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Title: Plethora of transitions during breakup of liquid filaments

Journal Article · · Proceedings of the National Academy of Sciences of the United States of America
 [1];  [2];  [3];  [3];  [1];  [4];  [4];  [3]
  1. Department of Engineering, University of Cambridge, Cambridge CB3 0FS, United Kingdom,
  2. Department of Engineering Science, University of Oxford, Oxford OX1 3PJ, United Kingdom,
  3. School of Chemical Engineering, Purdue University, West Lafayette, IN 47907-1283, and
  4. Department of Applied Mathematics and Theoretical Physics, University of Cambridge, Cambridge CB3 0WA, United Kingdom

Thinning and breakup of liquid filaments are central to dripping of leaky faucets, inkjet drop formation, and raindrop fragmentation. As the filament radius decreases, curvature and capillary pressure, both inversely proportional to radius, increase and fluid is expelled with increasing velocity from the neck. As the neck radius vanishes, the governing equations become singular and the filament breaks. In slightly viscous liquids, thinning initially occurs in an inertial regime where inertial and capillary forces balance. By contrast, in highly viscous liquids, initial thinning occurs in a viscous regime where viscous and capillary forces balance. As the filament thins, viscous forces in the former case and inertial forces in the latter become important, and theory shows that the filament approaches breakup in the final inertial–viscous regime where all three forces balance. However, previous simulations and experiments reveal that transition from an initial to the final regime either occurs at a value of filament radius well below that predicted by theory or is not observed. In this paper, we perform new simulations and experiments, and show that a thinning filament unexpectedly passes through a number of intermediate transient regimes, thereby delaying onset of the inertial–viscous regime. Finally, the new findings have practical implications regarding formation of undesirable satellite droplets and also raise the question as to whether similar dynamical transitions arise in other free-surface flows such as coalescence that also exhibit singularities.

Research Organization:
Purdue Univ., West Lafayette, IN (United States); Univ. of Cambridge (United Kingdom)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Procter & Gamble (United States); Chevron Corporation (United States); Engineering and Physical Sciences Research Council (EPSRC); John Fell Oxford Univ. Press Research Fund (United Kingdom); Royal Society (United Kingdom)
Contributing Organization:
Univ. of Oxford (United Kingdom)
Grant/Contract Number:
FG02-96ER14641; EP/H018913/1
OSTI ID:
1235161
Alternate ID(s):
OSTI ID: 1349047
Journal Information:
Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Vol. 112 Journal Issue: 15; ISSN 0027-8424
Publisher:
Proceedings of the National Academy of SciencesCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 132 works
Citation information provided by
Web of Science

References (36)

Coalescence of liquid drops journal December 1999
On The Instability Of Jets journal November 1878
Capillary breakup of a viscous thread surrounded by another viscous fluid journal November 1998
Computational and experimental analysis of dynamics of drop formation journal December 1999
Computational and Experimental Analysis of Pinch-Off and Scaling journal April 2002
MATERIALS SCIENCE: Printing Cells journal October 2007
High Yield, Single Droplet Electrode Arrays for Nanoscale Printed Electronics journal February 2010
Discretization of free surface flows and other moving boundary problems journal March 1992
Nonstandard Inkjets journal January 2013
DNA Microarray Technology Devices, Systems, and Applications journal August 2002
Measurement of Dynamic Surface Tension by a Growing Drop Technique journal November 1994
Self-Similar Capillary Pinchoff of an Inviscid Fluid journal January 1998
Fabrication of PLG microspheres with precisely controlled and monodisperse size distributions journal May 2001
High-Resolution Inkjet Printing of All-Polymer Transistor Circuits journal December 2000
On the breakup of viscous liquid threads journal July 1995
Surface Tension Driven Flows journal April 1983
Breakup of electrified jets journal September 2007
Theoretical Analysis of a Dripping Faucet journal December 2000
Analysis of the drop weight method journal June 2005
Universal pinching of 3D axisymmetric free-surface flow journal November 1993
The inexorable resistance of inertia determines the initial regime of drop coalescence journal April 2012
Single-molecule analysis of ultradilute solutions with guided streams of 1-µm water droplets journal January 1999
Dynamics of inviscid capillary breakup: collapse and pinchoff of a film bridge journal June 1997
Solvent Exchange Method: A Novel Microencapsulation Technique Using Dual Microdispensers journal August 2004
Small-scale free surface flows with breakup: Drop formation and emerging applications journal September 2002
Deformation and breakup of a stretching liquid bridge covered with an insoluble surfactant monolayer journal February 2006
Nonlinear dynamics and breakup of free-surface flows journal July 1997
Transition from Symmetric to Asymmetric Scaling Function before Drop Pinch-Off journal August 2001
Local dynamics during pinch-off of liquid threads of power law fluids: Scaling analysis and self-similarity journal October 2006
Drop formation - an overview journal June 2005
Future, Opportunities and Challenges of Inkjet Technologies journal January 2013
Dripping-Jetting Transitions in a Dripping Faucet journal July 2004
Single-drop fragmentation determines size distribution of raindrops journal July 2009
Formation of beads-on-a-string structures during break-up of viscoelastic filaments journal June 2010
Physics of liquid jets journal February 2008
Electric Field Driven Separations: Phenomena and Applications journal July 1992

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