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AUTOMATIC PARTICULATE SULFUR MEASUREMENTS WITH A DICHOTOMOUS SAMPLER AND ON-LINE X-RAY FLUORESCENCE ANALYSIS

Journal Article · · Environmental Science and Technology
OSTI ID:1022085
An instrument is described which employs a dichotomous sampler to acquire fine particulate samples on a continuous tape filter, Analyses for elemental sulfur are performed immediately following acquisition using a sensitive X-ray fluorescence spectrometer. Sample sequencing, data acquisition, and calculation of concentrations are performed continuously using an on-line calculator, Precision and accuracy of the method are discussed and results obtained from ambient measurements are presented. The increased emission of sulfur-containing compounds into the atmosphere has become a major consideration in the design of air pollution monitoring and control strategies. This has stimulated considerable interest in the development of monitoring equipment capable of analyzing the atmospheric aerosol for sulfur-containing compounds. We describe a rapid, sensitive and accurate X-ray fluorescence method for the analysis of elemental sulfur collected from ambient aerosol samples. The instrument includes a dichotomous sampler, air filter transport system and high-sensitivity wavelength dispersive X-ray fluorescence analyzer. An associated calculator/controller enables one to obtain real-time measurements of ambient particulate sulfur concentrations over short time intervals.
Research Organization:
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (US)
Sponsoring Organization:
Engineering Division
DOE Contract Number:
AC02-05CH11231
OSTI ID:
1022085
Report Number(s):
LBL-10882
Journal Information:
Environmental Science and Technology, Journal Name: Environmental Science and Technology Journal Issue: 6 Vol. 15; ISSN ESTHAG; ISSN 0013-936X
Country of Publication:
United States
Language:
English

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