Updates and Validation for the n+63,65Cu Cross Sections [Abstract]
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
The neutron induced total, elastic, and capture cross sections of 63,65Cu isotopes were selected for evaluation in the resolved and unresolved resonance energy ranges by the National Criticality Safety Program to resolve discrepancies related to benchmark performance. This is especially evident for the series of ZEUS benchmarks in which copper is used as a reflector. Because copper is also used as structural material in both fission and fusion reactors, the need to address benchmark discrepancies linked to nuclear data deficiencies is a task of primary importance. The aim of this work is to describe the steps of evaluation work towards a consistent improvement of the benchmark performance. The R-matrix analysis with the SAMMY code focused on the 63Cu(n,γ) reaction channel between 100-300 keV coupled to unresolved resonance region parameters up to 650 keV to fit average cross section data from a recent experiment. Due to the high sensitivity of many benchmarks to elastic scattering angular distribution data, especially for the 65Cu isotope, the impact of these data was tested by generating Legendre coefficients from both resonance parameters and the Hauser-Feshbach model. Guided by the findings of Shaw et al., the performance of the current evaluation for 65Cu was compared to that of ENDF/B-VII.1 and ENDF/B-VIII.0 by testing the reactivity coefficients corresponding to the validation suite of experimental criticality benchmarks for thermal, intermediate, and fast systems taken from the International Criticality Safety Benchmark Experiments Project Handbook. The benchmark performance is especially sensitive to 63Cu(n,γ) and 65Cu elastic scattering for neutron energies in the 100–500 keV region, whereas 100 keV is the upper limit of the resolved resonance region in the ENDF/B-VIII.0 evaluations for 63,65Cu. The results highlight the need to handle the transition from the resolved resonance region to the high energy region carefully.
- Research Organization:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Organization:
- USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
- DOE Contract Number:
- AC05-00OR22725
- OSTI ID:
- 1899769
- Resource Relation:
- Conference: 15.International Conference on Nuclear Data for Science and Technology (ND2022), Held Virtually, Sacramento, CA (United States), 21-29 Jul 2022; Related Information: https://indico.frib.msu.edu/event/52/contributions/865/
- Country of Publication:
- United States
- Language:
- English
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