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Title: Extending dry storage of spent LWR fuel for 100 years.

Conference ·
OSTI ID:10813

Because of delays in closing the back end of the fuel cycle in the U.S., there is a need to extend dry inert storage of spent fuel beyond its originally anticipated 20-year duration. Many of the methodologies developed to support initial licensing for 20-year storage should be able to support the longer storage periods envisioned. This paper evaluates the applicability of existing information and methodologies to support dry storage up to 100 years. The thrust of the analysis is the potential behavior of the spent fuel. In the USA, the criteria for dry storage of LWR spent fuel are delineated in 10 CFR 72 [1]. The criteria fall into four general categories: maintain subcriticality, prevent the release of radioactive material above acceptable limits, ensure that radiation rates and doses do not exceed acceptable levels, and maintain retrievability of the stored radioactive material. These criteria need to be considered for normal, off-normal, and postulated accident conditions. The initial safety analysis report submitted for licensing evaluated the fuel's ability to meet the requirements for 20 years. It is not the intent to repeat these calculations, but to look at expected behavior over the additional 80 years, during which the temperatures and radiation fields are lower. During the first 20 years, the properties of the components may change because of elevated temperatures, presence of moisture, effects of radiation, etc. During normal storage in an inert atmosphere, there is potential for the cladding mechanical properties to change due to annealing or interaction with cask materials. The emissivity of the cladding could also change due to storage conditions. If there is air leakage into the cask, additional degradation could occur through oxidation in breached rods, which could lead to additional fission gas release and enlargement of cladding breaches. Air in-leakage could also affect cover gas conductivity, cladding oxidation, emissivity changes, and excessive creep and mechanical property changes. Postulated accident scenarios would be the same for 20-year or 100-year storage, because they are mostly governed by operational or outside events, and not by the cask or fuel. Analyses of accident scenarios during extended dry storage could be impacted by fuel and cask changes that would result from the extended period of storage. Overall, the results of this work indicate that, based on fuel behavior, spent fuel at burnups below {approximately}45 GWd/MTU can be dry stored for 100 years. Long-term storage of higher burnup fuel or fuels with newer cladding will require the determination of temperature limits based on evaluation of stress-driven degradation mechanisms of the cladding.

Research Organization:
Argonne National Lab., IL (US)
Sponsoring Organization:
US Department of Energy (US)
DOE Contract Number:
W-31109-ENG-38
OSTI ID:
10813
Report Number(s):
ANL/CMT/CP-96494; TRN: US0103861
Resource Relation:
Conference: International Symposium on Storage of Spent Fuel from Power Reactors, Vienna (AT), 11/09/1998--11/13/1998; Other Information: PBD: 16 Dec 1998
Country of Publication:
United States
Language:
English