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Real-Time Characterization of Formation and Breakup of Iridium Clusters in Highly Dealuminated Zeolite Y

Journal Article · · Angew. Chem. Int. Ed.

The chemistry of formation of iridium clusters from mononuclear iridium diethylene complexes anchored in dealuminated Y zeolite, and their subsequent breakup -- all including changes in the metal-metal, metal-support, and metal-ligand interactions -- is demonstrated by time-resolved EXAFS, XANES, and IR spectroscopy.

Research Organization:
Advanced Photon Source (APS), Argonne National Laboratory (ANL), Argonne, IL (US)
Sponsoring Organization:
USDOE
OSTI ID:
1007013
Journal Information:
Angew. Chem. Int. Ed., Journal Name: Angew. Chem. Int. Ed. Journal Issue: (48) ; 2008 Vol. 47; ISSN 1433-7851
Country of Publication:
United States
Language:
ENGLISH