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Mathematical Analysis of a Novel Approach to Maximize Waste Recovery in a Life Support System

Technical Report ·
DOI:https://doi.org/10.2172/1009154· OSTI ID:1009154

NASA has been evaluating closed-loop atmosphere revitalization architectures carbon dioxide, CO2, reduction technologies. The CO2 and steam, H2O, co-electrolysis process is another option that NASA has investigated. Utilizing recent advances in the fuel cell technology sector, the Idaho National Laboratory, INL, has developed a CO2 and H2O co-electrolysis process to produce oxygen and syngas (carbon monoxide, CO and hydrogen, H2 mixture) for terrestrial (energy production) application. The technology is a combined process that involves steam electrolysis, CO2 electrolysis, and the reverse water gas shift (RWGS) reaction. Two process models were developed to evaluate novel approaches for waster recovery in a life support system. The first is a model INL co-electrolysis process combined with a methanol production process. The second is the INL co-electrolysis process combined with a pressure swing adsorption (PSA) process. For both processes, the overall power increases as the syngas ratio, H2/CO, increases because more water is needed to produce more hydrogen at a set CO2 incoming flow rate. The power for the methanol cases is less than the PSA because heat is available from the methanol reactor to preheat the water and carbon dioxide entering the co-electrolysis process.

Research Organization:
Idaho National Lab. (INL), Idaho Falls, ID (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
DE-AC07-05ID14517
OSTI ID:
1009154
Report Number(s):
INL/EXT-11-21041; TRN: US201107%%693
Country of Publication:
United States
Language:
English