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Title: Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics

Abstract

Nuclear forensic teams will be deployed to collect and evaluate fallout samples on the ground in the scenario of a low-yield nuclear detonation in a heavily populated area. Quick non-destructive methods of predicting the quality of the sample before it is analyzed in detail are essential for efficient post-event collections. In this work, the process of exporting Defense Land Fallout Interpretive Code (DELFIC) results into Gamma Detector Response and Analysis Software (GADRAS) has been automated within the Fallout Analysis Tool. This coupling allows for the simulation of detector responses to fallout samples with varying degrees of fractionation. The degree to which the samples are fractionated depends on the location of the samples in the fallout field. In the following study, this phenomenon is examined, as its understanding is important to the investigation of debris distribution. The simulated detector spectra from GADRAS can be used to compare peak ratios of volatile-refractory isotope pairs in order to determine the degree of fractionation. Simulated fractionated fallout samples from DELFIC for a 10 kt, pure 235U fission surface burst were modeled for distances ranging to 256 km out from ground zero, and for times up to 1 week from detonation. The fractionation ratios, alsomore » known as r values, from isotope concentrations, photon lines and peak areas of four volatile-refractory pairs were calculated and compared. Fractionation prediction via the peak areas method was evaluated for each pair by comparing the results with the simulated radionuclide inventory.« less

Authors:
 [1];  [1];  [1];  [1];  [1]
  1. ORNL
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1047031
DOE Contract Number:
DE-AC05-00OR22725
Resource Type:
Conference
Resource Relation:
Conference: INMM 53rd Annual Meeting, Orlando, FL, USA, 20120715, 20120719
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; DISTRIBUTION; EXPLOSIONS; FALLOUT; FISSION; FORECASTING; FRACTIONATION; PHOTONS; RADIOISOTOPES; SIMULATION; SPECTRA

Citation Formats

Monterial, Mateusz, Jodoin, Vincent J, Lefebvre, Jordan P, Peplow, Douglas E., and Hooper, David A. Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics. United States: N. p., 2012. Web.
Monterial, Mateusz, Jodoin, Vincent J, Lefebvre, Jordan P, Peplow, Douglas E., & Hooper, David A. Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics. United States.
Monterial, Mateusz, Jodoin, Vincent J, Lefebvre, Jordan P, Peplow, Douglas E., and Hooper, David A. Sun . "Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics". United States. doi:.
@article{osti_1047031,
title = {Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics},
author = {Monterial, Mateusz and Jodoin, Vincent J and Lefebvre, Jordan P and Peplow, Douglas E. and Hooper, David A},
abstractNote = {Nuclear forensic teams will be deployed to collect and evaluate fallout samples on the ground in the scenario of a low-yield nuclear detonation in a heavily populated area. Quick non-destructive methods of predicting the quality of the sample before it is analyzed in detail are essential for efficient post-event collections. In this work, the process of exporting Defense Land Fallout Interpretive Code (DELFIC) results into Gamma Detector Response and Analysis Software (GADRAS) has been automated within the Fallout Analysis Tool. This coupling allows for the simulation of detector responses to fallout samples with varying degrees of fractionation. The degree to which the samples are fractionated depends on the location of the samples in the fallout field. In the following study, this phenomenon is examined, as its understanding is important to the investigation of debris distribution. The simulated detector spectra from GADRAS can be used to compare peak ratios of volatile-refractory isotope pairs in order to determine the degree of fractionation. Simulated fractionated fallout samples from DELFIC for a 10 kt, pure 235U fission surface burst were modeled for distances ranging to 256 km out from ground zero, and for times up to 1 week from detonation. The fractionation ratios, also known as r values, from isotope concentrations, photon lines and peak areas of four volatile-refractory pairs were calculated and compared. Fractionation prediction via the peak areas method was evaluated for each pair by comparing the results with the simulated radionuclide inventory.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Sun Jan 01 00:00:00 EST 2012},
month = {Sun Jan 01 00:00:00 EST 2012}
}

Conference:
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