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Non-acidic Pd/Y zeolite catalysts from organopalladium precursors: Preparation and catalytic activity in MCP reforming

Journal Article · · Journal of Catalysis
; ;  [1]
  1. Universita di Milano (Italy); and others
Pd/NaY and Pd/NaHY catalysts have been obtained by chemical vapor deposition of allylcyclopentadienylpalladium and characterized by temperature-programmed reductive decomposition and by EXAFS. In the conversion of methylcyclopentane at 300{degrees}C, the non-acidic catalyst shows a constant 100% selectivity towards ring-opening without significant coke deposition. In particular, the deactivation rate is lower than with the non-acidic system prepared by a conventional method. With the bifunctional Pd/NaHY catalyst ring enlargement is predominant, and significant coke deposition occurs as confirmed by temperature-programmed oxidation measurements. 20 refs., 11 figs.
OSTI ID:
110980
Journal Information:
Journal of Catalysis, Journal Name: Journal of Catalysis Journal Issue: 1 Vol. 149; ISSN 0021-9517; ISSN JCTLA5
Country of Publication:
United States
Language:
English

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