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Title: FURTHER DEVELOPMENT OF MODIFIED MONOSODIUM TITANATE, AN IMPROVED SORBENT FOR PRETREATMENT OF HIGH LEVEL NUCLEAR WASTE AT THE SAVANNAH RIVER SITE

Conference ·
OSTI ID:1001777

High-level nuclear waste produced from fuel reprocessing operations at the Savannah River Site (SRS) requires pretreatment to remove Cs-137, Sr-90, and alpha-emitting radionuclides (i.e., actinides) prior to disposal onsite as low level waste. Separation processes planned at SRS include caustic side solvent extraction, for Cs-137 removal, and sorption of Sr-90 and alpha-emitting radionuclides onto monosodium titanate (MST). The predominant alpha-emitting radionuclides in the highly alkaline waste solutions include plutonium isotopes Pu-238, Pu-239, and Pu-240. This paper describes recent results from the development of an improved titanate material that exhibits increased removal kinetics and effective capacity for Sr-90 and alpha-emitting radionuclides compared to the baseline MST material.

Research Organization:
Savannah River Site (SRS), Aiken, SC (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
DE-AC09-08SR22470
OSTI ID:
1001777
Report Number(s):
SRNL-STI-2010-00491; TRN: US1100465
Resource Relation:
Conference: Waste Management
Country of Publication:
United States
Language:
English