Binary Heterogeneous Superlattices Assembled from Quantum Dots and Gold Nanoparticles with DNA
Journal Article
·
· Journal of the American Chemical Society
Controllable assembly of three-dimensional (3D) superlattices composed of different types of nanoscale objects opens new opportunities for material fabrication. Herein we show the successful assembly of heterogeneous 3D structures from gold nanoparticles (AuNPs) and quantum dots (QDs) using DNA encoding. By applying synchrotron-based small-angle X-ray scattering, we found that AuNPs and QDs are positioned in a body-centered cubic lattice, while each particle type, AuNP and QD, is arranged in a simple-cubic manner. Our studies demonstrate a route for assembly of integrated heterogeneous 3D structures from different nano-objects by DNA-encoded interactions.
- Research Organization:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Organization:
- USDOE SC OFFICE OF SCIENCE (SC)
- DOE Contract Number:
- DE-AC02-98CH10886
- OSTI ID:
- 1041917
- Report Number(s):
- BNL-97595-2012-JA; JACSAT; TRN: US201212%%328
- Journal Information:
- Journal of the American Chemical Society, Vol. 133, Issue 14; ISSN 0002-7863
- Country of Publication:
- United States
- Language:
- English
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