Optical Control of Fluorescence through plasmonic eigenmode extinction

Xu, Xiaoying; Lin, Shih-Che; Li, Quanshui; Zhang, Zhili; Ivanov, Ilia N.; Li, Yuan; Wang, Wenbin; Gu, Baohua; Zhang, Zhenyu; Hsueh, C. H.; Snijders, Paul C.; Seal, Katyayani

doi:10.1038/srep09911

Title: Optical Control of Fluorescence through plasmonic eigenmode extinction

Journal Article · Thu Apr 30 00:00:00 EDT 2015 · Scientific Reports

DOI:https://doi.org/10.1038/srep09911· OSTI ID:1185351

Xu, Xiaoying ^[1]; Lin, Shih-Che ^[2]; Li, Quanshui ^[3]; Zhang, Zhili ^[3]; Ivanov, Ilia N. ^[1]; Li, Yuan ^[1]; Wang, Wenbin ^[1]; Gu, Baohua ^[1]; Zhang, Zhenyu ^[4]; Hsueh, C. H. ^[2]; Snijders, Paul C. ^[1]; Seal, Katyayani ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
National Taiwan Univ., Taipei (Taiwan)
Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Science and Technology of China, Hefei (China). International Center for Quantum Design of Functional Materials (ICQD)

We introduce the concept of optical control of the fluorescence yield of CdSe quantum dots through plasmon-induced structural changes in random semicontinuous nanostructured gold films. We demonstrate that the wavelength- and polarization dependent coupling between quantum dots and the semicontinuous films, and thus the fluorescent emission spectrum, can be controlled and significantly increased through the optical extinction of a selective band of eigenmodes in the films. This optical method of effecting controlled changes in the metal nanostructure allows for versatile functionality in a single sample and opens a pathway to in situ control over the fluorescence spectrum.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1185351

Journal Information:: Scientific Reports, Vol. 5; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 4 works

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