skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Perspective: Extremely fine tuning of doping enabled by combinatorial molecular-beam epitaxy

Journal Article · · APL Materials
DOI:https://doi.org/10.1063/1.4917283· OSTI ID:1179642

Chemical doping provides an effective method to control the electric properties of complex oxides. However, the state-of-art accuracy in controlling doping is limited to about 1%. This hampers elucidation of the precise doping dependences of physical properties and phenomena of interest, such as quantum phase transitions. Using the combinatorial molecular beam epitaxy, we improve the accuracy in tuning the doping level by two orders of magnitude. We illustrate this novel method by two examples: a systematic investigation of the doping dependence of interface superconductivity, and a study of the competing ground states in the vicinity of the insulator-to-superconductor transition.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC00112704
OSTI ID:
1179642
Alternate ID(s):
OSTI ID: 1226035; OSTI ID: 1421208
Report Number(s):
BNL-108324-2015-JA
Journal Information:
APL Materials, Journal Name: APL Materials Vol. 3 Journal Issue: 6; ISSN 2166-532X
Publisher:
American Institute of PhysicsCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 13 works
Citation information provided by
Web of Science

References (12)

Photoinduced expansion of cuprate superconductors: Evidence of strong electron-lattice coupling journal March 2008
COMBE: A Powerful New Tool for Materials Science journal August 2000
Combinatorial molecular beam epitaxy of La2−xSrxCuO4+δ journal September 2007
Combinatorial measurements of Hall effect and resistivity in oxide films journal March 2008
Statistical Characterization and Process Control for Improved Growth of La2−x Sr x CuO4 Films journal June 2009
High-temperature interface superconductivity between metallic and insulating copper oxides journal October 2008
High-Temperature Superconductivity in a Single Copper-Oxygen Plane journal October 2009
Anomalous independence of interface superconductivity from carrier density journal August 2013
Superconductor‐Insulator Transitions in the Two‐Dimensional Limit journal November 1998
Superconductor–insulator quantum phase transition journal January 2010
Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance journal April 2011
Electrostatic Control of the Evolution from a Superconducting Phase to an Insulating Phase in Ultrathin YBa 2 Cu 3 O 7 x Films journal July 2011