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Title: Achieving atomic resolution magnetic dichroism by controlling the phase symmetry of an electron probe

Journal Article · · Physical Review Letters
 [1];  [2];  [3]
  1. Uppsala Univ., Uppsala (Sweden)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Indian Institute of Technology, Kanpur (India)

The calculations presented here reveal that an electron probe carrying orbital angular momentum is just a particular case of a wider class of electron beams that can be used to measure electron magnetic circular dichroism (EMCD) with atomic resolution. It is possible to obtain an EMCD signal with atomic resolution by simply breaking the symmetry of the electron probe phase front using the aberration-corrected optics of a scanning transmission electron microscope. The probe’s required phase distribution depends on the sample’s magnetic symmetry and crystal structure. The calculations indicate that EMCD signals that use the electron probe’s phase are as strong as those obtained by nanodiffraction methods.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1213313
Journal Information:
Physical Review Letters, Vol. 113, Issue 14; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 37 works
Citation information provided by
Web of Science

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Cited By (11)

Scanning Transmission Electron Microscopy book January 2019
Magnetic measurements with atomic-plane resolution journal August 2016
Three-dimensional nanomagnetism journal June 2017
Atomic scale imaging of magnetic circular dichroism by achromatic electron microscopy journal February 2018
Probing the localization of magnetic dichroism by atomic-size astigmatic and vortex electron beams journal March 2018
Atomic-scale mapping of interface reconstructions in multiferroic heterostructures journal December 2018
Prospect for detecting magnetism of a single impurity atom using electron magnetic chiral dichroism journal September 2019
Detecting magnetic ordering with atomic size electron probes journal May 2016
Three-dimensional nanomagnetism text January 2017
Scanning Transmission Electron Microscopy book January 2007
Using electron vortex beams to determine chirality of crystals in transmission electron microscopy text January 2014