Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy

Paul, J.; Dey, P.; Tokumoto, T.; Reno, J. L.; Hilton, D. J.; Karaiskaj, D.

doi:10.1063/1.4896777

Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy

Journal Article · Tue Oct 07 00:00:00 EDT 2014 · Journal of Chemical Physics

DOI:https://doi.org/10.1063/1.4896777· OSTI ID:1083698

Paul, J. ^[1]; Dey, P. ^[1]; Tokumoto, T. ^[2]; Reno, J. L. ^[3]; Hilton, D. J. ^[2]; Karaiskaj, D. ^[1]

Univ. of South Florida, Tampa, FL (United States)
Univ. of Alabama at Birmingham, Birmingham, AL (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

The dephasing of excitons in a modulation doped single quantum well was carefully measured using time integrated four-wave mixing (FWM) and two-dimensional Fourier transform (2DFT) spectroscopy. These are the first 2DFT measurements performed on a modulation doped single quantum well. The inhomogeneous and homogeneous excitonic line widths were obtained from the diagonal and cross-diagonal profiles of the 2DFT spectra. The laser excitation density and temperature were varied and 2DFT spectra were collected. A very rapid increase of the dephasing decay, and as a result, an increase in the cross-diagonal 2DFT linewidths with temperature was observed. Furthermore, the lineshapes of the 2DFT spectra suggest the presence of excitation induced dephasing and excitation induced shift.

View Accepted Manuscript (DOE)

Research Organization:: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1083698

Alternate ID(s):: OSTI ID: 1223047
OSTI ID: 22436564

Report Number(s):: SAND--2013-4782J; 456279

Journal Information:: Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 13 Vol. 141; ISSN JCPSA6; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Evidence of biexcitonic contributions to four-wave mixing in GaAs quantum wells Mayer, E. J.; Smith, G. O.; Heuckeroth, V. Physical Review B, Vol. 50, Issue 19 https://doi.org/10.1103/PhysRevB.50.14730	journal	November 1994
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Role of excitation-induced shift in the coherent optical response of semiconductors Shacklette, Justin M.; Cundiff, Steven T. Physical Review B, Vol. 66, Issue 4 https://doi.org/10.1103/PhysRevB.66.045309	journal	July 2002
Coulomb correlations in a two-dimensional electron gas in large magnetic fields Fromer, N. A.; Schüller, C.; Lai, C. W. Physical Review B, Vol. 66, Issue 20 https://doi.org/10.1103/PhysRevB.66.205314	journal	November 2002
Ultrafast nonlinear optical response of strongly correlated systems: Dynamics in the quantum Hall effect regime Karathanos, A. T.; Perakis, I. E.; Fromer, N. A. Physical Review B, Vol. 67, Issue 3 https://doi.org/10.1103/PhysRevB.67.035316	journal	January 2003
Two-dimensional optical spectroscopy of excitons in semiconductor quantum wells: Liouville-space pathway analysis Yang, Lijun; Schweigert, Igor V.; Cundiff, Steven T. Physical Review B, Vol. 75, Issue 12 https://doi.org/10.1103/PhysRevB.75.125302	journal	March 2007
Revealing exciton-exciton couplings in semiconductors using multidimensional four-wave mixing signals Yang, Lijun; Mukamel, Shaul Physical Review B, Vol. 77, Issue 7 https://doi.org/10.1103/PhysRevB.77.075335	journal	February 2008
Observation of an inter-Landau level quantum coherence in semiconductor quantum wells Dani, K. M.; Cotoros, I. A.; Wang, J. Physical Review B, Vol. 78, Issue 4 https://doi.org/10.1103/PhysRevB.78.041301	journal	July 2008
Transient terahertz spectroscopy of excitons and unbound carriers in quasi-two-dimensional electron-hole gases Kaindl, R. A.; Hägele, D.; Carnahan, M. A. Physical Review B, Vol. 79, Issue 4 https://doi.org/10.1103/PhysRevB.79.045320	journal	January 2009
Polarization dependence of semiconductor exciton and biexciton contributions to phase-resolved optical two-dimensional Fourier-transform spectra Bristow, Alan D.; Karaiskaj, Denis; Dai, Xingcan Physical Review B, Vol. 79, Issue 16 https://doi.org/10.1103/PhysRevB.79.161305	journal	April 2009
Quantum beats due to excitonic ground-state splitting in colloidal quantum dots Bylsma, J.; Dey, P.; Paul, J. Physical Review B, Vol. 86, Issue 12 https://doi.org/10.1103/PhysRevB.86.125322	journal	September 2012
Spin Texture and Magnetoroton Excitations at ν = 1 / 3 Groshaus, Javier G.; Dujovne, Irene; Gallais, Yann Physical Review Letters, Vol. 100, Issue 4 https://doi.org/10.1103/PhysRevLett.100.046804	journal	January 2008
Two-Dimensional Correlation Spectroscopy of Two-Exciton Resonances in Semiconductor Quantum Wells Yang, Lijun; Mukamel, Shaul Physical Review Letters, Vol. 100, Issue 5 https://doi.org/10.1103/PhysRevLett.100.057402	journal	February 2008
First-Order Quantum Phase Transition of Excitons in Quantum Hall Bilayers Karmakar, Biswajit; Pellegrini, Vittorio; Pinczuk, Aron Physical Review Letters, Vol. 102, Issue 3 https://doi.org/10.1103/PhysRevLett.102.036802	journal	January 2009
Two-Quantum Many-Body Coherences in Two-Dimensional Fourier-Transform Spectra of Exciton Resonances in Semiconductor Quantum Wells Karaiskaj, Denis; Bristow, Alan D.; Yang, Lijun Physical Review Letters, Vol. 104, Issue 11 https://doi.org/10.1103/PhysRevLett.104.117401	journal	March 2010
Higher-Energy Composite Fermion Levels in the Fractional Quantum Hall Effect Rhone, Trevor D.; Majumder, Dwipesh; Dennis, Brian S. Physical Review Letters, Vol. 106, Issue 9 https://doi.org/10.1103/PhysRevLett.106.096803	journal	March 2011
Rapid Collapse of Spin Waves in Nonuniform Phases of the Second Landau Level Rhone, Trevor D.; Yan, Jun; Gallais, Yann Physical Review Letters, Vol. 106, Issue 19 https://doi.org/10.1103/PhysRevLett.106.196805	journal	May 2011
Coherent Coupling of Excitons and Trions in a Photoexcited CdTe/CdMgTe Quantum Well Moody, G.; Akimov, I. A.; Li, H. Physical Review Letters, Vol. 112, Issue 9 https://doi.org/10.1103/PhysRevLett.112.097401	journal	March 2014
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Optical investigations of the integer and fractional quantum Hall effects: Energy plateaus, intensity minima, and line splitting in band-gap emission Goldberg, B. B.; Heiman, D.; Pinczuk, A. Physical Review Letters, Vol. 65, Issue 5 https://doi.org/10.1103/PhysRevLett.65.641	journal	July 1990
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Collapse of Spin Excitations in Quantum Hall States of Coupled Electron Double Layers Pellegrini, Vittorio; Pinczuk, Aron; Dennis, Brian S. Physical Review Letters, Vol. 78, Issue 2 https://doi.org/10.1103/PhysRevLett.78.310	journal	January 1997
Collective Excitations in the Dilute 2D Electron System Eriksson, M. A.; Pinczuk, A.; Dennis, B. S. Physical Review Letters, Vol. 82, Issue 10 https://doi.org/10.1103/PhysRevLett.82.2163	journal	March 1999
Electronic Dephasing in the Quantum Hall Regime Fromer, N. A.; Schüller, C.; Chemla, D. S. Physical Review Letters, Vol. 83, Issue 22 https://doi.org/10.1103/PhysRevLett.83.4646	journal	November 1999
Inelastic Light Scattering by Gap Excitations of Fractional Quantum Hall States at 1 / 3 ≤ ν ≤ 2 / 3 Kang, Moonsoo; Pinczuk, A.; Dennis, B. S. Physical Review Letters, Vol. 84, Issue 3 https://doi.org/10.1103/PhysRevLett.84.546	journal	January 2000
Observation of Multiple Magnetorotons in the Fractional Quantum Hall Effect Kang, Moonsoo; Pinczuk, A.; Dennis, B. S. Physical Review Letters, Vol. 86, Issue 12 https://doi.org/10.1103/PhysRevLett.86.2637	journal	March 2001
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Evidence of Landau Levels and Interactions in Low-Lying Excitations of Composite Fermions at 1 / 3 ≤ ν ≤ 2 / 5 Dujovne, Irene; Pinczuk, A.; Kang, Moonsoo Physical Review Letters, Vol. 90, Issue 3 https://doi.org/10.1103/PhysRevLett.90.036803	journal	January 2003
Observation of Soft Magnetorotons in Bilayer Quantum Hall Ferromagnets Luin, Stefano; Pellegrini, Vittorio; Pinczuk, Aron Physical Review Letters, Vol. 90, Issue 23 https://doi.org/10.1103/PhysRevLett.90.236802	journal	June 2003
Crossover and Coexistence of Quasiparticle Excitations in the Fractional Quantum Hall Regime at ν ≤ 1 / 3 Hirjibehedin, C. F.; Pinczuk, A.; Dennis, B. S. Physical Review Letters, Vol. 91, Issue 18 https://doi.org/10.1103/PhysRevLett.91.186802	journal	October 2003
Observation of Collapse of Pseudospin Order in Bilayer Quantum Hall Ferromagnets Luin, Stefano; Pellegrini, Vittorio; Pinczuk, Aron Physical Review Letters, Vol. 94, Issue 14 https://doi.org/10.1103/PhysRevLett.94.146804	journal	April 2005
Composite-Fermion Spin Excitations as ν Approaches 1 / 2 : Interactions in the Fermi Sea Dujovne, Irene; Pinczuk, A.; Kang, Moonsoo Physical Review Letters, Vol. 95, Issue 5 https://doi.org/10.1103/PhysRevLett.95.056808	journal	July 2005
Many-Body Interactions in Semiconductors Probed by Optical Two-Dimensional Fourier Transform Spectroscopy Li, Xiaoqin; Zhang, Tianhao; Borca, Camelia N. Physical Review Letters, Vol. 96, Issue 5 https://doi.org/10.1103/PhysRevLett.96.057406	journal	February 2006
Transition from Free to Interacting Composite Fermions away from ν = 1 / 3 Gallais, Y.; Kirschenmann, T. H.; Dujovne, I. Physical Review Letters, Vol. 97, Issue 3 https://doi.org/10.1103/PhysRevLett.97.036804	journal	July 2006
Ultrafast Dynamics of Coherences in a Quantum Hall System Dani, K. M.; Tignon, J.; Breit, M. Physical Review Letters, Vol. 97, Issue 5 https://doi.org/10.1103/PhysRevLett.97.057401	journal	August 2006
Colloquium: Topological insulators Hasan, M. Z.; Kane, C. L. Reviews of Modern Physics, Vol. 82, Issue 4, p. 3045-3067 https://doi.org/10.1103/RevModPhys.82.3045	journal	November 2010
Coherent spectroscopy of semiconductors Cundiff, Steven T. Optics Express, Vol. 16, Issue 7 https://doi.org/10.1364/OE.16.004639	journal	January 2008

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77 NANOSCIENCE AND NANOTECHNOLOGY
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Exploring two-dimensional electron gases with two-dimensional Fourier transform spectroscopy

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