Monolayer PtSe 2 , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt

Wang, Yeliang; Li, Linfei; Yao, Wei; Song, Shiru; Sun, J. T.; Pan, Jinbo; Ren, Xiao; Li, Chen; Okunishi, Eiji; Wang, Yu-Qi; Wang, Eryin; Shao, Yan; Zhang, Y. Y.; Yang, Hai-tao; Schwier, Eike F.; Iwasawa, Hideaki; Shimada, Kenya; Taniguchi, Masaki; Cheng, Zhaohua; Zhou, Shuyun; Du, Shixuan; Pennycook, Stephen J.; Pantelides, Sokrates T.; Gao, Hong-Jun

doi:10.1021/acs.nanolett.5b00964

Monolayer PtSe ₂ , a New Semiconducting Transition-Metal-Dichalcogenide, Epitaxially Grown by Direct Selenization of Pt

Journal Article · Thu May 21 00:00:00 EDT 2015 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.5b00964· OSTI ID:1185929

Wang, Yeliang ^[1]; Li, Linfei ^[2]; Yao, Wei ^[3]; Song, Shiru ^[2]; Sun, J. T. ^[2]; Pan, Jinbo ^[2]; Ren, Xiao ^[2]; Li, Chen ^[4]; Okunishi, Eiji ^[5]; Wang, Yu-Qi ^[2]; Wang, Eryin ^[3]; Shao, Yan ^[2]; Zhang, Y. Y. ^[6]; Yang, Hai-tao ^[2]; Schwier, Eike F. ^[7]; Iwasawa, Hideaki ^[7]; Shimada, Kenya ^[7]; Taniguchi, Masaki ^[7]; Cheng, Zhaohua ^[2]; Zhou, Shuyun ^[8] more »

Chinese Academy of Sciences (CAS), Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
Chinese Academy of Sciences (CAS), Beijing (China)
Tsinghua Univ., Beijing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Jeol Ltd., Tokyo (Japan)
Chinese Academy of Sciences (CAS), Beijing (China); Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Hiroshima Univ., Higashi-Hiroshima (Japan)
Tsinghua Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
National Univ. of Singapore (Singapore)
Vanderbilt Univ., Nashville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

For single-layer transition-metal dichalcogenides (TMDs) receive significant attention due to their intriguing physical properties for both fundamental research and potential applications in electronics, optoelectronics, spintronics, catalysis, and so on. Here, we demonstrate the epitaxial growth of high-quality single-crystal, monolayer platinum diselenide (PtSe2), a new member of the layered TMDs family, by a single step of direct selenization of a Pt(111) substrate. We found that a combination of atomic-resolution experimental characterizations and first-principle theoretic calculations reveals the atomic structure of the monolayer PtSe2/Pt(111). Angle-resolved photoemission spectroscopy measurements confirm for the first time the semiconducting electronic structure of monolayer PtSe2 (in contrast to its semimetallic bulk counterpart). The photocatalytic activity of monolayer PtSe2 film is evaluated by a methylene-blue photodegradation experiment, demonstrating its practical application as a promising photocatalyst. Moreover, circular polarization calculations predict that monolayer PtSe2 has also potential applications in valleytronics.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Vanderbilt Univ., Nashville, TN (United States)

Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E)

Grant/Contract Number:: AC05-00OR22725; FG02-09ER46554

OSTI ID:: 1185929

Alternate ID(s):: OSTI ID: 1597683

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 6 Vol. 15; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Quantum anomalous Hall effect in a stable 1T-YN ₂ monolayer with a large nontrivial bandgap and a high Chern number Kong, Xiangru; Li, Linyang; Leenaerts, Ortwin Nanoscale, Vol. 10, Issue 17 https://doi.org/10.1039/c8nr00571k	journal	January 2018
Emerging 2D materials beyond graphene for ultrashort pulse generation in fiber lasers He, Junshan; Tao, Lili; Zhang, Han Nanoscale, Vol. 11, Issue 6 https://doi.org/10.1039/c8nr09368g	journal	January 2019
Charge carrier injection and transport engineering in two-dimensional transition metal dichalcogenides Durán Retamal, José Ramón; Periyanagounder, Dharmaraj; Ke, Jr-Jian Chemical Science, Vol. 9, Issue 40 https://doi.org/10.1039/c8sc02609b	journal	January 2018
Two-dimensional Janus PtSSe for photocatalytic water splitting under the visible or infrared light Peng, Rui; Ma, Yandong; Huang, Baibiao Journal of Materials Chemistry A, Vol. 7, Issue 2 https://doi.org/10.1039/c8ta09177c	journal	January 2019
Novel structures of two-dimensional tungsten boride and their superconductivity Yan, Luo; Bo, Tao; Zhang, Wenxue Physical Chemistry Chemical Physics, Vol. 21, Issue 28 https://doi.org/10.1039/c9cp02727k	journal	January 2019
Controlled assembly of artificial 2D materials based on the transfer of oxo-functionalized graphene Hußmann, Marleen; Weintrub, Benjamin; Feicht, Patrick Nanoscale Advances, Vol. 2, Issue 1 https://doi.org/10.1039/c9na00594c	journal	January 2020
The visible nonlinear optical properties and passively Q-switched laser application of a layered PtSe ₂ material Cui, Na; Zhang, Feng; Zhao, Yuqing Nanoscale, Vol. 12, Issue 2 https://doi.org/10.1039/c9nr08980b	journal	January 2020
2D material broadband photodetectors Yao, Jiandong; Yang, Guowei Nanoscale, Vol. 12, Issue 2 https://doi.org/10.1039/c9nr09070c	journal	January 2020
Magnetism and magnetocrystalline anisotropy in single-layer PtSe ₂ : Interplay between strain and vacancy Zhang, Wei; Guo, Hai Tao; Jiang, Jing Journal of Applied Physics, Vol. 120, Issue 1 https://doi.org/10.1063/1.4955468	journal	July 2016
Epitaxial fabrication of two-dimensional NiSe ₂ on Ni(111) substrate Shao, Yan; Song, Shiru; Wu, Xu Applied Physics Letters, Vol. 111, Issue 11 https://doi.org/10.1063/1.4991065	journal	September 2017
Review of mid-infrared mode-locked laser sources in the 2.0 μ m–3.5 μ m spectral region Ma, Jie; Qin, Zhipeng; Xie, Guoqiang Applied Physics Reviews, Vol. 6, Issue 2 https://doi.org/10.1063/1.5037274	journal	June 2019
2D WSe ₂ /MoS ₂ van der Waals heterojunction photodiode for visible-near infrared broadband detection Lee, Hyo Sun; Ahn, Jongtae; Shim, Wooyoung Applied Physics Letters, Vol. 113, Issue 16 https://doi.org/10.1063/1.5042440	journal	October 2018
A low-temperature scanning probe microscopy system with molecular beam epitaxy and optical access Wu, Ze-Bin; Gao, Zhao-Yan; Chen, Xi-Ya Review of Scientific Instruments, Vol. 89, Issue 11 https://doi.org/10.1063/1.5046466	journal	November 2018
Tuning the electronic structures and transport coefficients of Janus PtSSe monolayer with biaxial strain Guo, San-Dong; Guo, Xiao-Shu; Deng, Ye Journal of Applied Physics, Vol. 126, Issue 15 https://doi.org/10.1063/1.5124677	journal	October 2019
Tunable giant Rashba-type spin splitting in PtSe ₂ /MoSe ₂ heterostructure Xiang, Longjun; Ke, Youqi; Zhang, Qingyun Applied Physics Letters, Vol. 115, Issue 20 https://doi.org/10.1063/1.5125303	journal	November 2019
Janus PtSSe and graphene heterostructure with tunable Schottky barrier Cao, Liemao; Ang, Yee Sin; Wu, Qingyun Applied Physics Letters, Vol. 115, Issue 24 https://doi.org/10.1063/1.5130756	journal	December 2019
Planar Hall effect in PtSe ₂ Li, Zhaoguo; Xiao, Tingting; Zou, Ruijiao Journal of Applied Physics, Vol. 127, Issue 5 https://doi.org/10.1063/1.5133809	journal	February 2020
Thickness-dependent ultrafast nonlinear absorption properties of PtSe ₂ films with both semiconducting and semimetallic phases Zhao, Xin; Liu, Fang; Liu, Dongqi Applied Physics Letters, Vol. 115, Issue 26 https://doi.org/10.1063/1.5135375	journal	December 2019
Ferromagnetism regulated by edged cutting and optical identification in monolayer PtSe ₂ nanoribbons Meng, Ming; Zhang, QiZhen; Wang, Lifen Journal of Physics D: Applied Physics, Vol. 51, Issue 22 https://doi.org/10.1088/1361-6463/aabf30	journal	May 2018
Photoresponse of wafer-scale palladium diselenide films prepared by selenization method Mak, Chun Hin; Lin, Shenghuang; Rogée, Lukas Journal of Physics D: Applied Physics, Vol. 53, Issue 6 https://doi.org/10.1088/1361-6463/ab57a8	journal	December 2019
Inversion symmetry breaking induced triply degenerate points in orderly arranged PtSeTe family materials Xiao, R. C.; Cheung, C. H.; Gong, P. L. Journal of Physics: Condensed Matter, Vol. 30, Issue 24 https://doi.org/10.1088/1361-648x/aac298	journal	May 2018
Engineering the magnetic properties of PtSe ₂ monolayer through transition metal doping Kar, Moumita; Sarkar, Ritabrata; Pal, Sougata Journal of Physics: Condensed Matter, Vol. 31, Issue 14 https://doi.org/10.1088/1361-648x/aaff40	journal	February 2019
Structural, vibrational and electrical properties of type-II Dirac semimetal PtSe ₂ under high pressure An, Chao; Chen, Xuliang; Zhou, Yonghui Journal of Physics: Condensed Matter, Vol. 31, Issue 41 https://doi.org/10.1088/1361-648x/ab315e	journal	July 2019
Structural engineering of bilayer PtSe ₂ thin films: a first-principles study Fang, Limei; Liang, Weizheng; Feng, Qingguo Journal of Physics: Condensed Matter, Vol. 31, Issue 45 https://doi.org/10.1088/1361-648x/ab34bc	journal	August 2019
Suppression of magnetoresistance in PtSe ₂ microflakes with antidot arrays Li, Zhaoguo; Zeng, Yong; Zhou, Minjie Nanotechnology, Vol. 29, Issue 40 https://doi.org/10.1088/1361-6528/aad349	journal	July 2018
PtSe ₂ /graphene hetero-multilayer: gate-tunable Schottky barrier height and contact type Xia, Congxin; Du, Juan; Fang, Lizhen Nanotechnology, Vol. 29, Issue 46 https://doi.org/10.1088/1361-6528/aaddb9	journal	September 2018
Temperature dependence of Raman responses of few-layer PtS ₂ Pi, Lejing; Li, Liang; Hu, Xiaozong Nanotechnology, Vol. 29, Issue 50 https://doi.org/10.1088/1361-6528/aae41f	journal	October 2018
Structural, electronic and phononic properties of PtSe ₂ : from monolayer to bulk Kandemir, A.; Akbali, B.; Kahraman, Z. Semiconductor Science and Technology, Vol. 33, Issue 8 https://doi.org/10.1088/1361-6641/aacba2	journal	June 2018
The Computational 2D Materials Database: high-throughput modeling and discovery of atomically thin crystals Haastrup, Sten; Strange, Mikkel; Pandey, Mohnish 2D Materials, Vol. 5, Issue 4 https://doi.org/10.1088/2053-1583/aacfc1	journal	September 2018
Experimental progress on layered topological semimetals Ma, Junchao; Deng, Ke; Zheng, Lu 2D Materials, Vol. 6, Issue 3 https://doi.org/10.1088/2053-1583/ab0902	journal	April 2019
Optical properties of chemical vapor deposition-grown PtSe ₂ characterized by spectroscopic ellipsometry Xie, Junfang; Zhang, Di; Yan, Xiao-Qing 2D Materials, Vol. 6, Issue 3 https://doi.org/10.1088/2053-1583/ab1490	journal	April 2019
PtSe ₂ grown directly on polymer foil for use as a robust piezoresistive sensor Boland, Conor S.; Coileáin, Cormac Ó; Wagner, Stefan 2D Materials, Vol. 6, Issue 4 https://doi.org/10.1088/2053-1583/ab33a1	journal	August 2019
Visualization of point defects in ultrathin layered 1T-PtSe ₂ Zheng, Husong; Choi, Yichul; Baniasadi, Fazel 2D Materials, Vol. 6, Issue 4 https://doi.org/10.1088/2053-1583/ab3beb	journal	September 2019
First-principles study on the gas sensing property of the Ge, As, and Br doped PtSe ₂ Zhang, Jing; Yang, Gui; Tian, Junlong Materials Research Express, Vol. 5, Issue 3 https://doi.org/10.1088/2053-1591/aab4e3	journal	March 2018
Hydrogen-induced ferromagnetism in two-dimensional Pt dichalcogenides Manchanda, P.; Enders, A.; Sellmyer, D. J. Physical Review B, Vol. 94, Issue 10 https://doi.org/10.1103/physrevb.94.104426	journal	September 2016
Experimental evidence for type-II Dirac semimetal in PtSe 2 Zhang, Kenan; Yan, Mingzhe; Zhang, Haoxiong Physical Review B, Vol. 96, Issue 12 https://doi.org/10.1103/physrevb.96.125102	journal	September 2017
Observation of negative longitudinal magnetoresistance in the type-II Dirac semimetal PtSe 2 Li, Zhaoguo; Zeng, Yong; Zhang, Jicheng Physical Review B, Vol. 98, Issue 16 https://doi.org/10.1103/physrevb.98.165441	journal	October 2018
Novel Pd 2 Se 3 Two-Dimensional Phase Driven by Interlayer Fusion in Layered PdSe 2 Lin, Junhao; Zuluaga, Sebastian; Yu, Peng Physical Review Letters, Vol. 119, Issue 1 https://doi.org/10.1103/physrevlett.119.016101	journal	July 2017
3D Dirac Plasmons in the Type-II Dirac Semimetal PtTe 2 Politano, Antonio; Chiarello, Gennaro; Ghosh, Barun Physical Review Letters, Vol. 121, Issue 8 https://doi.org/10.1103/physrevlett.121.086804	journal	August 2018
Dimensionality-Mediated Semimetal-Semiconductor Transition in Ultrathin PtTe 2 Films Lin, Meng-Kai; Villaos, Rovi Angelo B.; Hlevyack, Joseph A. Physical Review Letters, Vol. 124, Issue 3 https://doi.org/10.1103/physrevlett.124.036402	journal	January 2020
Tunable electron-phonon coupling superconductivity in platinum diselenide Cheng, Cai; Sun, Jia-Tao; Liu, Min Physical Review Materials, Vol. 1, Issue 7 https://doi.org/10.1103/physrevmaterials.1.074804	journal	December 2017
Bilayer platinum diselenide saturable absorber for 20 μm passively Q-switched bulk lasers Yan, Bingzheng; Zhang, Baitao; Nie, Hongkun Optics Express, Vol. 26, Issue 24 https://doi.org/10.1364/oe.26.031657	journal	January 2018
Bulk-structured PtSe ₂ for femtosecond fiber laser mode-locking Huang, Bin; Du, Lin; Yi, Qian Optics Express, Vol. 27, Issue 3 https://doi.org/10.1364/oe.27.002604	journal	January 2019
Vertically standing PtSe ₂ film: a saturable absorber for a passively mode-locked Nd:LuVO ₄ laser Tao, Lili; Huang, Xiaowen; He, Junshan Photonics Research, Vol. 6, Issue 7 https://doi.org/10.1364/prj.6.000750	journal	January 2018
Q-switched and mode-locked Er-doped fiber laser using PtSe ₂ as a saturable absorber Zhang, Kang; Feng, Ming; Ren, Yangyang Photonics Research, Vol. 6, Issue 9 https://doi.org/10.1364/prj.6.000893	journal	January 2018
Direct observation of interlayer coherent acoustic phonon dynamics in bilayer and few-layer PtSe ₂ Chen, Xin; Zhang, Saifeng; Wang, Lei Photonics Research, Vol. 7, Issue 12 https://doi.org/10.1364/prj.7.001416	journal	January 2019
Controlled assembly of artificial 2D materials based on the transfer of oxo-functionalized graphene Hußmann, Marleen; Weintrub, Benjamin; Feicht, Patrick Freie Universität Berlin https://doi.org/10.17169/refubium-26715	text	January 2019
Electrical devices from top-down structured platinum diselenide films Yim, Chanyoung; Passi, Vikram; Lemme, Max Christian RWTH Aachen University https://doi.org/10.18154/rwth-conv-224671	text	January 2018
Tuning the Catalytic Activity of a Quantum Nutcracker for Hydrogen Dissociation Tao, Lei; Zhang, Yu-Yang; Pantelides, Sokrates T. Surfaces, Vol. 3, Issue 1 https://doi.org/10.3390/surfaces3010004	journal	January 2020
Lorentz-violating type-II Dirac fermions in transition metal dichalcogenide PtTe$_2$ Yan, Mingzhe; Huang, Huaqing; Zhang, Kenan arXiv https://doi.org/10.48550/arxiv.1607.03643	text	January 2016
Low-Temperature Eutectic Synthesis of PtTe2 with Weak Antilocalization and Controlled Layer Thinning Hao, Song; Zeng, Junwen; Xu, Tao arXiv https://doi.org/10.48550/arxiv.1808.02283	text	January 2018
Experimental Progress on Layered Topological Semimetals Ma, Junchao; Deng, Ke; Zheng, Lu arXiv https://doi.org/10.48550/arxiv.1902.06874	text	January 2019
PtSe2 grown directly on polymer foil for use as a robust piezoresistive sensor Boland, Conor S.; Coileáin, Cormac Ó; Wagner, Stefan arXiv https://doi.org/10.48550/arxiv.1903.11894	preprint	January 2019
Van der Waals heterostructures for high-performance device applications: challenges and opportunities Liang, Shi-Jun; Cheng, Bin; Cui, Xinyi arXiv https://doi.org/10.48550/arxiv.1912.10886	text	January 2019

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36 MATERIALS SCIENCE
PtSe2
epitaxial growth
monolayer
photocatalyst
transition-metal dichalcogenides
two-dimensional materials