Zirconia and Pyrochlore Oxides for Thermal Barrier Coatings in Gas Turbine Engines

Fergus, Jeffrey W.

doi:10.1007/s40553-014-0012-y

Zirconia and Pyrochlore Oxides for Thermal Barrier Coatings in Gas Turbine Engines

Journal Article · Sat Apr 12 00:00:00 EDT 2014 · Metallurgical and Materials Transactions. E, Materials for Energy Systems

DOI:https://doi.org/10.1007/s40553-014-0012-y· OSTI ID:1178999

Fergus, Jeffrey W. ^[1]

Auburn University, Auburn, AL (United States). Materials Research and Education Center; Auburn University

One of the important applications of yttria stabilized zirconia is as a thermal barrier coating for gas turbine engines. While yttria stabilized zirconia performs well in this function, the need for increased operating temperatures to achieve higher energy conversion efficiencies, requires the development of improved materials. To meet this challenge, some rare-earth zirconates that form the cubic fluorite derived pyrochlore structure are being developed for use in thermal barrier coatings due to their low thermal conductivity, excellent chemical stability and other suitable properties. In this paper, the thermal conductivities of current and prospective oxides for use in thermal barrier coatings are reviewed. The factors affecting the variations and differences in the thermal conductivities and the degradation behaviors of these materials are discussed.

View Accepted Manuscript (DOE)

Research Organization:: Auburn University, Auburn, AL (United States)

Sponsoring Organization:: USDOE Office of Fossil Energy (FE), Clean Coal and Carbon (FE-20)

Contributing Organization:: Auburn University

Grant/Contract Number:: FE0011245

OSTI ID:: 1178999

Journal Information:: Metallurgical and Materials Transactions. E, Materials for Energy Systems, Journal Name: Metallurgical and Materials Transactions. E, Materials for Energy Systems Journal Issue: 2 Vol. 1; ISSN 2196-2936

Publisher:: ASM InternationalCopyright Statement

Country of Publication:: United States

Language:: English

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Reaction, transformation and delamination of samarium zirconate thermal barrier coatings Zhao, Hengbei; Begley, Matthew R.; Heuer, Arthur Surface and Coatings Technology, Vol. 205, Issue 19 https://doi.org/10.1016/j.surfcoat.2011.03.028	journal	June 2011
Correlation of thermal conductivity changes with anisotropic nano-pores of EB-PVD deposited FYSZ-coatings Saruhan, Bilge; Ryukhtin, Vasyl; Kelm, Klemens Surface and Coatings Technology, Vol. 205, Issue 23-24 https://doi.org/10.1016/j.surfcoat.2011.05.051	journal	September 2011
Cyclic oxidation behavior and thermal barrier effect of YSZ–(Al2O3/YAG) double-layer TBCs prepared by the composite sol–gel method Ren, C.; He, Y. D.; Wang, D. R. Surface and Coatings Technology, Vol. 206, Issue 6 https://doi.org/10.1016/j.surfcoat.2011.09.025	journal	December 2011
Plasma sprayed gadolinium zirconate thermal barrier coatings that are resistant to damage by molten Ca–Mg–Al–silicate glass Drexler, Julie M.; Chen, Chun-Hu; Gledhill, Andrew D. Surface and Coatings Technology, Vol. 206, Issue 19-20 https://doi.org/10.1016/j.surfcoat.2012.03.051	journal	May 2012
Calcium–magnesium–alumino-silicate (CMAS) degradation of EB-PVD thermal barrier coatings: Characterization of CMAS damage on ex-service high pressure blade TBCs Vidal-Setif, M. H.; Chellah, N.; Rio, C. Surface and Coatings Technology, Vol. 208 https://doi.org/10.1016/j.surfcoat.2012.07.074	journal	September 2012
Lanthanum zirconate thermal barrier coatings deposited by spray pyrolysis Weber, Sophie B.; Lein, Hilde L.; Grande, Tor Surface and Coatings Technology, Vol. 227 https://doi.org/10.1016/j.surfcoat.2012.09.019	journal	July 2013
Preparation and thermophysical properties of La2(Zr0.7Ce0.3)2O7 ceramic via sol–gel process Wang, Chunjie; Wang, Yue; Fan, Xizhi Surface and Coatings Technology, Vol. 212 https://doi.org/10.1016/j.surfcoat.2012.09.026	journal	November 2012
Local stress evolution in thermal barrier coating system during isothermal growth of irregular oxide layer Sun, Yongle; Li, Jianguo; Zhang, Weixu Surface and Coatings Technology, Vol. 216 https://doi.org/10.1016/j.surfcoat.2012.11.052	journal	February 2013
The effect of vermiculite on the degradation and spallation of plasma sprayed thermal barrier coatings Shinozaki, M.; Clyne, T. W. Surface and Coatings Technology, Vol. 216 https://doi.org/10.1016/j.surfcoat.2012.11.054	journal	February 2013
Lifetime prediction of plasma-sprayed thermal barrier coating systems Wei, Shen; Fu-chi, Wang; Qun-bo, Fan Surface and Coatings Technology, Vol. 217 https://doi.org/10.1016/j.surfcoat.2012.11.069	journal	February 2013
Influence of temperature on phase stability and thermal conductivity of single- and double-ceramic-layer EB–PVD TBC top coats consisting of 7YSZ, Gd2Zr2O7 and La2Zr2O7 Bobzin, K.; Bagcivan, N.; Brögelmann, T. Surface and Coatings Technology, Vol. 237 https://doi.org/10.1016/j.surfcoat.2013.08.013	journal	December 2013
Calcium–magnesium aluminosilicate (CMAS) reactions and degradation mechanisms of advanced environmental barrier coatings Ahlborg, Nadia L.; Zhu, Dongming Surface and Coatings Technology, Vol. 237 https://doi.org/10.1016/j.surfcoat.2013.08.036	journal	December 2013
Anisotropic TGO morphology and stress distribution in EB-PVD Y2O3-ZrO2 thermal barrier coating after in-phase thermo-mechanical test Kitazawa, Rumi; Kakisawa, Hideki; Kagawa, Yutaka Surface and Coatings Technology, Vol. 238 https://doi.org/10.1016/j.surfcoat.2013.10.041	journal	January 2014
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Thermochemical Interaction of Thermal Barrier Coatings with Molten CaO?MgO?Al ₂ O ₃ ?SiO ₂ (CMAS) Deposits Krämer, Stephan; Yang, James; Levi, Carlos G. Journal of the American Ceramic Society, Vol. 89, Issue 10 https://doi.org/10.1111/j.1551-2916.2006.01209.x	journal	October 2006
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Perovskite-Type Strontium Zirconate as a New Material for Thermal Barrier Coatings Ma, Wen; Mack, Daniel E.; Vaßen, Robert Journal of the American Ceramic Society, Vol. 91, Issue 8 https://doi.org/10.1111/j.1551-2916.2008.02472.x	journal	August 2008
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The Tetragonal-Monoclinic Transformation in Zirconia: Lessons Learned and Future Trends Chevalier, Jérôme; Gremillard, Laurent; Virkar, Anil V. Journal of the American Ceramic Society, Vol. 92, Issue 9 https://doi.org/10.1111/j.1551-2916.2009.03278.x	journal	September 2009
Order-Disorder Transition and Unconventional Thermal Conductivities of the (Sm1−xYbx)2Zr2O7 Series: Order-Disorder Transition and Unconventional Thermal Conductivities Wan, Chunlei; Qu, Zhixue; Du, Aibing Journal of the American Ceramic Society, Vol. 94, Issue 2 https://doi.org/10.1111/j.1551-2916.2010.04113.x	journal	September 2010
High-Temperature Corrosion of EB-PVD Yttria Partially Stabilized Zirconia Thermal Barrier Coatings with an Artificial Volcanic Ash Overlay: HT-Corrosion of EB-PVD Y-PSZ TBC with an Artificial Volcanic Ash Overlay Mechnich, Peter; Braue, Wolfgang; Schulz, Uwe Journal of the American Ceramic Society, Vol. 94, Issue 3 https://doi.org/10.1111/j.1551-2916.2010.04166.x	journal	October 2010
Damage Evolution in Thermal Barrier Coatings with Thermal Cycling: Damage Evolution in Thermal Barrier Coatings Heeg, Bauke; Tolpygo, Vladimir K.; Clarke, David R. Journal of the American Ceramic Society, Vol. 94 https://doi.org/10.1111/j.1551-2916.2011.04496.x	journal	April 2011
Phase Stability of t′-Zirconia-Based Thermal Barrier Coatings: Mechanistic Insights: Phase Stability of t′-Zirconia-Based TBCs Krogstad, Jessica A.; Krämer, Stephan; Lipkin, Don M. Journal of the American Ceramic Society, Vol. 94 https://doi.org/10.1111/j.1551-2916.2011.04531.x	journal	May 2011
Recession of an EB-PVDYSZ Coated Turbine Blade by CaSO4 and Fe, Ti-Rich CMAS-Type Deposits Braue, Wolfgang; Mechnich, Peter Journal of the American Ceramic Society, Vol. 94, Issue 12 https://doi.org/10.1111/j.1551-2916.2011.04747.x	journal	July 2011
Phase Evolution upon Aging of Air-Plasma Sprayed t ′-Zirconia Coatings: I-Synchrotron X-Ray Diffraction Lipkin, Don M.; Krogstad, Jessica A.; Gao, Yan Journal of the American Ceramic Society, Vol. 96, Issue 1 https://doi.org/10.1111/j.1551-2916.2012.05451.x	journal	October 2012
Phase Evolution upon Aging of Air Plasma Sprayed t′-Zirconia Coatings: II-Microstructure Evolution Krogstad, Jessica A.; Leckie, Rafael M.; Krämer, Stephan Journal of the American Ceramic Society, Vol. 96, Issue 1 https://doi.org/10.1111/j.1551-2916.2012.05460.x	journal	October 2012
Effect of CMAS Infiltration on Radiative Transport Through an EB-PVD Thermal Barrier Coating Li, Li; Clarke, David R. International Journal of Applied Ceramic Technology, Vol. 5, Issue 3 https://doi.org/10.1111/j.1744-7402.2008.02225.x	journal	May 2008
CMAS-Resistant Thermal Barrier Coatings (TBC): CMAS-Resistant Thermal Barrier Coatings Rai, Amarendra K.; Bhattacharya, Rabi S.; Wolfe, Douglas E. International Journal of Applied Ceramic Technology, Vol. 7, Issue 5 https://doi.org/10.1111/j.1744-7402.2009.02373.x	journal	May 2009
Correlations Between Microstructure and Mechanical Properties of Air Plasma-Sprayed Thermal Barrier Coatings Exposed to a High Temperature Osorio, Julián D.; Maya, Deiby; Barrios, Augusto C. Journal of the American Ceramic Society, Vol. 96, Issue 12 https://doi.org/10.1111/jace.12621	journal	November 2013
Effects of RE ³⁺ Ionic Radius on Monoclinic Phase Content of 8 mol% REO _1.5 Partially Stabilized ZrO ₂ (RE = Yb, Y, Gd, and Nd) Powder Compacts after Annealing at High Temperature Jiang, Kuo; Liu, Songbai; Li, Yuan Journal of the American Ceramic Society, Vol. 97, Issue 3 https://doi.org/10.1111/jace.12733	journal	December 2013
Thermal Barrier Coatings for Gas-Turbine Engine Applications Padture, N. P. Science, Vol. 296, Issue 5566 https://doi.org/10.1126/science.1068609	journal	April 2002
Thermal barrier coatings technology: critical review, progress update, remaining challenges and prospects Darolia, R. International Materials Reviews, Vol. 58, Issue 6 https://doi.org/10.1179/1743280413Y.0000000019	journal	August 2013
Thermal Conductivity and Elastic Modulus Evolution of Thermal Barrier Coatings under High Heat Flux Conditions Zhu, Dongming; Miller, Robert A. Journal of Thermal Spray Technology, Vol. 9, Issue 2 https://doi.org/10.1361/105996300770349890	journal	June 2000
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Environmental degradation of thermal-barrier coatings by molten deposits Levi, Carlos G.; Hutchinson, John W.; Vidal-Sétif, Marie-Hélène MRS Bulletin, Vol. 37, Issue 10 https://doi.org/10.1557/mrs.2012.230	journal	October 2012
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Processing science of advanced thermal-barrier systems Sampath, Sanjay; Schulz, Uwe; Jarligo, Maria Ophelia MRS Bulletin, Vol. 37, Issue 10 https://doi.org/10.1557/mrs.2012.233	journal	October 2012
Low thermal conductivity oxides Pan, Wei; Phillpot, Simon R.; Wan, Chunlei MRS Bulletin, Vol. 37, Issue 10 https://doi.org/10.1557/mrs.2012.234	journal	October 2012
Multifunctional coating interlayers for thermal-barrier systems Pollock, T. M.; Lipkin, D. M.; Hemker, K. J. MRS Bulletin, Vol. 37, Issue 10 https://doi.org/10.1557/mrs.2012.238	journal	October 2012
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