Raman vibrational spectra of bulk to monolayer ReS2 with lower symmetry

Feng, Yanqing; Zhou, Wei; Wang, Yaojia; Zhou, Jian; Liu, Erfu; Fu, Yajun; Ni, Zhenhua; Wu, Xinglong; Yuan, Hongtao; Miao, Feng; Wang, Baigeng; Wan, Xiangang; Xing, Dingyu

doi:10.1103/PhysRevB.92.054110

Raman vibrational spectra of bulk to monolayer $Re S_{2}$ with lower symmetry

Journal Article · Wed Aug 26 00:00:00 EDT 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.92.054110· OSTI ID:1326980

Feng, Yanqing ^[1]; Zhou, Wei ^[1]; Wang, Yaojia ^[1]; Zhou, Jian ^[1]; Liu, Erfu ^[1]; Fu, Yajun ^[1]; Ni, Zhenhua ^[2]; Wu, Xinglong ^[1]; Yuan, Hongtao ^[3]; Miao, Feng ^[1]; Wang, Baigeng ^[1]; Wan, Xiangang ^[1]; Xing, Dingyu ^[1]

Nanjing Univ., Nanjing (China)
Southeast Univ., Nanjing (China)
Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

Lattice structure and symmetry of two-dimensional (2D) layered materials are of key importance to their fundamental mechanical, thermal, electronic and optical properties. Raman spectroscopy, as a convenient and nondestructive tool, however has its limitations on identifying all symmetry allowing Raman modes and determining the corresponding crystal structure of 2D layered materials with high symmetry like graphene and MoS₂. Due to lower structural symmetry and extraordinary weak interlayer coupling of ReS₂, we successfully identified all 18 first-order Raman active modes for bulk and monolayer ReS₂. Without van der Waals (vdW) correction, our local density approximation (LDA) calculations successfully reproduce all the Raman modes. Our calculations also suggest no surface reconstruction effect and the absence of low frequency rigid-layer Raman modes below 100 cm^-1. As a result, combining with Raman and LDA thus provides a general approach for studying the vibrational and structural properties of 2D layered materials with lower symmetry.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1326980

Alternate ID(s):: OSTI ID: 1213111

Report Number(s):: SLAC-PUB--16716

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Issue: 5 Vol. 92; ISSN 1098-0121; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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