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Electrically Controllable Spontaneous Magnetism in Nanoscale Mixed Phase Multiferroics

Journal Article · · Nature Communications
OSTI ID:1015563

The emergence of enhanced spontaneous magnetic moments in self-assembled, epitaxial nanostructures of tetragonal (T-phase) and rhombohedral phases (R-phase) of the multiferroic BiFeO{sub 3} system is demonstrated. X-ray magnetic circular dichroism based photoemission electron microscopy (PEEM) was applied to investigate the local nature of this magnetism. We find that the spontaneous magnetization of the R-phase is significantly enhanced above the canted antiferromagnetic moment in the bulk phase, as a consequence of a piezomagnetic coupling to the adjacent T-phase and the epitaxial constraint. Reversible electric field control and manipulation of this magnetic moment at room temperature is shown using a combination of piezoresponse force microscopy and PEEM studies.

Research Organization:
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (US)
Sponsoring Organization:
Advanced Light Source Division; Materials Sciences Division
DOE Contract Number:
AC02-05CH11231
OSTI ID:
1015563
Report Number(s):
LBNL-4511E
Journal Information:
Nature Communications, Journal Name: Nature Communications
Country of Publication:
United States
Language:
English

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