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Title: Improved zircon fission-track annealing model based on reevaluation of annealing data

Journal Article · · Physics and Chemistry of Minerals, 40(2):93-106
 [1];  [1];  [2];  [3];  [1]
  1. Univ. of Campinas (Brazil)
  2. Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
  3. Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

The thermal recovery (annealing) of mineral structure modified by the passage of fission fragments has long been studied by the etching technique. In minerals like apatite and zircon, the annealing kinetics are fairly well constrained from the hour to the million-year timescale and have been described by empirical and semi-empirical equations. On the other hand, laboratory experiments, in which ion beams interact with minerals and synthetic ceramics, have shown that there is a threshold temperature beyond which thermal recovery impedes ion-induced amorphization. In this work, it is assumed that this behavior can be extended to the annealing of fission tracks in minerals. It is proposed that there is a threshold temperature, T 0, beyond which fission tracks are erased within a time t 0, which is independent of the current state of lattice deformation. This implies that iso-annealing curves should converge to a fanning point in the Arrhenius pseudo-space (ln t vs. 1/T). Based on the proposed hypothesis, and laboratory and geological data, annealing equations are reevaluated. The geological timescale estimations of a model arising from this study are discussed through the calculation of partial annealing zone and closure temperature, and comparison with geological sample constraints found in literature. It is shown that the predictions given by this model are closer to field data on closure temperature and partial annealing zone than predictions given by previous models.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States). Environmental Molecular Sciences Lab. (EMSL)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1063077
Report Number(s):
PNNL-SA-92276; 47464; KC0201020
Journal Information:
Physics and Chemistry of Minerals, 40(2):93-106, Vol. 40, Issue 2; ISSN ‎0342-1791
Country of Publication:
United States
Language:
English