Successive magnetic orderings in the Ising spin chain magnet DyNi5Ge3

Ge, H.; Zhang, L.; Zhao, N.; Yang, J.; Wang, L.; Zhou, L.; Fu, Y.; Li, T. T.; Song, Z. M.; Ding, F.; Xu, J. B.; Zhang, Y. F.; Wang, S. M.; Mei, J. W.; Tong, X.; Miao, P.; He, H.; Zhang, Q.; Wu, L. S.; Sheng, J. M.

doi:10.1103/physrevmaterials.6.085001

Title: Successive magnetic orderings in the Ising spin chain magnet DyNi₅Ge₃

Journal Article · Mon Aug 08 00:00:00 EDT 2022 · Physical Review Materials

DOI:https://doi.org/10.1103/physrevmaterials.6.085001· OSTI ID:1883773

Ge, H. ^[1];

^[2]; Zhao, N. ^[1]; Yang, J. ^[1]; Wang, L. ^[1]; Zhou, L. ^[1]; Fu, Y. ^[1]; Li, T. T. ^[1]; Song, Z. M. ^[1]; Ding, F. ^[1]; Xu, J. B. ^[1];

^[1]; Wang, S. M. ^[1]; Mei, J. W. ^[3];

^[4];

^[4]; He, H. ^[5];

^[6]; Wu, L. S. ^[1]; Sheng, J. M. ^[1]

Southern University of Science and Technology (SUSTech), Shenzhen (China)
Chinese Academy of Sciences (CAS), Ganzhou (China); Southern University of Science and Technology (SUSTech), Shenzhen (China)
Southern University of Science and Technology (SUSTech), Shenzhen (China); Shenzhen Institute for Quantum Science and Engineering (China)
Chinese Academy of Sciences (CAS), Beijing (China); Spallation Neutron Source Science Center, Dongguan (China)
University of Chinese Academy of Sciences, Beijing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

In this report, we investigated a new rare-earth-based one-dimensional Ising spin chain magnet DyNi₅Ge₃ by means of magnetization, specific heat, and powder neutron diffraction measurements. Due to the crystalline electrical field splitting, the magnetic Dy ions share an Ising-like ground doublet state. Owning to the local point symmetry, these Ising moments form into two canted magnetic sublattices, which were further confirmed by the angle-dependent magnetization measurement. In zero fields, two successive antiferromagnetic phase transitions were found at temperatures T_N1=6K and T_N2=5K, respectively. Only part of the moments are statically ordered in this intermediate state between T_N1 and T_N2. Powder neutron diffraction experiments at different temperatures were performed as well. Further, an incommensurate magnetic propagation vector of k_m=(0.5,0.4,0.5) was identified. The refined spin configurations through the irreducible representation analysis confirmed that these Ising spins are canted in the crystal ab plane.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Natural Science Foundation of China (NSFC); Guangdong Basic and Applied Basic Research Foundation; Guangdong Introducing Innovative and Entrepreneurial Teams; Shenzhen Key Laboratory of Advanced Quantum Functional Materials and Devices

Grant/Contract Number:: AC05-00OR22725; 12134020; 11974157; 11875265; 12104255; 2021B1515120015; 2017ZT07C062; ZDSYS20190902092905285

OSTI ID:: 1883773

Journal Information:: Physical Review Materials, Vol. 6, Issue 8; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (35)

Spin-stripe phase in a frustrated zigzag spin-1/2 chain Pregelj, M.; Zorko, A.; Zaharko, O. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms8255	journal	June 2015
Quantum Phase Transitions in an Yb-based Semiconductor YbCuS₂ with an Effective Spin-1/2 Zigzag Chain Ohmagari, Yudai; Onimaru, Takahiro; Yamane, Yu Journal of the Physical Society of Japan, Vol. 89, Issue 9 https://doi.org/10.7566/JPSJ.89.093701	journal	September 2020
One-dimensional physics in the 21st century Giamarchi, Thierry Comptes Rendus Physique, Vol. 17, Issue 3-4 https://doi.org/10.1016/j.crhy.2015.11.009	journal	March 2016
Realization of the kagome spin ice state in a frustrated intermetallic compound Zhao, Kan; Deng, Hao; Chen, Hua Science, Vol. 367, Issue 6483 https://doi.org/10.1126/science.aaw1666	journal	March 2020
Magnetic ground state of the Ising-like antiferromagnet ${DyScO}_{3}$ Wu, L. S.; Nikitin, S. E.; Frontzek, M. Physical Review B, Vol. 96, Issue 14 https://doi.org/10.1103/PhysRevB.96.144407	journal	October 2017
Orbital-exchange and fractional quantum number excitations in an f-electron metal, Yb ₂ Pt ₂ Pb Wu, L. S.; Gannon, W. J.; Zaliznyak, I. A. Science, Vol. 352, Issue 6290 https://doi.org/10.1126/science.aaf0981	journal	June 2016
Topological quantum phase transition in the Ising-like antiferromagnetic spin chain BaCo2V2O8 Faure, Quentin; Takayoshi, Shintaro; Petit, Sylvain Nature Physics, Vol. 14, Issue 7 https://doi.org/10.1038/s41567-018-0126-8	journal	May 2018
Multispinon Continua at Zero and Finite Temperature in a Near-Ideal Heisenberg Chain Lake, B.; Tennant, D. A.; Caux, J. -S. Physical Review Letters, Vol. 111, Issue 13 https://doi.org/10.1103/PhysRevLett.111.137205	journal	September 2013
Hierarchy of Bound States in the One-Dimensional Ferromagnetic Ising Chain ${CoNb}_{2} O_{6}$ Investigated by High-Resolution Time-Domain Terahertz Spectroscopy Morris, C. M.; Valdés Aguilar, R.; Ghosh, A. Physical Review Letters, Vol. 112, Issue 13 https://doi.org/10.1103/PhysRevLett.112.137403	journal	April 2014
Magnetic, electrical and thermodynamic properties of CePd5Ge3 Kaczorowski, D.; Czopnik, A.; Suski, W. Solid State Communications, Vol. 117, Issue 6 https://doi.org/10.1016/S0038-1098(00)00465-8	journal	January 2001
Recent advances in magnetic structure determination by neutron powder diffraction Rodríguez-Carvajal, Juan Physica B: Condensed Matter, Vol. 192, Issue 1-2 https://doi.org/10.1016/0921-4526(93)90108-I	journal	October 1993
Magnetization Process of Atacamite: A Case of Weakly Coupled S=1/2 Sawtooth Chains Heinze, L.; Jeschke, H. O.; Mazin, I. I. Physical Review Letters, Vol. 126, Issue 20 https://doi.org/10.1103/PhysRevLett.126.207201	journal	May 2021
Dispersions of many-body Bethe strings Bera, Anup Kumar; Wu, Jianda; Yang, Wang Nature Physics, Vol. 16, Issue 6 https://doi.org/10.1038/s41567-020-0835-7	journal	April 2020
Metamagnetism in CePd ₅ Ge ₃ Gnida, Daniel; Wiśniewski, Piotr; Gribanov, Alexander V. Journal of Physics: Condensed Matter, Vol. 25, Issue 12 https://doi.org/10.1088/0953-8984/25/12/126001	journal	February 2013
Magnetic transitions in the 1D chain compounds NdPd ₅ Ge ₃ and NdPt ₅ Ge ₃ Gui, Xin; Cava, Robert J. Journal of Physics: Condensed Matter, Vol. 33, Issue 43 https://doi.org/10.1088/1361-648X/ac196a	journal	August 2021
Heat transport by lattice and spin excitations in the spin-chain compounds ${SrCuO}_{2}$ and ${Sr}_{2} {CuO}_{3}$ Sologubenko, A. V.; Giannò, K.; Ott, H. R. Physical Review B, Vol. 64, Issue 5 https://doi.org/10.1103/PhysRevB.64.054412	journal	July 2001
Magnetization Plateaus in Spin Chains: “Haldane Gap” for Half-Integer Spins Oshikawa, Masaki; Yamanaka, Masanori; Affleck, Ian Physical Review Letters, Vol. 78, Issue 10 https://doi.org/10.1103/PhysRevLett.78.1984	journal	March 1997
Antiferromagnetic ordering and dipolar interactions of ${YbAlO}_{3}$ Wu, L. S.; Nikitin, S. E.; Brando, M. Physical Review B, Vol. 99, Issue 19 https://doi.org/10.1103/PhysRevB.99.195117	journal	May 2019
Quantum Criticality of an Ising-like Spin- $1 / 2$ Antiferromagnetic Chain in a Transverse Magnetic Field Wang, Zhe; Lorenz, T.; Gorbunov, D. I. Physical Review Letters, Vol. 120, Issue 20 https://doi.org/10.1103/PhysRevLett.120.207205	journal	May 2018
Experimental observation of Bethe strings Wang, Zhe; Wu, Jianda; Yang, Wang Nature, Vol. 554, Issue 7691 https://doi.org/10.1038/nature25466	journal	February 2018
Magnetic order of CePd5Ge3 and CePt5Ge3 Stockert, O.; Hossain, Z.; Deppe, M. Journal of Magnetism and Magnetic Materials, Vol. 272-276 https://doi.org/10.1016/j.jmmm.2003.12.476	journal	May 2004
Magnetic structures of RNi2Ge2 (R = Dy, Ho and Er) and YbNi2Si2 André, G.; Bonville, P.; Bourée, F. Journal of Alloys and Compounds, Vol. 224, Issue 2 https://doi.org/10.1016/0925-8388(95)01545-0	journal	July 1995
What is the spin of a spin wave? Faddeev, L. D.; Takhtajan, L. A. Physics Letters A, Vol. 85, Issue 6-7 https://doi.org/10.1016/0375-9601(81)90335-2	journal	October 1981
Quantum Criticality in an Ising Chain: Experimental Evidence for Emergent E ₈ Symmetry Coldea, R.; Tennant, D. A.; Wheeler, E. M. Science, Vol. 327, Issue 5962 https://doi.org/10.1126/science.1180085	journal	January 2010
The magnetic structures of DyNi2Ge2 Islam, Zahirul; Detlefs, C.; Goldman, A. I. Solid State Communications, Vol. 108, Issue 6 https://doi.org/10.1016/S0038-1098(98)00387-1	journal	October 1998
Magnetic field tuning of antiferromagnetic Yb $_{3}$ Pt $_{4}$ Wu, L. S.; Janssen, Y.; Marques, C. Physical Review B, Vol. 84, Issue 13 https://doi.org/10.1103/PhysRevB.84.134409	journal	October 2011
From confined spinons to emergent fermions: Observation of elementary magnetic excitations in a transverse-field Ising chain Wang, Zhe; Wu, Jianda; Xu, Shenglong Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/PhysRevB.94.125130	journal	September 2016
Evidence for low-dimensional magnetic behaviour in CePt₅Ge₃ Hossain, Z.; Takabatake, T.; Geibel, C. Journal of Physics: Condensed Matter, Vol. 13, Issue 20 https://doi.org/10.1088/0953-8984/13/20/314	journal	May 2001
Spinon confinement in the one-dimensional Ising-like antiferromagnet ${SrCo}_{2} V_{2} O_{8}$ Wang, Zhe; Schmidt, M.; Bera, A. K. Physical Review B, Vol. 91, Issue 14 https://doi.org/10.1103/PhysRevB.91.140404	journal	April 2015
Quantum Criticality of the Ising-like Screw Chain Antiferromagnet ${SrCo}_{2} V_{2} O_{8}$ in a Transverse Magnetic Field Cui, Y.; Zou, H.; Xi, N. Physical Review Letters, Vol. 123, Issue 6 https://doi.org/10.1103/PhysRevLett.123.067203	journal	August 2019
Tomonaga–Luttinger liquid behavior and spinon confinement in YbAlO3 Wu, L. S.; Nikitin, S. E.; Wang, Z. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08485-7	journal	February 2019
Zur Theorie der Metalle: I. Eigenwerte und Eigenfunktionen der linearen Atomkette Bethe, H. Zeitschrift f�r Physik, Vol. 71, Issue 3-4 https://doi.org/10.1007/BF01341708	journal	March 1931
An Exactly Soluble Model of a Many‐Fermion System Luttinger, J. M. Journal of Mathematical Physics, Vol. 4, Issue 9 https://doi.org/10.1063/1.1704046	journal	September 1963
Novel Longitudinal Mode in the Coupled Quantum Chain Compound ${KCuF}_{3}$ Lake, B.; Tennant, D. A.; Nagler, S. E. Physical Review Letters, Vol. 85, Issue 4 https://doi.org/10.1103/PhysRevLett.85.832	journal	July 2000
Confinement of fractional quantum number particles in a condensed-matter system Lake, Bella; Tsvelik, Alexei M.; Notbohm, Susanne Nature Physics, Vol. 6, Issue 1 https://doi.org/10.1038/nphys1462	journal	November 2009

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