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{ital Ab} {ital initio} characterization of the low-lying vibrations of HCO (DCO) in the {ital {tilde B}} {sup 2}{ital A}{prime} state

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.470289· OSTI ID:124790
;  [1];  [2]
  1. Department of Chemistry and Cherry L. Emerson Center for Scientific Computation, Emory University, Atlanta, Georgia 30322 (United States)
  2. U.S. Army Research Laboratory, AMSRL-WT-PC, Aberdeen Proving Ground, Maryland 21005 (United States)
We report a force field for HCO in the {ital {tilde B}} {sup 2}{ital A}{prime} electronic state, based on {ital ab} {ital initio} electronic energies obtained using state-averaged multiconfiguration-self-consistent field/configuration interaction wave functions. The force field is used in rigorous calculations of 27 excited vibrational states of HCO and DCO, which are compared with experiment. A detailed analysis of the fundamentals of HCO and DCO suggests a reassignment of the experimental fundamentals of DCO is necessary. {copyright} {ital 1995} {ital American} {ital Institute} {ital of} {ital Physics}.
DOE Contract Number:
FG05-86ER13568
OSTI ID:
124790
Journal Information:
Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 18 Vol. 103; ISSN JCPSA6; ISSN 0021-9606
Country of Publication:
United States
Language:
English

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