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A generalized approximation for the thermophoretic force on a free-molecular particle.

Journal Article · · Proposed for publication in Aerosol Science and Technology.
OSTI ID:1002128

A general, approximate expression is described that can be used to predict the thermophoretic force on a free-molecular, motionless, spherical particle suspended in a quiescent gas with a temperature gradient. The thermophoretic force is equal to the product of an order-unity coefficient, the gas-phase translational heat flux, the particle cross-sectional area, and the inverse of the mean molecular speed. Numerical simulations are used to test the accuracy of this expression for monatomic gases, polyatomic gases, and mixtures thereof. Both continuum and noncontinuum conditions are examined; in particular, the effects of low pressure, wall proximity, and high heat flux are investigated. The direct simulation Monte Carlo (DSMC) method is used to calculate the local molecular velocity distribution, and the force-Green's-function method is used to calculate the thermophoretic force. The approximate expression is found to predict the calculated thermophoretic force to within 10% for all cases examined.

Research Organization:
Sandia National Laboratories
Sponsoring Organization:
USDOE
DOE Contract Number:
AC04-94AL85000
OSTI ID:
1002128
Report Number(s):
SAND2003-2776J
Journal Information:
Proposed for publication in Aerosol Science and Technology., Journal Name: Proposed for publication in Aerosol Science and Technology. Journal Issue: 7 Vol. 38; ISSN 1521-7388; ISSN 0278-6826; ISSN ASTYDQ
Country of Publication:
United States
Language:
English