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Measurements of radionuclide in Par Pond sediments with an underwater HPGe detector

Technical Report ·
DOI:https://doi.org/10.2172/10104999· OSTI ID:10104999
Savannah River Site (SRS) effluent gamma emitting radionuclides in Par Pond sediment were examined in situ with an underwater HPGe detector prior to and following a 19 ft drawdown of the pond in 1991 to address dam repairs. These measurements provide a map of the {sup 137}Cs concentrations of the pond sediment, indicating that 9.4 {plus_minus} 1.5 Ci is exposed by the drawdown and that 46.6 {plus_minus} 7.2 Ci is the entire pond inventory. The highest individual {sup 137}Cs concentration was 25 {mu}Ci/m{sup 2} for the exposed sediment and 50 {mu}Ci/m{sup 2} for the entire pond. The results are consistent with parallel studies conducted by SREL, as well as historical data. Aside from {sup 137}Cs, the only other SRS-produced isotope observed was {sup 60}Co, with activity of only about 1% of that for {sup 137}Cs. This observation was also confirmed in grab samples of pond sediment and vegetation, which were returned to the laboratory for ultra-low-level gamma spectrometry analysis. A special effort was required to calibrate the underwater HPGe detector, where both measurements and calculational models were used. The effects of sediment depth profiles for density and {sup 137}Cs concentration were addressed in the calibration. Calibration factors for sediment surface concentrations ({mu}Ci/m{sup 2}/cpm) and sediment mass concentrations (pCi/kg/cpm) were obtained. In general, the {mu}Ci/m{sup 2}/cpm factor is recommended, as the pCi/kg/cpm factor depends on the depth location of the sediment of interest. However, a pCi/kg/cpm factor, which is dependent on the depth within the sediment is presented to address dose calculations that require it.
Research Organization:
Westinghouse Savannah River Co., Aiken, SC (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
AC09-89SR18035
OSTI ID:
10104999
Report Number(s):
WSRC-TR--93-0209; ON: DE94003125
Country of Publication:
United States
Language:
English

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