Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells

Shao, Yuchuan; Xiao, Zhengguo; Bi, Cheng; Yuan, Yongbo; Huang, Jinsong

doi:10.1038/ncomms6784

Origin and elimination of photocurrent hysteresis by fullerene passivation in CH₃NH₃PbI₃ planar heterojunction solar cells

Journal Article · Mon Dec 15 00:00:00 EST 2014 · Nature Communications

DOI:https://doi.org/10.1038/ncomms6784· OSTI ID:1237996

Shao, Yuchuan ^[1]; Xiao, Zhengguo ^[2]; Bi, Cheng ^[2]; Yuan, Yongbo ^[2]; Huang, Jinsong ^[2]

Univ. of Nebraska, Lincoln, NE (United States); University of Nebraska, Lincoln
Univ. of Nebraska, Lincoln, NE (United States)

The large photocurrent hysteresis observed in many organometal trihalide perovskite solar cells has become a major hindrance impairing the ultimate performance and stability of these devices, while its origin was unknown. Here we demonstrate the trap states on the surface and grain boundaries of the perovskite materials to be the origin of photocurrent hysteresis and that the fullerene layers deposited on perovskites can effectively passivate these charge trap states and eliminate the notorious photocurrent hysteresis. Fullerenes deposited on the top of the perovskites reduce the trap density by two orders of magnitude and double the power conversion efficiency of CH₃NH₃PbI₃ solar cells. As a result, the elucidation of the origin of photocurrent hysteresis and its elimination by trap passivation in perovskite solar cells provides important directions for future enhancements to device efficiency.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Nebraska, Lincoln, NE (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: EE0006709

OSTI ID:: 1237996

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 37 Vol. 5; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Organometal Halide Perovskite Artificial Synapses Xu, Wentao; Cho, Himchan; Kim, Young-Hoon Advanced Materials, Vol. 28, Issue 28 https://doi.org/10.1002/adma.201506363	journal	May 2016
Employing Lead Thiocyanate Additive to Reduce the Hysteresis and Boost the Fill Factor of Planar Perovskite Solar Cells Ke, Weijun; Xiao, Chuanxiao; Wang, Changlei Advanced Materials, Vol. 28, Issue 26 https://doi.org/10.1002/adma.201600594	journal	May 2016
Enhanced Efficiency and Stability of Inverted Perovskite Solar Cells Using Highly Crystalline SnO ₂ Nanocrystals as the Robust Electron-Transporting Layer Zhu, Zonglong; Bai, Yang; Liu, Xiao Advanced Materials, Vol. 28, Issue 30 https://doi.org/10.1002/adma.201600619	journal	May 2016
Thin Insulating Tunneling Contacts for Efficient and Water-Resistant Perovskite Solar Cells Wang, Qi; Dong, Qingfeng; Li, Tao Advanced Materials, Vol. 28, Issue 31 https://doi.org/10.1002/adma.201600969	journal	May 2016
Efficient Low-Temperature Solution-Processed Lead-Free Perovskite Infrared Light-Emitting Diodes Hong, Wei-Li; Huang, Yu-Chi; Chang, Che-Yu Advanced Materials, Vol. 28, Issue 36 https://doi.org/10.1002/adma.201601024	journal	July 2016
Ultrahigh Carrier Mobility Achieved in Photoresponsive Hybrid Perovskite Films via Coupling with Single-Walled Carbon Nanotubes Li, Feng; Wang, Hong; Kufer, Dominik Advanced Materials, Vol. 29, Issue 16 https://doi.org/10.1002/adma.201602432	journal	February 2017
Lead-Free Inverted Planar Formamidinium Tin Triiodide Perovskite Solar Cells Achieving Power Conversion Efficiencies up to 6.22% Liao, Weiqiang; Zhao, Dewei; Yu, Yue Advanced Materials, Vol. 28, Issue 42 https://doi.org/10.1002/adma.201602992	journal	August 2016
High-Performance Color-Tunable Perovskite Light Emitting Devices through Structural Modulation from Bulk to Layered Film Chen, Ziming; Zhang, Chongyang; Jiang, Xiao-Fang Advanced Materials, Vol. 29, Issue 8 https://doi.org/10.1002/adma.201603157	journal	December 2016
A Self-Powered, Sub-nanosecond-Response Solution-Processed Hybrid Perovskite Photodetector for Time-Resolved Photoluminescence-Lifetime Detection Shen, Liang; Fang, Yanjun; Wang, Dong Advanced Materials, Vol. 28, Issue 48 https://doi.org/10.1002/adma.201603573	journal	October 2016
Carbon-Based Perovskite Solar Cells without Hole Transport Materials: The Front Runner to the Market? Chen, Haining; Yang, Shihe Advanced Materials, Vol. 29, Issue 24 https://doi.org/10.1002/adma.201603994	journal	February 2017
Charge-Carrier Balance for Highly Efficient Inverted Planar Heterojunction Perovskite Solar Cells Chen, Ke; Hu, Qin; Liu, Tanghao Advanced Materials, Vol. 28, Issue 48 https://doi.org/10.1002/adma.201604048	journal	October 2016
Toward All Room-Temperature, Solution-Processed, High-Performance Planar Perovskite Solar Cells: A New Scheme of Pyridine-Promoted Perovskite Formation Zhang, Hong; Cheng, Jiaqi; Li, Dan Advanced Materials, Vol. 29, Issue 13 https://doi.org/10.1002/adma.201604695	journal	January 2017
A Review on Organic-Inorganic Halide Perovskite Photodetectors: Device Engineering and Fundamental Physics Ahmadi, Mahshid; Wu, Ting; Hu, Bin Advanced Materials, Vol. 29, Issue 41 https://doi.org/10.1002/adma.201605242	journal	September 2017
Two-Dimensional Materials for Halide Perovskite-Based Optoelectronic Devices Chen, Shan; Shi, Gaoquan Advanced Materials, Vol. 29, Issue 24 https://doi.org/10.1002/adma.201605448	journal	March 2017
Efficient Flexible Solar Cell based on Composition-Tailored Hybrid Perovskite Bi, Cheng; Chen, Bo; Wei, Haotong Advanced Materials, Vol. 29, Issue 30 https://doi.org/10.1002/adma.201605900	journal	June 2017
Achieving Large-Area Planar Perovskite Solar Cells by Introducing an Interfacial Compatibilizer Lee, Jinho; Kang, Hongkyu; Kim, Geunjin Advanced Materials, Vol. 29, Issue 22 https://doi.org/10.1002/adma.201606363	journal	April 2017
Chemical Reduction of Intrinsic Defects in Thicker Heterojunction Planar Perovskite Solar Cells Liu, Zonghao; Hu, Junnan; Jiao, Haoyang Advanced Materials, Vol. 29, Issue 23 https://doi.org/10.1002/adma.201606774	journal	April 2017
High-Temperature Ionic Epitaxy of Halide Perovskite Thin Film and the Hidden Carrier Dynamics Wang, Yiping; Sun, Xin; Chen, Zhizhong Advanced Materials, Vol. 29, Issue 35 https://doi.org/10.1002/adma.201702643	journal	July 2017
Planar‐Structure Perovskite Solar Cells with Efficiency beyond 21% Jiang, Qi; Chu, Zema; Wang, Pengyang Advanced Materials, Vol. 29, Issue 46 https://doi.org/10.1002/adma.201703852	journal	October 2017
Critical Role of Interface and Crystallinity on the Performance and Photostability of Perovskite Solar Cell on Nickel Oxide Nie, Wanyi; Tsai, Hsinhan; Blancon, Jean-Christophe Advanced Materials, Vol. 30, Issue 5 https://doi.org/10.1002/adma.201703879	journal	December 2017
From Nanostructural Evolution to Dynamic Interplay of Constituents: Perspectives for Perovskite Solar Cells Hwang, Taehyun; Lee, Byungho; Kim, Jinhyun Advanced Materials, Vol. 30, Issue 42 https://doi.org/10.1002/adma.201704208	journal	March 2018
Polymer-Passivated Inorganic Cesium Lead Mixed-Halide Perovskites for Stable and Efficient Solar Cells with High Open-Circuit Voltage over 1.3 V Zeng, Qingsen; Zhang, Xiaoyu; Feng, Xiaolei Advanced Materials, Vol. 30, Issue 9 https://doi.org/10.1002/adma.201705393	journal	January 2018
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Trash into Treasure: δ-FAPbI ₃ Polymorph Stabilized MAPbI ₃ Perovskite with Power Conversion Efficiency beyond 21% Zhang, Yi; Zhou, Zhongmin; Ji, Fuxiang Advanced Materials, Vol. 30, Issue 22 https://doi.org/10.1002/adma.201707143	journal	April 2018
Interstitial Occupancy by Extrinsic Alkali Cations in Perovskites and Its Impact on Ion Migration Cao, Jie; Tao, Shu Xia; Bobbert, Peter A. Advanced Materials, Vol. 30, Issue 26 https://doi.org/10.1002/adma.201707350	journal	May 2018
Ion-Migration Inhibition by the Cation-π Interaction in Perovskite Materials for Efficient and Stable Perovskite Solar Cells Wei, Dong; Ma, Fusheng; Wang, Rui Advanced Materials, Vol. 30, Issue 31 https://doi.org/10.1002/adma.201707583	journal	June 2018
Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering Rajagopal, Adharsh; Yao, Kai; Jen, Alex K. -Y. Advanced Materials, Vol. 30, Issue 32 https://doi.org/10.1002/adma.201800455	journal	June 2018
Grain-Boundary “Patches” by In Situ Conversion to Enhance Perovskite Solar Cells Stability Liu, Lang; Huang, Sheng; Lu, Yue Advanced Materials, Vol. 30, Issue 29 https://doi.org/10.1002/adma.201800544	journal	June 2018
Causes and Solutions of Recombination in Perovskite Solar Cells Chen, Jiangzhao; Park, Nam‐Gyu Advanced Materials, Vol. 31, Issue 47 https://doi.org/10.1002/adma.201803019	journal	September 2018
Reliable Measurement of Perovskite Solar Cells Wang, Yanbo; Liu, Xiao; Zhou, Zhongmin Advanced Materials, Vol. 31, Issue 47 https://doi.org/10.1002/adma.201803231	journal	September 2018
Interface and Defect Engineering for Metal Halide Perovskite Optoelectronic Devices Han, Tae‐Hee; Tan, Shaun; Xue, Jingjing Advanced Materials, Vol. 31, Issue 47 https://doi.org/10.1002/adma.201803515	journal	September 2018
Intensive Exposure of Functional Rings of a Polymeric Hole-Transporting Material Enables Efficient Perovskite Solar Cells Zhang, Luozheng; Liu, Chang; Zhang, Jie Advanced Materials, Vol. 30, Issue 39 https://doi.org/10.1002/adma.201804028	journal	August 2018
All-Solution-Processed Pure Formamidinium-Based Perovskite Light-Emitting Diodes Wang, Juanhong; Song, Chen; He, Zhiwei Advanced Materials, Vol. 30, Issue 39 https://doi.org/10.1002/adma.201804137	journal	August 2018
SnO ₂ ‐in‐Polymer Matrix for High‐Efficiency Perovskite Solar Cells with Improved Reproducibility and Stability Wei, Jing; Guo, Fengwan; Wang, Xi Advanced Materials, Vol. 30, Issue 52 https://doi.org/10.1002/adma.201805153	journal	November 2018
Versatile Defect Passivation Methods for Metal Halide Perovskite Materials and their Application to Light‐Emitting Devices Lee, Seungjin; Kim, Da Bin; Yu, Jae Choul Advanced Materials, Vol. 31, Issue 20 https://doi.org/10.1002/adma.201805244	journal	December 2018
Defect and Contact Passivation for Perovskite Solar Cells Aydin, Erkan; Bastiani, Michele; Wolf, Stefaan Advanced Materials, Vol. 31, Issue 25 https://doi.org/10.1002/adma.201900428	journal	April 2019
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Synergistic Effect of Elevated Device Temperature and Excess Charge Carriers on the Rapid Light‐Induced Degradation of Perovskite Solar Cells Chen, Bo; Song, Jingfeng; Dai, Xuezeng Advanced Materials, Vol. 31, Issue 35 https://doi.org/10.1002/adma.201902413	journal	July 2019
Interphases, Interfaces, and Surfaces of Active Materials in Rechargeable Batteries and Perovskite Solar Cells Liu, Chaofeng; Yuan, Jifeng; Masse, Robert Advanced Materials https://doi.org/10.1002/adma.201905245	journal	January 2020
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Graphdiyne Quantum Dots for Much Improved Stability and Efficiency of Perovskite Solar Cells Zhang, Xisheng; Wang, Qian; Jin, Zhiwen Advanced Materials Interfaces, Vol. 5, Issue 2 https://doi.org/10.1002/admi.201701117	journal	November 2017
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Defect Engineering toward Highly Efficient and Stable Perovskite Solar Cells Li, Bowei; Ferguson, Victoria; Silva, S. Ravi P. Advanced Materials Interfaces, Vol. 5, Issue 22 https://doi.org/10.1002/admi.201800326	journal	July 2018
Pb‐Bi Binary Metal All‐Inorganic Absorber Layer for Stability Enhancement in Perovskite Solar Cells Huang, Jin; Zhang, Dan; Ding, Lei Advanced Materials Interfaces https://doi.org/10.1002/admi.201900517	journal	June 2019
Surface Plasmon Resonance Effect in Inverted Perovskite Solar Cells Cui, Jin; Chen, Cheng; Han, Junbo Advanced Science, Vol. 3, Issue 3 https://doi.org/10.1002/advs.201500312	journal	January 2016
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Modeling Thin Film Solar Cells: From Organic to Perovskite Li, Deli; Song, Lin; Chen, Yonghua Advanced Science, Vol. 7, Issue 1 https://doi.org/10.1002/advs.201901397	journal	November 2019
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Vertical Organic-Inorganic Hybrid Perovskite Schottky Junction Transistors Yu, Hyeonggeun; Cheng, Yuanhang; Shin, Donghun Advanced Electronic Materials, Vol. 4, Issue 5 https://doi.org/10.1002/aelm.201800039	journal	March 2018
Recent Advances in Memory Devices with Hybrid Materials Hwang, Bohee; Lee, Jang-Sik Advanced Electronic Materials, Vol. 5, Issue 1 https://doi.org/10.1002/aelm.201800519	journal	October 2018
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Stability of Metal Halide Perovskite Solar Cells Leijtens, Tomas; Eperon, Giles E.; Noel, Nakita K. Advanced Energy Materials, Vol. 5, Issue 20 https://doi.org/10.1002/aenm.201500963	journal	September 2015
Recent Advances in Improving the Stability of Perovskite Solar Cells Tiep, Nguyen Huy; Ku, Zhiliang; Fan, Hong Jin Advanced Energy Materials, Vol. 6, Issue 3 https://doi.org/10.1002/aenm.201501420	journal	November 2015
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Critical Role of Grain Boundaries for Ion Migration in Formamidinium and Methylammonium Lead Halide Perovskite Solar Cells Yun, Jae S.; Seidel, Jan; Kim, Jincheol Advanced Energy Materials, Vol. 6, Issue 13 https://doi.org/10.1002/aenm.201600330	journal	May 2016
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Direct Evidence of Ion Diffusion for the Silver-Electrode-Induced Thermal Degradation of Inverted Perovskite Solar Cells Li, Jiangwei; Dong, Qingshun; Li, Nan Advanced Energy Materials, Vol. 7, Issue 14 https://doi.org/10.1002/aenm.201602922	journal	March 2017
Structure of Organometal Halide Perovskite Films as Determined with Grazing-Incidence X-Ray Scattering Methods Schlipf, Johannes; Müller-Buschbaum, Peter Advanced Energy Materials, Vol. 7, Issue 16 https://doi.org/10.1002/aenm.201700131	journal	March 2017
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Rubidium Multication Perovskite with Optimized Bandgap for Perovskite-Silicon Tandem with over 26% Efficiency Duong, The; Wu, YiLiang; Shen, Heping Advanced Energy Materials, Vol. 7, Issue 14 https://doi.org/10.1002/aenm.201700228	journal	April 2017
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Limiting Perovskite Solar Cell Performance by Heterogeneous Carrier Extraction Tian, Wenming; Cui, Rongrong; Leng, Jing Angewandte Chemie, Vol. 128, Issue 42 https://doi.org/10.1002/ange.201606574	journal	October 2016
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Suppressing Charge Recombination and Ultraviolet Light Degradation of Perovskite Solar Cells Using Silicon Oxide Passivation Ren, Jing; Luo, Qiang; Hou, Qinzhi ChemElectroChem, Vol. 6, Issue 12 https://doi.org/10.1002/celc.201900688	journal	May 2019
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Highly crystalline Zn ₂ SnO ₄ nanoparticles as efficient electron-transporting layers toward stable inverted and flexible conventional perovskite solar cells Liu, Xiao; Chueh, Chu-Chen; Zhu, Zonglong Journal of Materials Chemistry A, Vol. 4, Issue 40 https://doi.org/10.1039/c6ta05745d	journal	January 2016
Enhancing the photovoltaic performance of planar heterojunction perovskite solar cells by doping the perovskite layer with alkali metal ions Chang, Jingjing; Lin, Zhenhua; Zhu, Hai Journal of Materials Chemistry A, Vol. 4, Issue 42 https://doi.org/10.1039/c6ta06851k	journal	January 2016
Enhanced performance and light soaking stability of planar perovskite solar cells using an amine-based fullerene interfacial modifier Zhang, Yunhai; Wang, Peng; Yu, Xuegong Journal of Materials Chemistry A, Vol. 4, Issue 47 https://doi.org/10.1039/c6ta08992e	journal	January 2016
Performance enhancement of perovskite solar cells using a La-doped BaSnO ₃ electron transport layer Zhu, Liangzheng; Ye, Jiajiu; Zhang, Xuhui Journal of Materials Chemistry A, Vol. 5, Issue 7 https://doi.org/10.1039/c6ta09689a	journal	January 2017
Interface passivation using ultrathin polymer–fullerene films for high-efficiency perovskite solar cells with negligible hysteresis Peng, Jun; Wu, Yiliang; Ye, Wang Energy & Environmental Science, Vol. 10, Issue 8 https://doi.org/10.1039/c7ee01096f	journal	January 2017
Impact of H ₂ O on organic–inorganic hybrid perovskite solar cells Huang, Jianbing; Tan, Shunquan; Lund, Peter D. Energy & Environmental Science, Vol. 10, Issue 11 https://doi.org/10.1039/c7ee01674c	journal	January 2017
In situ induced core/shell stabilized hybrid perovskites via gallium( iii ) acetylacetonate intermediate towards highly efficient and stable solar cells Li, Wenzhe; Zhang, Cuiling; Ma, Yunping Energy & Environmental Science, Vol. 11, Issue 2 https://doi.org/10.1039/c7ee03113k	journal	January 2018
Fullerene derivative with a branched alkyl chain exhibits enhanced charge extraction and stability in inverted planar perovskite solar cells Tian, Chengbo; Castro, Edison; Betancourt-Solis, German New Journal of Chemistry, Vol. 42, Issue 4 https://doi.org/10.1039/c7nj04978a	journal	January 2018
Enhanced planar perovskite solar cell efficiency and stability using a perovskite/PCBM heterojunction formed in one step Zhou, Long; Chang, Jingjing; Liu, Ziye Nanoscale, Vol. 10, Issue 6 https://doi.org/10.1039/c7nr07753j	journal	January 2018
Efficient and ultraviolet durable planar perovskite solar cells via a ferrocenecarboxylic acid modified nickel oxide hole transport layer Zhang, Jiankai; Luo, Hui; Xie, Weijia Nanoscale, Vol. 10, Issue 12 https://doi.org/10.1039/c7nr08750k	journal	January 2018
A dimeric fullerene derivative for efficient inverted planar perovskite solar cells with improved stability Tian, Chengbo; Kochiss, Kevin; Castro, Edison Journal of Materials Chemistry A, Vol. 5, Issue 16 https://doi.org/10.1039/c7ta00362e	journal	January 2017
Recent advances in perovskite solar cells: efficiency, stability and lead-free perovskite Yang, Shida; Fu, Weifei; Zhang, Zhongqiang Journal of Materials Chemistry A, Vol. 5, Issue 23 https://doi.org/10.1039/c7ta00366h	journal	January 2017
Tailored Au@TiO ₂ nanostructures for the plasmonic effect in planar perovskite solar cells Fan, Rundong; Wang, Ligang; Chen, Yihua Journal of Materials Chemistry A, Vol. 5, Issue 24 https://doi.org/10.1039/c7ta02937c	journal	January 2017
Highly efficient and stable low-temperature processed ZnO solar cells with triple cation perovskite absorber Song, Jiaxing; Liu, Leijing; Wang, Xiao-Feng Journal of Materials Chemistry A, Vol. 5, Issue 26 https://doi.org/10.1039/c7ta03331a	journal	January 2017
Fluorinated fused nonacyclic interfacial materials for efficient and stable perovskite solar cells Liu, Kuan; Dai, Shuixing; Meng, Fanqi J. Mater. Chem. A, Vol. 5, Issue 40 https://doi.org/10.1039/c7ta06923e	journal	January 2017
Efficient PbS quantum dot solar cells employing a conventional structure Lu, Kunyuan; Wang, Yongjie; Yuan, Jianyu Journal of Materials Chemistry A, Vol. 5, Issue 45 https://doi.org/10.1039/c7ta07014d	journal	January 2017
Post-healing of defects: an alternative way for passivation of carbon-based mesoscopic perovskite solar cells via hydrophobic ligand coordination Huang, Guangguang; Wang, Chunlei; Zhang, Hao Journal of Materials Chemistry A, Vol. 6, Issue 6 https://doi.org/10.1039/c7ta09646a	journal	January 2018
High mobility, hole transport materials for highly efficient PEDOT:PSS replacement in inverted perovskite solar cells Neophytou, Marios; Griffiths, Jack; Fraser, James Journal of Materials Chemistry C, Vol. 5, Issue 20 https://doi.org/10.1039/c7tc00858a	journal	January 2017
Exploring the effects of interfacial carrier transport layers on device performance and optoelectronic properties of planar perovskite solar cells Khadka, Dhruba B.; Shirai, Yasuhiro; Yanagida, Masatoshi Journal of Materials Chemistry C, Vol. 5, Issue 34 https://doi.org/10.1039/c7tc02822a	journal	January 2017
Amorphous polymer with CO to improve the performance of perovskite solar cells Zhang, Ying; Zhuang, Xueheng; Zhou, Kang Journal of Materials Chemistry C, Vol. 5, Issue 35 https://doi.org/10.1039/c7tc02954c	journal	January 2017
Degradation of encapsulated perovskite solar cells driven by deep trap states and interfacial deterioration Khadka, Dhruba B.; Shirai, Yasuhiro; Yanagida, Masatoshi Journal of Materials Chemistry C, Vol. 6, Issue 1 https://doi.org/10.1039/c7tc03733c	journal	January 2018
Morphological and compositional progress in halide perovskite solar cells Kim, Hui-Seon; Hagfeldt, Anders; Park, Nam-Gyu Chemical Communications, Vol. 55, Issue 9 https://doi.org/10.1039/c8cc08653b	journal	January 2019
Improved fill factor in inverted planar perovskite solar cells with zirconium acetate as the hole-and-ion-blocking layer Zhang, Xuewen; Liang, Chunjun; Sun, Mengjie Physical Chemistry Chemical Physics, Vol. 20, Issue 11 https://doi.org/10.1039/c8cp00563j	journal	January 2018
Photo-induced dual passivation via Usanovich acid–base on surface defects of methylammonium lead triiodide perovskite Yu, Yue; Wan, Sushu; Hong, Daocheng Physical Chemistry Chemical Physics, Vol. 20, Issue 44 https://doi.org/10.1039/c8cp06112b	journal	January 2018
Imperfections and their passivation in halide perovskite solar cells Chen, Bo; Rudd, Peter N.; Yang, Shuang Chemical Society Reviews, Vol. 48, Issue 14 https://doi.org/10.1039/c8cs00853a	journal	January 2019
Slow surface passivation and crystal relaxation with additives to improve device performance and durability for tin-based perovskite solar cells Jokar, Efat; Chien, Cheng-Hsun; Fathi, Amir Energy & Environmental Science, Vol. 11, Issue 9 https://doi.org/10.1039/c8ee00956b	journal	January 2018
Fullerene derivative anchored SnO ₂ for high-performance perovskite solar cells Liu, Kuan; Chen, Shuang; Wu, Jionghua Energy & Environmental Science, Vol. 11, Issue 12 https://doi.org/10.1039/c8ee02172d	journal	January 2018
Thermally stable, planar hybrid perovskite solar cells with high efficiency Choi, Kyoungwon; Lee, Junwoo; Kim, Hong Il Energy & Environmental Science, Vol. 11, Issue 11 https://doi.org/10.1039/c8ee02242a	journal	January 2018
Photo-induced dynamic processes in perovskite solar cells: the influence of perovskite composition in the charge extraction and the carrier recombination Montcada, Núria F.; Méndez, Maria; Cho, Kyung Taek Nanoscale, Vol. 10, Issue 13 https://doi.org/10.1039/c8nr00180d	journal	January 2018
Grain engineering by ultrasonic substrate vibration post-treatment of wet perovskite films for annealing-free, high performance, and stable perovskite solar cells Xiong, Hao; Zabihi, Fatemeh; Wang, Hongzhi Nanoscale, Vol. 10, Issue 18 https://doi.org/10.1039/c8nr00540k	journal	January 2018
Spray coating of the PCBM electron transport layer significantly improves the efficiency of p-i-n planar perovskite solar cells Zheng, Yifan; Kong, Jaemin; Huang, Di Nanoscale, Vol. 10, Issue 24 https://doi.org/10.1039/c8nr01763h	journal	January 2018
Structural design considerations of solution-processable graphenes as interfacial materials via a controllable synthesis method for the achievement of highly efficient, stable, and printable planar perovskite solar cells Yeo, Jun-Seok; Seo, You-Hyun; Jung, Chan-Hee Nanoscale, Vol. 11, Issue 3 https://doi.org/10.1039/c8nr05698f	journal	January 2019
Totally room-temperature solution-processing method for fabricating flexible perovskite solar cells using an Nb ₂ O ₅ –TiO ₂ electron transport layer Jiang, Jun; Wang, Shubo; Jia, Xuguang RSC Advances, Vol. 8, Issue 23 https://doi.org/10.1039/c8ra01571f	journal	January 2018
Reduced graphene oxide-induced crystallization of CuPc interfacial layer for high performance of perovskite photodetectors Zou, Taoyu; Zhang, Jianqi; Huang, Shuyi RSC Advances, Vol. 9, Issue 7 https://doi.org/10.1039/c8ra08864k	journal	January 2019
Blue and red wavelength resolved impedance response of efficient perovskite solar cells Prochowicz, Daniel; Tavakoli, Mohammad Mahdi; Turren-Cruz, Silver-Hamill Sustainable Energy & Fuels, Vol. 2, Issue 11 https://doi.org/10.1039/c8se00280k	journal	January 2018
Facile surface modification of CH ₃ NH ₃ PbI ₃ films leading to simultaneously improved efficiency and stability of inverted perovskite solar cells Zhu, Hongmei; Huang, Boyuan; Wu, Shaohang Journal of Materials Chemistry A, Vol. 6, Issue 15 https://doi.org/10.1039/c8ta00267c	journal	January 2018
Enhanced performance of perovskite solar cells via anti-solvent nonfullerene Lewis base IT-4F induced trap-passivation Guo, Yaxiong; Ma, Junjie; Lei, Hongwei Journal of Materials Chemistry A, Vol. 6, Issue 14 https://doi.org/10.1039/c8ta00583d	journal	January 2018
High-air-flow-velocity assisted intermediate phase engineering for controlled crystallization of mixed perovskite in high efficiency photovoltaics Wang, Shi; Zhang, Chunyang; Feng, Yulin Journal of Materials Chemistry A, Vol. 6, Issue 19 https://doi.org/10.1039/c8ta02144a	journal	January 2018
Controlled surface decomposition derived passivation and energy-level alignment behaviors for high performance perovskite solar cells Li, Zhipeng; Zhang, Cuiping; Shao, Zhipeng Journal of Materials Chemistry A, Vol. 6, Issue 20 https://doi.org/10.1039/c8ta02652a	journal	January 2018
Monolayer-like hybrid halide perovskite films prepared by additive engineering without antisolvents for solar cells Wang, Mengru; Li, Bo; Siffalovic, Peter Journal of Materials Chemistry A, Vol. 6, Issue 31 https://doi.org/10.1039/c8ta04794d	journal	January 2018
Achieving high-performance thick-film perovskite solar cells with electron transporting Bingel fullerenes Yan, Kangrong; Chen, Jiehuan; Ju, Huanxin Journal of Materials Chemistry A, Vol. 6, Issue 32 https://doi.org/10.1039/c8ta05636f	journal	January 2018
Catalytic metal-induced crystallization of sol–gel metal oxides for high-efficiency flexible perovskite solar cells Hou, Cheng-Hung; Shyue, Jing-Jong; Su, Wei-Fang Journal of Materials Chemistry A, Vol. 6, Issue 34 https://doi.org/10.1039/c8ta05973j	journal	January 2018
A perylene diimide-based electron transport layer enabling efficient inverted perovskite solar cells Jiang, Kui; Wu, Fei; Yu, Hui Journal of Materials Chemistry A, Vol. 6, Issue 35 https://doi.org/10.1039/c8ta06081a	journal	January 2018
Regulating the electron transporting properties of indacenodithiophene derivatives for perovskite solar cells with PCEs up to 19.51% Zhu, Linna; Gao, Wei; Wu, Fei Journal of Materials Chemistry A, Vol. 6, Issue 37 https://doi.org/10.1039/c8ta06730a	journal	January 2018
Interfacial engineering enables high efficiency with a high open-circuit voltage above 1.23 V in 2D perovskite solar cells Chen, Jiehuan; Lian, Xiaomei; Zhang, Yingzhu Journal of Materials Chemistry A, Vol. 6, Issue 37 https://doi.org/10.1039/c8ta06925e	journal	January 2018
Highly efficient planar perovskite solar cells achieved by simultaneous defect engineering and formation kinetic control Cheng, Jiaqi; Zhang, Hong; Zhang, Shaoqing Journal of Materials Chemistry A, Vol. 6, Issue 46 https://doi.org/10.1039/c8ta08819e	journal	January 2018
Surface & grain boundary co-passivation by fluorocarbon based bifunctional molecules for perovskite solar cells with efficiency over 21% Guo, Pengfei; Ye, Qian; Yang, Xiaokun Journal of Materials Chemistry A, Vol. 7, Issue 6 https://doi.org/10.1039/c8ta11524a	journal	January 2019
Energy level-modulated non-fullerene small molecule acceptors for improved V _OC and efficiency of inverted perovskite solar cells Liu, Xiaohui; Li, Xiaodong; Zou, Yang Journal of Materials Chemistry A, Vol. 7, Issue 7 https://doi.org/10.1039/c8ta12028e	journal	January 2019
Pyridine-functionalized fullerene additive enabling coordination interactions with CH ₃ NH ₃ PbI ₃ perovskite towards highly efficient bulk heterojunction solar cells Zhen, Jieming; Zhou, Weiran; Chen, Muqing Journal of Materials Chemistry A, Vol. 7, Issue 6 https://doi.org/10.1039/c8ta12206g	journal	January 2019
Exploring the role of spin-triplets and trap states in photovoltaic processes of perovskite solar cells Lu, Kai; Zhao, Chen; Luan, Lin Journal of Materials Chemistry C, Vol. 6, Issue 18 https://doi.org/10.1039/c8tc00455b	journal	January 2018
Light-activated inorganic CsPbBr ₂ I perovskite for room-temperature self-powered chemical sensing Chen, Hongjun; Zhang, Meng; Fu, Xiao Physical Chemistry Chemical Physics, Vol. 21, Issue 43 https://doi.org/10.1039/c9cp03059j	journal	January 2019
It's a trap! On the nature of localised states and charge trapping in lead halide perovskites Jin, Handong; Debroye, Elke; Keshavarz, Masoumeh Materials Horizons, Vol. 7, Issue 2 https://doi.org/10.1039/c9mh00500e	journal	January 2020
Fabrication of pyramidal (111) MAPbBr ₃ film with low surface defect density using homogeneous quantum-dot seeds Jeong, Hyeon Jun; Bang, Seungho; Park, Dae Young Nanoscale, Vol. 12, Issue 3 https://doi.org/10.1039/c9nr10070a	journal	January 2020
Highly bright perovskite light-emitting diodes based on quasi-2D perovskite film through synergetic solvent engineering Yue, Huanxin; Song, Dandan; Zhao, Suling RSC Advances, Vol. 9, Issue 15 https://doi.org/10.1039/c9ra00912d	journal	January 2019
Beneficial effects of potassium iodide incorporation on grain boundaries and interfaces of perovskite solar cells Yang, Yin; Wu, Lili; Hao, Xia RSC Advances, Vol. 9, Issue 49 https://doi.org/10.1039/c9ra05371a	journal	January 2019
In situ transfer of CH ₃ NH ₃ PbI ₃ single crystals in mesoporous scaffolds for efficient perovskite solar cells Guan, Yanjun; Xu, Mi; Zhang, Wenhao Chemical Science, Vol. 11, Issue 2 https://doi.org/10.1039/c9sc04900b	journal	January 2020
Unravelling fullerene–perovskite interactions introduces advanced blend films for performance-improved solar cells Pascual, Jorge; Collavini, Silvia; Völker, Sebastian F. Sustainable Energy & Fuels, Vol. 3, Issue 10 https://doi.org/10.1039/c9se00438f	journal	January 2019
Hybrid CdSe/CsPbI ₃ quantum dots for interface engineering in perovskite solar cells Ge, Jing; Li, Weixin; He, Xuan Sustainable Energy & Fuels, Vol. 4, Issue 4 https://doi.org/10.1039/c9se01205b	journal	January 2020
Enhanced efficacy of defect passivation and charge extraction for efficient perovskite photovoltaics with a small open circuit voltage loss Liao, Jin-Feng; Wu, Wu-Qiang; Zhong, Jun-Xing Journal of Materials Chemistry A, Vol. 7, Issue 15 https://doi.org/10.1039/c9ta01760g	journal	January 2019
Engineering the underlying surface to manipulate the growth of 2D perovskites for highly efficient solar cells Tian, Shuoxun; Chen, Jiehuan; Lian, Xiaomei Journal of Materials Chemistry A, Vol. 7, Issue 23 https://doi.org/10.1039/c9ta03022k	journal	January 2019
Phenethylammonium bismuth halides: from single crystals to bulky-organic cation promoted thin-film deposition for potential optoelectronic applications Ghasemi, Mehri; Lyu, Miaoqiang; Roknuzzaman, Md Journal of Materials Chemistry A, Vol. 7, Issue 36 https://doi.org/10.1039/c9ta07454f	journal	January 2019
Perovskite solar cell-hybrid devices: thermoelectrically, electrochemically, and piezoelectrically connected power packs Zabihi, Fatemeh; Tebyetekerwa, Mike; Xu, Zhen Journal of Materials Chemistry A, Vol. 7, Issue 47 https://doi.org/10.1039/c9ta08070h	journal	January 2019
Efficient perovskite solar cells enabled by ion-modulated grain boundary passivation with a fill factor exceeding 84% Li, Zhiqi; Wang, Feng; Liu, Chunyu Journal of Materials Chemistry A, Vol. 7, Issue 39 https://doi.org/10.1039/c9ta08081c	journal	January 2019
Inverted planar perovskite solar cells based on CsI-doped PEDOT:PSS with efficiency beyond 20% and small energy loss Jiang, Kui; Wu, Fei; Zhang, Guangye Journal of Materials Chemistry A, Vol. 7, Issue 38 https://doi.org/10.1039/c9ta08995k	journal	January 2019
Br-containing alkyl ammonium salt-enabled scalable fabrication of high-quality perovskite films for efficient and stable perovskite modules Xu, Zhongyuan; Chen, Ruihao; Wu, Yazhuo Journal of Materials Chemistry A, Vol. 7, Issue 47 https://doi.org/10.1039/c9ta09101g	journal	January 2019
Molecular aggregation method for perovskite–fullerene bulk heterostructure solar cells Ha, Su Ryong; Jeong, Woo Hyeon; Liu, Yanliang Journal of Materials Chemistry A, Vol. 8, Issue 3 https://doi.org/10.1039/c9ta11854c	journal	January 2020
Morphology control towards a greener, non-halogenated solvent system processed CH ₃ NH ₃ PbI ₃ film for high performance perovskite solar cells Tan, Wan-Yi; Cheng, Peng-Peng; Zhang, Yong-Wen Journal of Materials Chemistry C, Vol. 7, Issue 20 https://doi.org/10.1039/c9tc00812h	journal	January 2019
A facile method to evaluate the influence of trap densities on perovskite solar cell performance Chen, Bingbing; Hu, Hongwei; Salim, Teddy Journal of Materials Chemistry C, Vol. 7, Issue 19 https://doi.org/10.1039/c9tc00816k	journal	January 2019
Efficient perovskite solar cells with negligible hysteresis achieved by sol–gel-driven spinel nickel cobalt oxide thin films as the hole transport layer Lee, Ju Ho; Noh, Young Wook; Jin, In Su Journal of Materials Chemistry C, Vol. 7, Issue 24 https://doi.org/10.1039/c9tc00902g	journal	January 2019
Incorporation of two electron acceptors to improve the electron mobility and stability of perovskite solar cells Tang, Xianglan; Xiao, Shuqin; Fu, Qingxia Journal of Materials Chemistry C, Vol. 7, Issue 27 https://doi.org/10.1039/c9tc02457c	journal	January 2019
Electric dipole moment-assisted charge extraction and effective defect passivation in perovskite solar cells by depositing a PCBM:TIPD blend film on a CH ₃ NH ₃ PbI ₃ layer Weng, Yujuan; Shen, Zhitao; Guo, Mingxuan Journal of Materials Chemistry C, Vol. 7, Issue 37 https://doi.org/10.1039/c9tc03881g	journal	January 2019
Barium acetate as an additive for high performance perovskite solar cells Wang, Yueming; Wu, Yulei; Fu, Sheng Journal of Materials Chemistry C, Vol. 7, Issue 37 https://doi.org/10.1039/c9tc04067f	journal	January 2019
Formamidine-assisted fast crystallization to fabricate formamidinium-based perovskite films for high-efficiency and stable solar cells Zhang, Shasha; Wu, Shaohang; Chen, Rui Journal of Materials Chemistry C, Vol. 8, Issue 5 https://doi.org/10.1039/c9tc05465k	journal	January 2020
Single crystals of mixed Br/Cl and Sn-doped formamidinium lead halide perovskites via inverse temperature crystallization Ng, Michael; Halpert, Jonathan E. RSC Advances, Vol. 10, Issue 7 https://doi.org/10.1039/d0ra00060d	journal	January 2020
Minimizing performance degradation induced by interfacial recombination in perovskite solar cells through tailoring of the transport layer electronic properties Xu, Liang; Molaei Imenabadi, Rouzbeh; Vandenberghe, William G. APL Materials, Vol. 6, Issue 3 https://doi.org/10.1063/1.5021138	journal	March 2018
High efficiency flexible perovskite solar cells using SnO ₂ /graphene electron selective layer and silver nanowires electrode Liu, Xiangyang; Yang, Xiaodu; Liu, Xinsheng Applied Physics Letters, Vol. 113, Issue 20 https://doi.org/10.1063/1.5042299	journal	November 2018
Inverted perovskite solar cells with transparent hole transporting layer based on semiconducting nickel oxide Di Girolamo, Diego; Matteocci, Fabio; Lamanna, Enrico EMERGING TECHNOLOGIES: MICRO TO NANO (ETMN-2017): Proceedings of the 3rd International Conference on Emerging Technologies: Micro to Nano, AIP Conference Proceedings https://doi.org/10.1063/1.5047765	conference	January 2018
Thin‐film solar cells exceeding 22% solar cell efficiency: An overview on CdTe-, Cu(In,Ga)Se ₂ -, and perovskite-based materials Powalla, Michael; Paetel, Stefan; Ahlswede, Erik Applied Physics Reviews, Vol. 5, Issue 4 https://doi.org/10.1063/1.5061809	journal	December 2018
The two faces of capacitance: New interpretations for electrical impedance measurements of perovskite solar cells and their relation to hysteresis Jacobs, Daniel A.; Shen, Heping; Pfeffer, Florian Journal of Applied Physics, Vol. 124, Issue 22 https://doi.org/10.1063/1.5063259	journal	December 2018
Ion induced passivation of grain boundaries in perovskite solar cells Nandal, Vikas; Nair, Pradeep R. Journal of Applied Physics, Vol. 125, Issue 17 https://doi.org/10.1063/1.5082967	journal	May 2019
In situ investigation of light soaking in organolead halide perovskite films Zhong, Yu; Luna, Carlos Andres Melo; Hildner, Richard APL Materials, Vol. 7, Issue 4 https://doi.org/10.1063/1.5086125	journal	April 2019
Methylammonium-chloride post-treatment on perovskite surface and its correlation to photovoltaic performance in the aspect of electronic traps Hwang, Taehyun; Yun, Alan Jiwan; Lee, Byungho Journal of Applied Physics, Vol. 126, Issue 2 https://doi.org/10.1063/1.5098336	journal	July 2019
Research progress on organic–inorganic halide perovskite materials and solar cells Ono, Luis K.; Qi, Yabing Journal of Physics D: Applied Physics, Vol. 51, Issue 9 https://doi.org/10.1088/1361-6463/aaa727	journal	February 2018
Comparison of the Al back contact deposited by sputtering, e-beam, or thermal evaporation for inverted perovskite solar cells Wahl, Tina; Hanisch, Jonas; Ahlswede, Erik Journal of Physics D: Applied Physics, Vol. 51, Issue 13 https://doi.org/10.1088/1361-6463/aab0d8	journal	March 2018
Inverted hysteresis in MAPbI ₃ perovskite solar cells induced by presetting bias voltage Xiang, Jin; Li, Yana; Huang, Feng Journal of Physics D: Applied Physics, Vol. 52, Issue 31 https://doi.org/10.1088/1361-6463/ab1e2b	journal	May 2019
Synthesis and Characterization of Methylammonium Lead Iodide Perovskite and its Application in Planar Hetero-junction Devices Upadhyaya, Aditi; Negi, Chandra Mohan Singh; Yadav, Anjali Semiconductor Science and Technology, Vol. 33, Issue 6 https://doi.org/10.1088/1361-6641/aac066	journal	May 2018
The roles of acetylacetone additives in enhancing perovskite solar cell performance Zhuang, Xueheng; Zhang, Ying; Zhang, Jing Materials Research Express, Vol. 6, Issue 2 https://doi.org/10.1088/2053-1591/aaeeb2	journal	November 2018
Light-induced effects on crystal size and photo-stability of colloidal CsPbBr ₃ perovskite nanocrystals Esparza, Diego; Sidhik, Siraj; López-Luke, Tzarara Materials Research Express, Vol. 6, Issue 4 https://doi.org/10.1088/2053-1591/aafbce	journal	January 2019
First-principles calculation of stability, electronic and optical properties of PCBM-adsorbed MAPbI ₃ surface Tian, Ying; Xue, Hongtao; Tang, Fuling Materials Research Express, Vol. 6, Issue 11 https://doi.org/10.1088/2053-1591/ab51dc	journal	September 2019
Printable materials for printed perovskite solar cells Li, Wangnan; Zhong, Zhicheng; Huang, Fuzhi Flexible and Printed Electronics, Vol. 5, Issue 1 https://doi.org/10.1088/2058-8585/ab56b4	journal	January 2020
First-principles study on the material properties of the inorganic perovskite Rb 1 − x Cs x PbI 3 for solar cell applications Jong, Un-Gi; Yu, Chol-Jun; Kim, Yun-Sim Physical Review B, Vol. 98, Issue 12 https://doi.org/10.1103/physrevb.98.125116	journal	September 2018
Pathways toward high-performance perovskite solar cells: review of recent advances in organo-metal halide perovskites for photovoltaic applications Song, Zhaoning; Watthage, Suneth C.; Phillips, Adam B. Journal of Photonics for Energy, Vol. 6, Issue 2 https://doi.org/10.1117/1.jpe.6.022001	journal	April 2016
Stabilizing halide perovskite surfaces for solar cell operation with wide-bandgap lead oxysalts Yang, Shuang; Chen, Shangshang; Mosconi, Edoardo Science, Vol. 365, Issue 6452 https://doi.org/10.1126/science.aax3294	journal	August 2019
The Effect of Decomposed PbI2 on Microscopic Mechanisms of Scattering in CH3NH3PbI3 Films Shan, Dan; Tong, Guoqing; Cao, Yunqing Nanoscale Research Letters, Vol. 14, Issue 1 https://doi.org/10.1186/s11671-019-3022-y	journal	June 2019
Matching Charge Extraction Contact for Wide-Bandgap Perovskite Solar Cells B., Chen,; Y., Shao,; J., Huang, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/50rf-ma51	text	January 2017
Stabilizing halide perovskite surfaces for solar cell operation with wide-bandgap lead oxysalts X., Xiao,; E., Mosconi,; Y., Gao, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/j2pq-mf32	text	January 2019
Attaining High Photovoltaic Efficiency and Stability with Multidimensional Perovskites. Kosasih, Felix; Ducati, Caterina Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.33139	text	January 2018
Influence of Interfacial Traps on the Operating Temperature of Perovskite Solar Cells Mehdizadeh-Rad, Hooman; Singh, Jai Materials, Vol. 12 https://doi.org/10.20944/preprints201906.0281.v1	journal	June 2019
A Review on Improving the Quality of Perovskite Films in Perovskite Solar Cells via the Weak Forces Induced by Additives Yang, Jien; Chen, Songhua; Xu, Jinjin Applied Sciences, Vol. 9, Issue 20 https://doi.org/10.3390/app9204393	journal	October 2019
High Performance Planar Structure Perovskite Solar Cells Using a Solvent Dripping Treatment on Hole Transporting Layer Wang, Xuhui; Lu, Gang; Zhang, Min Coatings, Vol. 10, Issue 2 https://doi.org/10.3390/coatings10020127	journal	February 2020
Analysing the Prospects of Perovskite Solar Cells within the Purview of Recent Scientific Advancements Bhat, Aakash; Dhamaniya, Bhanu; Chhillar, Priyanka Crystals, Vol. 8, Issue 6 https://doi.org/10.3390/cryst8060242	journal	June 2018
Hysteresis Passivation in Planar Perovskite Solar Cells Utilizing Facile Chemical Vapor Deposition Process and PCBM Interlayer Yang, Chongqiu; Shan, Xiaobiao; Xie, Tao Energies, Vol. 12, Issue 23 https://doi.org/10.3390/en12234508	journal	November 2019
Emission Enhancement and Intermittency in Polycrystalline Organolead Halide Perovskite Films Li, Cheng; Zhong, Yu; Luna, Carlos Molecules, Vol. 21, Issue 8 https://doi.org/10.3390/molecules21081081	journal	August 2016
Controlling competing photochemical reactions stabilizes perovskite solar cells Motti, Silvia G.; Meggiolaro, Daniele; Barker, Alex J. Zenodo https://doi.org/10.5281/zenodo.3738939	text	January 2019
On the origin of open-circuit voltage losses in flexible n-i-p perovskite solar cells Pisoni, Stefano; Stolterfoht, Martin; Löckinger, Johannes Taylor & Francis https://doi.org/10.6084/m9.figshare.8305928	text	January 2019

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14 SOLAR ENERGY
36 MATERIALS SCIENCE
applied physics
materials science
physical sciences