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Neutron scattering studies of spin-phonon hybridization and superconducting spin gaps in the high temperature superconductor La2-x(Sr;Ba)xCuO4

Journal Article · · Physical Review B
 [1];  [2];  [1];  [1];  [3];  [3];  [3];  [3];  [3];  [4];  [4];  [4];  [5];  [1];  [1];  [1];  [1];  [6]
  1. McMaster Univ., Hamilton, ON (Canada)
  2. McMaster Univ., Hamilton, ON (Canada); Villanova Univ., Villanova, PA (United States)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  4. Univ. of Toronto, Toronto, ON (Canada)
  5. National Institute of Standards and Technology, Gaithersburg, MD (United States); Univ. of Maryland, College Park, MD (United States)
  6. McMaster Univ., Hamilton, ON (Canada); Canadian Institute for Advanced Research, Toronto, ON (Canada)
We present time-of-flight neutron-scattering measurements on single crystals of La2-xBaxCuO4 (LBCO) with 0 ≤ x ≤ 0.095 and La2-xSrxCuO4 (LSCO) with x = 0.08 and 0.11. This range of dopings spans much of the phase diagram relevant to high temperature cuprate superconductivity, ranging from insulating, three dimensional commensurate long range antiferromagnetic order for x ≤ 0.02 to two dimensional (2D) incommensurate antiferromagnetism co-existing with superconductivity for x ≥ 0.05. Previous work on lightly doped LBCO with x = 0.035 showed a clear resonant enhancement of the inelastic scattering coincident with the low energy crossings of the highly dispersive spin excitations and quasi-2D optic phonons. The present work extends these measurements across the phase diagram and shows this enhancement to be a common feature to this family of layered quantum magnets. Furthermore we show that the low temperature, low energy magnetic spectral weight is substantially larger for samples with non-superconducting ground states relative to any of the samples with superconducting ground states. Lastly spin gaps, suppression of low energy magnetic spectral weight, are observed in both superconducting LBCO and LSCO samples, consistent with previous observations for superconducting LSCO
Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC); USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1244192
Alternate ID(s):
OSTI ID: 1242615
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 9 Vol. 93; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Energy-dependent crossover from anisotropic to isotropic magnetic dispersion in lightly doped La 1.96 Sr 0.04 CuO 4 journal February 2013
Glassy low-energy spin fluctuations and anisotropy gap in La 1.88 Sr 0.12 CuO 4 journal April 2013
Two-dimensional incommensurate and three-dimensional commensurate magnetic order and fluctuations in La 2 − x Ba x CuO 4 journal July 2013
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