skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Moment analysis for spatiotemporal fractional dispersion

Journal Article · · Water Resources Research
DOI:https://doi.org/10.1029/2007wr006291· OSTI ID:1051557
 [1];  [2];  [3]
  1. Hydrologic Science Division Desert Research Institute Las Vegas Nevada USA
  2. Department of Geology and Geological Engineering Colorado School of Mines Golden Colorado USA
  3. Department of Mathematics and Statistics University of Otago Dunedin New Zealand

The evolution of the first five nonnegative integer‐order spatial moments (corresponding to the mass, mean, variance, skewness, and kurtosis) are investigated systematically for spatiotemporal nonlocal, fractional dispersion. Three commonly used fractional‐order transport equations, including the time fractional advection‐dispersion equation (Time‐FADE), the fractal mobile‐immobile (MIM) equation, and the fully fractional advection‐dispersion equation (FFADE), are considered. Analytical solutions verify our numerical results and reveal the anomalous evolution of the moments. Following Adams and Gelhar's (1992) work on the classical ADE, we find that a simultaneous analysis of all moments is critical in discriminating between different nonlocal models. The evolution of dispersion among the subdiffusive to superdiffusive rates is then further explored numerically by a non‐Markovian random walk particle‐tracking method that can be used for any heterogeneous boundary or initial value problem in three dimensions. Both the analytical and the numerical results also show the similarity (at the early time) and the difference (at the late time) of moment growth for solutes in different phases (mobile versus total) described by the MIM models. Further simulations of the 1‐D bromide snapshots measured at the MADE experiments, using all three models with parameters fitted by the observed zeroth to fourth moments, indicate that (1) both the time and space nonlocality strongly affect the solute transport at the MADE site, (2) all five spatial moments should be considered in transport model selection and calibration because those up to the variance cannot effectively discriminate between nonlocal models, and (3) the log concentration should be used when evaluating the plume leading edge and the effects of space nonlocality.

Research Organization:
Colorado School of Mines, Golden, CO (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
DOE Contract Number:
FG02-07ER15841
OSTI ID:
1051557
Report Number(s):
DOE/ER/15841-19
Journal Information:
Water Resources Research, Vol. 44, Issue 4; ISSN 0043-1397
Publisher:
American Geophysical Union (AGU)
Country of Publication:
United States
Language:
English

References (43)

Field study of dispersion in a heterogeneous aquifer: 2. Spatial moments analysis journal December 1992
Fractional diffusion with two time scales journal January 2007
Subordinated advection‐dispersion equation for contaminant transport journal June 2001
Advection and dispersion in time and space journal May 2005
Investigating the Macrodispersion Experiment (MADE) site in Columbus, Mississippi, using a three-dimensional inverse flow and transport model: MADE SITE USING 3-D INVERSE MODEL journal April 2004
Application of a fractional advection-dispersion equation journal February 2000
The fractional-order governing equation of Lévy Motion journal February 2000
Theory of anomalous chemical transport in random fracture networks journal May 1998
Physical pictures of transport in heterogeneous media: Advection-dispersion, random-walk, and fractional derivative formulations: TRANSPORT IN HETEROGENEOUS MEDIA journal October 2002
Modeling non-Fickian transport in geological formations as a continuous time random walk journal January 2006
Field study of dispersion in a heterogeneous aquifer: 1. Overview and site description journal December 1992
Delineating Alluvial Aquifer Heterogeneity Using Resistivity and GPR Data journal August 2005
Anomalous diffusion and fractional advection-diffusion equation journal January 2005
Fractional advection-dispersion equation: A classical mass balance with convolution-Fickian Flux journal December 2000
Numerical Solution of Fractional Advection-Dispersion Equation journal May 2004
A fractional dispersion model for overland solute transport journal March 2006
A dual-domain mass transfer approach for modeling solute transport in heterogeneous aquifers: Application to the Macrodispersion Experiment (MADE) site journal September 2000
On the late-time behavior of tracer test breakthrough curves journal December 2000
Power-law residence time distribution in the hyporheic zone of a 2nd-order mountain stream journal January 2002
Rate-limited mass transfer or macrodispersion: Which dominates plume evolution at the macrodispersion experiment (MADE) site? journal March 2000
Hydraulic conductivity, velocity, and the order of the fractional dispersion derivative in a highly heterogeneous system journal November 2002
Reply to comment by F. Molz et al. on “Investigating the Macrodispersion Experiment (MADE) site in Columbus, Mississippi, using a three‐dimensional inverse flow and transport model” journal June 2006
Evidence of one-dimensional scale-dependent fractional advection–dispersion journal May 2006
Numerical Simulation of a Natural Gradient Tracer Experiment for the Natural Attenuation Study: Flow and Physical Transport journal July 2001
Generalized Fick’s Law and Fractional ADE for Pollution Transport in a River: Detailed Derivation journal January 2006
Heavy‐tailed log hydraulic conductivity distributions imply heavy‐tailed log velocity distributions journal April 2006
Limits of applicability of the advection-dispersion model in aquifers containing connected high-conductivity channels: LIMITS OF ADVECTION-DISPERSION MODEL journal August 2004
Fractional Fokker-Planck dynamics: Stochastic representation and computer simulation journal January 2007
Is transport in porous media always diffusive? A counterexample journal October 1980
A simple robust estimation method for the thickness of heavy tails journal August 1998
The random walk's guide to anomalous diffusion: a fractional dynamics approach journal December 2000
A physical interpretation for the fractional derivative in Levy diffusion journal October 2002
Comment on “Investigating the Macrodispersion Experiment (MADE) site in Columbus, Mississippi, using a three‐dimensional inverse flow and transport model” by Heidi Christiansen Barlebo, Mary C. Hill, and Dan Rosbjerg journal June 2006
Eulerian derivation of the fractional advection–dispersion equation journal March 2001
Fractal mobile/immobile solute transport: FRACTAL MOBILE-IMMOBILE SOLUTE TRANSPORT journal October 2003
A mass balance based numerical method for the fractional advection‐dispersion equation: Theory and application journal July 2005
On Using Random Walks to Solve the Space-Fractional Advection-Dispersion Equations journal April 2006
Relationship between flux and resident concentrations for anomalous dispersion: RESIDENT AND FLUX CONCENTRATIONS FOR ANOMALOUS DIFFUSION journal September 2006
Space-fractional advection-dispersion equations with variable parameters: Diverse formulas, numerical solutions, and application to the Macrodispersion Experiment site data: SPATIAL FADE WITH VARIABLE PARAMETERS journal May 2007
Predicting the Tails of Breakthrough Curves in Regional-Scale Alluvial Systems journal July 2007
Analysis of Solute Transport in Flow Fields Influenced by Preferential Flowpaths at the Decimeter Scale journal March 2003
Numerical Simulation of Tracer Tests in Heterogeneous Aquifer journal June 1998
Application of the Fractional Advection-Dispersion Equation in Porous Media journal July 2003

Similar Records

Preface: Nonclassical Transport
Journal Article · Mon Sep 01 00:00:00 EDT 2008 · Vadose Zone Journal · OSTI ID:1051557

Final Report
Technical Report · Mon Sep 24 00:00:00 EDT 2012 · OSTI ID:1051557

Time and space nonlocalities underlying fractional-derivative models: Distinction and literature review of field applications
Journal Article · Wed Apr 01 00:00:00 EDT 2009 · Advances in Water Resources · OSTI ID:1051557