The photodissociation and reaction dynamics of vibrationally excited molecules. Technical progress report, 1992--1993
We have used combined vibrational overtone excitation and laser induced fluorescence detection to study dissociation dynamics of hydroxylamine (NH{sub 2}OH), have performed our first laser induced grating experiments on water, and have begun assembling a new apparatus for preparing vibrationally excited molecules with simulated Raman excitation. We study role of vibrational excitation in photodissociation dynamics by using a vibrational state preparation technique, such as vibrational overtone excitation or stimulated Raman excitation, to create molecules with particular nuclear motions and then to excite that molecule to a dissociative electronic state.
- Research Organization:
- Wisconsin Univ., Madison, WI (United States)
- Sponsoring Organization:
- USDOE, Washington, DC (United States)
- DOE Contract Number:
- FG02-86ER13500
- OSTI ID:
- 10136002
- Report Number(s):
- DOE/ER/13500--T3; ON: DE93010896
- Country of Publication:
- United States
- Language:
- English
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