau in a Quantum Anomalous Hall Insulator
journal, September 2015
- Feng, Yang; Feng, Xiao; Ou, Yunbo
- Physical Review Letters, Vol. 115, Issue 12
Valley-Polarized Metals and Quantum Anomalous Hall Effect in Silicene
journal, August 2012
- Ezawa, Motohiko
- Physical Review Letters, Vol. 109, Issue 5
Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet
journal, September 2000
- Ohgushi, Kenya; Murakami, Shuichi; Nagaosa, Naoto
- Physical Review B, Vol. 62, Issue 10
Quantum Anomalous Hall Effect with Higher Plateaus
journal, September 2013
- Wang, Jing; Lian, Biao; Zhang, Haijun
- Physical Review Letters, Vol. 111, Issue 13
Anomalous Edge Transport in the Quantum Anomalous Hall State
journal, August 2013
- Wang, Jing; Lian, Biao; Zhang, Haijun
- Physical Review Letters, Vol. 111, Issue 8
Interface engineering of quantum Hall effects in digital transition metal oxide heterostructures
journal, September 2011
- Xiao, Di; Zhu, Wenguang; Ran, Ying
- Nature Communications, Vol. 2, Issue 1
General theorem relating the bulk topological number to edge states in two-dimensional insulators
journal, July 2006
- Qi, Xiao-Liang; Wu, Yong-Shi; Zhang, Shou-Cheng
- Physical Review B, Vol. 74, Issue 4
Spontaneous symmetry breaking in a two-dimensional kagome lattice
journal, July 2010
- Liu, Qin; Yao, Hong; Ma, Tianxing
- Physical Review B, Vol. 82, Issue 4
Universal scaling of the quantum anomalous Hall plateau transition
journal, February 2014
- Wang, Jing; Lian, Biao; Zhang, Shou-Cheng
- Physical Review B, Vol. 89, Issue 8
Quantum Spin Hall Effect in Graphene
journal, November 2005
- Kane, C. L.; Mele, E. J.
- Physical Review Letters, Vol. 95, Issue 22
High-Temperature Fractional Quantum Hall States
journal, June 2011
- Tang, Evelyn; Mei, Jia-Wei; Wen, Xiao-Gang
- Physical Review Letters, Vol. 106, Issue 23
High-precision realization of robust quantum anomalous Hall state in a hard ferromagnetic topological insulator
journal, March 2015
- Chang, Cui-Zu; Zhao, Weiwei; Kim, Duk Y.
- Nature Materials, Vol. 14, Issue 5
Maximally localized generalized Wannier functions for composite energy bands
journal, November 1997
- Marzari, Nicola; Vanderbilt, David
- Physical Review B, Vol. 56, Issue 20
Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator
journal, March 2013
- Chang, C. -Z.; Zhang, J.; Feng, X.
- Science, Vol. 340, Issue 6129
Quantum Anomalous Hall Effect in Quantum Wells
journal, October 2008
- Liu, Chao-Xing; Qi, Xiao-Liang; Dai, Xi
- Physical Review Letters, Vol. 101, Issue 14
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Topological field theory of time-reversal invariant insulators
journal, November 2008
- Qi, Xiao-Liang; Hughes, Taylor L.; Zhang, Shou-Cheng
- Physical Review B, Vol. 78, Issue 19, Article No. 195424
Electrically Tunable Quantum Anomalous Hall Effect in Graphene Decorated by Transition-Metal Adatoms
journal, February 2012
- Zhang, Hongbin; Lazo, Cesar; Blügel, Stefan
- Physical Review Letters, Vol. 108, Issue 5
Proximity-Induced Ferromagnetism in Graphene Revealed by the Anomalous Hall Effect
journal, January 2015
- Wang, Zhiyong; Tang, Chi; Sachs, Raymond
- Physical Review Letters, Vol. 114, Issue 1
Trajectory of the anomalous Hall effect towards the quantized state in a ferromagnetic topological insulator
journal, August 2014
- Checkelsky, J. G.; Yoshimi, R.; Tsukazaki, A.
- Nature Physics, Vol. 10, Issue 10
Topological States in Ferromagnetic CdO/EuO Superlattices and Quantum Wells
journal, March 2014
- Zhang, Haijun; Wang, Jing; Xu, Gang
- Physical Review Letters, Vol. 112, Issue 9
Inhomogeneous Electron Gas
journal, March 1973
- Rajagopal, A. K.; Callaway, J.
- Physical Review B, Vol. 7, Issue 5
A Structurally Perfect S = 1 / 2 Kagomé Antiferromagnet
journal, October 2005
- Shores, Matthew P.; Nytko, Emily A.; Bartlett, Bart M.
- Journal of the American Chemical Society, Vol. 127, Issue 39
Model for a Quantum Hall Effect without Landau Levels: Condensed-Matter Realization of the "Parity Anomaly"
journal, October 1988
- Haldane, F. D. M.
- Physical Review Letters, Vol. 61, Issue 18
Narrowing of Topological Bands due to Electronic Orbital Degrees of Freedom
journal, September 2011
- Venderbos, Jörn W. F.; Daghofer, Maria; van den Brink, Jeroen
- Physical Review Letters, Vol. 107, Issue 11
Maximally localized Wannier functions for entangled energy bands
journal, December 2001
- Souza, Ivo; Marzari, Nicola; Vanderbilt, David
- Physical Review B, Vol. 65, Issue 3
First-principles determination of Heisenberg Hamiltonian parameters for the spin- kagome antiferromagnet ZnCu (OH) Cl
journal, August 2013
- Jeschke, Harald O.; Salvat-Pujol, Francesc; Valentí, Roser
- Physical Review B, Vol. 88, Issue 7
Jahn-Teller ordering in Kagomé-type layers of compounds A2A′Mn3IIIF12 (ARb, Cs; A′Li, Na, K)
journal, January 1997
- Englich, Ulrich; Frommen, Christoph; Massa, Werner
- Journal of Alloys and Compounds, Vol. 246, Issue 1-2
Quantum Anomalous Hall Effect in Graphene Proximity Coupled to an Antiferromagnetic Insulator
journal, March 2014
- Qiao, Zhenhua; Ren, Wei; Chen, Hua
- Physical Review Letters, Vol. 112, Issue 11
Prediction of a Two-Dimensional Organic Topological Insulator
journal, May 2013
- Wang, Z. F.; Su, Ninghai; Liu, Feng
- Nano Letters, Vol. 13, Issue 6, p. 2842-2845
Ab initiomolecular dynamics for liquid metals
journal, January 1993
- Kresse, G.; Hafner, J.
- Physical Review B, Vol. 47, Issue 1, p. 558-561
Virtual crystal approximation revisited: Application to dielectric and piezoelectric properties of perovskites
journal, March 2000
- Bellaiche, L.; Vanderbilt, David
- Physical Review B, Vol. 61, Issue 12
Quantized Anomalous Hall Effect in Magnetic Topological Insulators
journal, June 2010
- Yu, R.; Zhang, W.; Zhang, H. -J.
- Science, Vol. 329, Issue 5987
Structural distortion and magnetism in transition metal oxides: crucial roles of orbital degrees of freedom
journal, March 2002
- Fang, Zhong; Terakura, Kiyoyuki
- Journal of Physics: Condensed Matter, Vol. 14, Issue 11
Highly convergent schemes for the calculation of bulk and surface Green functions
journal, April 1985
- Sancho, M. P. Lopez; Sancho, J. M. Lopez; Sancho, J. M. L.
- Journal of Physics F: Metal Physics, Vol. 15, Issue 4
Quantum Anomalous Hall Effect in Magnetic Insulator Heterostructure
journal, February 2015
- Xu, Gang; Wang, Jing; Felser, Claudia
- Nano Letters, Vol. 15, Issue 3
Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965
- Kohn, W.; Sham, L. J.
- Physical Review, Vol. 140, Issue 4A, p. A1133-A1138
Model for a Quantum Hall Effect without Landau Levels: Condensed-Matter Realization of the "Parity Anomaly"
journal, October 1988
- Haldane, F. D. M.
- Physical Review Letters, Vol. 61, Issue 18
General theorem relating the bulk topological number to edge states in two-dimensional insulators
journal, July 2006
- Qi, Xiao-Liang; Wu, Yong-Shi; Zhang, Shou-Cheng
- Physical Review B, Vol. 74, Issue 4
Topological field theory of time-reversal invariant insulators
journal, November 2008
- Qi, Xiao-Liang; Hughes, Taylor L.; Zhang, Shou-Cheng
- Physical Review B, Vol. 78, Issue 19, Article No. 195424
Quantum Anomalous Hall Effect in Quantum Wells
journal, October 2008
- Liu, Chao-Xing; Qi, Xiao-Liang; Dai, Xi
- Physical Review Letters, Vol. 101, Issue 14
Chern Semimetal and the Quantized Anomalous Hall Effect in
journal, October 2011
- Xu, Gang; Weng, Hongming; Wang, Zhijun
- Physical Review Letters, Vol. 107, Issue 18
Topological insulators from complex orbital order in transition-metal oxides heterostructures
journal, November 2011
- Rüegg, Andreas; Fiete, Gregory A.
- Physical Review B, Vol. 84, Issue 20
Quantum Anomalous Hall Effect with Higher Plateaus
journal, September 2013
- Wang, Jing; Lian, Biao; Zhang, Haijun
- Physical Review Letters, Vol. 111, Issue 13
Anomalous Edge Transport in the Quantum Anomalous Hall State
journal, August 2013
- Wang, Jing; Lian, Biao; Zhang, Haijun
- Physical Review Letters, Vol. 111, Issue 8
Topological States in Ferromagnetic CdO/EuO Superlattices and Quantum Wells
journal, March 2014
- Zhang, Haijun; Wang, Jing; Xu, Gang
- Physical Review Letters, Vol. 112, Issue 9
Chern insulator at a magnetic rocksalt interface
journal, September 2014
- Garrity, Kevin F.; Vanderbilt, David
- Physical Review B, Vol. 90, Issue 12
Universal scaling of the quantum anomalous Hall plateau transition
journal, February 2014
- Wang, Jing; Lian, Biao; Zhang, Shou-Cheng
- Physical Review B, Vol. 89, Issue 8
Scale-Invariant Quantum Anomalous Hall Effect in Magnetic Topological Insulators beyond the Two-Dimensional Limit
journal, September 2014
- Kou, Xufeng; Guo, Shih-Ting; Fan, Yabin
- Physical Review Letters, Vol. 113, Issue 13
Observation of the Zero Hall Plateau in a Quantum Anomalous Hall Insulator
journal, September 2015
- Feng, Yang; Feng, Xiao; Ou, Yunbo
- Physical Review Letters, Vol. 115, Issue 12
Quantum anomalous Hall effect in graphene from Rashba and exchange effects
journal, October 2010
- Qiao, Zhenhua; Yang, Shengyuan A.; Feng, Wanxiang
- Physical Review B, Vol. 82, Issue 16
Electrically Tunable Quantum Anomalous Hall Effect in Graphene Decorated by Transition-Metal Adatoms
journal, February 2012
- Zhang, Hongbin; Lazo, Cesar; Blügel, Stefan
- Physical Review Letters, Vol. 108, Issue 5
Valley-Polarized Metals and Quantum Anomalous Hall Effect in Silicene
journal, August 2012
- Ezawa, Motohiko
- Physical Review Letters, Vol. 109, Issue 5
Quantum Anomalous Hall Effect in Graphene Proximity Coupled to an Antiferromagnetic Insulator
journal, March 2014
- Qiao, Zhenhua; Ren, Wei; Chen, Hua
- Physical Review Letters, Vol. 112, Issue 11
Proximity-Induced Ferromagnetism in Graphene Revealed by the Anomalous Hall Effect
journal, January 2015
- Wang, Zhiyong; Tang, Chi; Sachs, Raymond
- Physical Review Letters, Vol. 114, Issue 1
Spin anisotropy and quantum Hall effect in the kagomé lattice: Chiral spin state based on a ferromagnet
journal, September 2000
- Ohgushi, Kenya; Murakami, Shuichi; Nagaosa, Naoto
- Physical Review B, Vol. 62, Issue 10
Jahn-Teller ordering in Kagomé-type layers of compounds A2A′Mn3IIIF12 (ARb, Cs; A′Li, Na, K)
journal, January 1997
- Englich, Ulrich; Frommen, Christoph; Massa, Werner
- Journal of Alloys and Compounds, Vol. 246, Issue 1-2
High-Temperature Fractional Quantum Hall States
journal, June 2011
- Tang, Evelyn; Mei, Jia-Wei; Wen, Xiao-Gang
- Physical Review Letters, Vol. 106, Issue 23
Narrowing of Topological Bands due to Electronic Orbital Degrees of Freedom
journal, September 2011
- Venderbos, Jörn W. F.; Daghofer, Maria; van den Brink, Jeroen
- Physical Review Letters, Vol. 107, Issue 11
Metal-Insulator Transition of Fermions on a Kagome Lattice at 1/3 Filling
journal, May 2010
- Nishimoto, Satoshi; Nakamura, Masaaki; O’Brien, Aroon
- Physical Review Letters, Vol. 104, Issue 19
Spontaneous symmetry breaking in a two-dimensional kagome lattice
journal, July 2010
- Liu, Qin; Yao, Hong; Ma, Tianxing
- Physical Review B, Vol. 82, Issue 4
Inhomogeneous Electron Gas
journal, November 1964
- Hohenberg, P.; Kohn, W.
- Physical Review, Vol. 136, Issue 3B, p. B864-B871
Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965
- Kohn, W.; Sham, L. J.
- Physical Review, Vol. 140, Issue 4A, p. A1133-A1138
Soft self-consistent pseudopotentials in a generalized eigenvalue formalism
journal, April 1990
- Vanderbilt, David
- Physical Review B, Vol. 41, Issue 11, p. 7892-7895
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Virtual crystal approximation revisited: Application to dielectric and piezoelectric properties of perovskites
journal, March 2000
- Bellaiche, L.; Vanderbilt, David
- Physical Review B, Vol. 61, Issue 12
Ab initiomolecular dynamics for liquid metals
journal, January 1993
- Kresse, G.; Hafner, J.
- Physical Review B, Vol. 47, Issue 1, p. 558-561
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996
- Kresse, G.; Furthmüller, J.
- Physical Review B, Vol. 54, Issue 16, p. 11169-11186
First-principles determination of Heisenberg Hamiltonian parameters for the spin- kagome antiferromagnet ZnCu (OH) Cl
journal, August 2013
- Jeschke, Harald O.; Salvat-Pujol, Francesc; Valentí, Roser
- Physical Review B, Vol. 88, Issue 7
Quantum Spin Hall Effect in Graphene
journal, November 2005
- Kane, C. L.; Mele, E. J.
- Physical Review Letters, Vol. 95, Issue 22
Maximally localized generalized Wannier functions for composite energy bands
journal, November 1997
- Marzari, Nicola; Vanderbilt, David
- Physical Review B, Vol. 56, Issue 20
Maximally localized Wannier functions for entangled energy bands
journal, December 2001
- Souza, Ivo; Marzari, Nicola; Vanderbilt, David
- Physical Review B, Vol. 65, Issue 3
Works referencing / citing this record:
Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal
journal, July 2018
- Liu, Enke; Sun, Yan; Kumar, Nitesh
- Nature Physics, Vol. 14, Issue 11
Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet
journal, September 2018
- Yin, Jia-Xin; Zhang, Songtian S.; Li, Hang
- Nature, Vol. 562, Issue 7725
Highly-ordered wide bandgap materials for quantized anomalous Hall and magnetoelectric effects
journal, April 2017
- Otrokov, M. M.; Menshchikova, T. V.; Vergniory, M. G.
- 2D Materials, Vol. 4, Issue 2
Topological semimetal in honeycomb lattice LnSI
journal, September 2017
- Nie, Simin; Xu, Gang; Prinz, Fritz B.
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 40
Monolayer of the transition metal trichloride : A playground for two-dimensional magnetism, room-temperature quantum anomalous Hall effect, and topological phase transitions
journal, May 2017
- Sheng, Xian-Lei; Nikolić, Branislav K.
- Physical Review B, Vol. 95, Issue 20
Dirac fermions and flat bands in the ideal kagome metal FeSn
journal, December 2019
- Kang, Mingu; Ye, Linda; Fang, Shiang
- Nature Materials, Vol. 19, Issue 2
Intrinsic Dirac half-metal and quantum anomalous Hall phase in a hexagonal metal-oxide lattice
journal, November 2017
- Zhang, Shou-juan; Zhang, Chang-wen; Zhang, Shu-feng
- Physical Review B, Vol. 96, Issue 20
Massive Dirac fermions in a ferromagnetic kagome metal
journal, March 2018
- Ye, Linda; Kang, Mingu; Liu, Junwei
- Nature, Vol. 555, Issue 7698