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Quantum Dot–Bridge–Fullerene Heterodimers with Controlled Photoinduced Electron Transfer

Journal Article · · Angewandte Chemie - International Edition
OSTI ID:1024332

A series of donor-bridge-acceptor systems in the form of core/shell CdSe/ZnS quantum dot-bridge-fullerene heterodimers (see picture) with varying bridge length and varying quantum dot size were self-assembled by a surface-based stepwise method to demonstrate control of the rate and of the magnitude of fluctuations of photoinduced electron transfer at the single-molecule level.

Research Organization:
Brookhaven National Laboratory (BNL) Center for Functional Nanomaterials
Sponsoring Organization:
DOE - OFFICE OF SCIENCE
DOE Contract Number:
AC02-98CH10886
OSTI ID:
1024332
Report Number(s):
BNL--94026-2011-JA
Journal Information:
Angewandte Chemie - International Edition, Journal Name: Angewandte Chemie - International Edition Journal Issue: 27 Vol. 50; ISSN 1433-7851
Country of Publication:
United States
Language:
English