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Photothermal deflection spectroscopy and detection

Journal Article · · Applied Optics
DOI:https://doi.org/10.1364/AO.20.001333· OSTI ID:1077131
 [1];  [1];  [2];  [2]
  1. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Applied Physics & Laser Spectroscopy Group; Univ. of California, Berkeley, CA (United States)
  2. Ecole Superieure de Physique et de Chimie Industrielles (ESPCI), ParisTech (France). Lab. d'Optique Physique
The theory for a sensitive spectroscopy based on the photothermal deflection of a laser beam is developed. We consider cw and pulsed cases of both transverse and collinear photothermal deflection spectroscopy for solids, liquids, gases, and thin films. The predictions of the theory are experimentally verified, its implications for imaging and microscopy are given, and the sources of noise are analyzed. The sensitivity and versatility of photothermal deflection spectroscopy are compared with thermal lensing and photoacoustic spectroscopy.
Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC02-05CH11231; W-7405-ENG-48
OSTI ID:
1077131
Report Number(s):
LBL--11541
Journal Information:
Applied Optics, Journal Name: Applied Optics Journal Issue: 8 Vol. 20; ISSN 0003-6935; ISSN APOPAI
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English

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