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Title: Laser-Directed Hierarchical Assembly of Liquid Crystal Defects and Control of Optical Phase Singularities

Journal Article · · Scientific Reports
DOI:https://doi.org/10.1038/srep00414· OSTI ID:1050143

Topological defect lines are ubiquitous and important in a wide variety of fascinating phenomena and theories in many fields ranging from materials science to early-universe cosmology, and to engineering of laser beams. However, they are typically hard to control in a reliable manner. Here we describe facile erasable 'optical drawing' of self-assembled defect clusters in liquid crystals. These quadrupolar defect clusters, stabilized by the medium's chirality and the tendency to form twisted configurations, are shaped into arbitrary two-dimensional patterns, including reconfigurable phase gratings capable of generating and controlling optical phase singularities in laser beams. Our findings bridge the studies of defects in condensed matter physics and optics and may enable applications in data storage, singular optics, displays, electro-optic devices, diffraction gratings, as well as in both optically- and electrically-addressed pixel-free spatial light modulators.

Research Organization:
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
DOE Contract Number:
AC36-08GO28308
OSTI ID:
1050143
Report Number(s):
NREL/JA-5900-55917; TRN: US201218%%499
Journal Information:
Scientific Reports, Vol. 2, Issue 414
Country of Publication:
United States
Language:
English

References (37)

Orbital angular momentum of light and the transformation of Laguerre-Gaussian laser modes journal June 1992
Vortex knots in light journal January 2005
Knotted threads of darkness journal November 2004
Generation of electron beams carrying orbital angular momentum journal April 2010
Skyrmion Lattice in a Chiral Magnet journal February 2009
Pleats in crystals on curved surfaces journal December 2010
Production and application of electron vortex beams journal September 2010
Isolated optical vortex knots journal January 2010
Frustrated nematic order in spherical geometries journal February 2011
Power of the Poincaré Group: Elucidating the Hidden Symmetries in Focal Conic Domains journal June 2010
Linked and knotted beams of light journal August 2008
Cosmology in the Laboratory: Defect Dynamics in Liquid Crystals journal March 1991
Novel Colloidal Interactions in Anisotropic Fluids journal March 1997
A continuous-viewing-angle-controllable liquid-crystal display using a blue-phase liquid crystal journal January 2011
The Physics of Liquid Crystals journal May 1995
Liquid crystal ‘blue phases’ with a wide temperature range journal August 2005
Printed artificial cilia from liquid-crystal network actuators modularly driven by light journal June 2009
Liquid-crystal materials find a new order in biomedical applications journal November 2007
Three-dimensional structure and multistable optical switching of triple-twisted particle-like excitations in anisotropic fluids journal December 2009
Electric-field-induced nematic-cholesteric transition and three-dimensional director structures in homeotropic cells journal December 2005
Static and dynamic properties of cholesteric fingers in electric field journal October 2000
Multimodal nonlinear optical polarizing microscopy of long-range molecular order in liquid crystals journal January 2010
Mapping phases of singular scalar light fields journal December 2007
Optics of light beams with screw dislocations journal December 1993
Dislocations in Wave Trains journal January 1974
Optically generated adaptive localized structures in confined chiral liquid crystals doped with fullerene journal November 2010
Optically generated reconfigurable photonic structures of elastic quasiparticles in frustrated cholesteric liquid crystals journal January 2012
Shape-Dependent Oriented Trapping and Scaffolding of Plasmonic Nanoparticles by Topological Defects for Self-Assembly of Colloidal Dimers in Liquid Crystals journal January 2012
Particle-Stabilized Defect Gel in Cholesteric Liquid Crystals journal January 1999
Rheology of defect networks in cholesteric liquid crystals journal September 2002
Three-dimensional colloidal crystals in liquid crystalline blue phases journal February 2011
Reconfigurable interactions and three-dimensional patterning of colloidal particles and defects in lamellar soft media journal March 2012
Shape-Controlled Colloidal Interactions in Nematic Liquid Crystals journal November 2009
Hierarchical self-assembly of nematic colloidal superstructures journal June 2008
Geometrical frustration and defects in condensed matter systems journal March 2008
Relaxation kinetics of stretched disclination lines in a nematic liquid crystal journal June 2010
A Self-Quenched Defect Glass in a Colloid-Nematic Liquid Crystal Composite journal October 2011