Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy

Sun, Yanwen; Carini, Gabriella; Chollet, Matthieu; Decker, Franz-Josef; Dunne, Mike; Fuoss, Paul; Hruszkewycz, Stephan O.; Lane, Thomas J.; Nakahara, Kazutaka; Nelson, Silke; Robert, Aymeric; Sato, Takahiro; Song, Sanghoon; Stephenson, G. Brian; Sutton, Mark; Van Driel, Tim B.; Weninger, Clemens; Zhu, Diling

doi:10.1103/physrevlett.127.058001

Title: Nonuniform Flow Dynamics Probed by Nanosecond X-Ray Speckle Visibility Spectroscopy

Journal Article · Wed Jul 28 00:00:00 EDT 2021 · Physical Review Letters

DOI:https://doi.org/10.1103/physrevlett.127.058001· OSTI ID:1809065

^[1]; Carini, Gabriella ^[1]; Chollet, Matthieu ^[1]; Decker, Franz-Josef ^[1]; Dunne, Mike ^[1]; Fuoss, Paul ^[1];

^[2]; Lane, Thomas J. ^[1]; Nakahara, Kazutaka ^[1]; Nelson, Silke ^[1];

^[1]; Sato, Takahiro ^[1];

^[1];

^[2]; Sutton, Mark ^[3]; Van Driel, Tim B. ^[1]; Weninger, Clemens ^[1]; Zhu, Diling ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)
Argonne National Lab. (ANL), Argonne, IL (United States)
McGill Univ., Montreal, QC (Canada); SLAC National Accelerator Lab., Menlo Park, CA (United States). Linac Coherent Light Source (LCLS)

We report observations of nanosecond nonuniform colloidal dynamics in a free flowing liquid jet using ultrafast x-ray speckle visibility spectroscopy. Utilizing a nanosecond double-bunch mode, the Linac Coherent Light Source free electron laser produced pairs of femtosecond coherent hard x-ray pulses. By exploring anisotropy in the visibility of summed speckle patterns which relates to the correlation functions, we evaluate not only the average particle flow rate in a colloidal nanoparticle jet, but also the nonuniform flow field within. The methodology presented here establishes the foundation for the study of nano- and atomic-scale inhomogeneous fluctuations in complex matter using x-ray free electron laser sources.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States); Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; AC02-76SF00515; AC02-06CH11357

OSTI ID:: 1809065

Alternate ID(s):: OSTI ID: 1819702; OSTI ID: 1828894

Report Number(s):: BNL-221842-2021-JAAM; TRN: US2213142

Journal Information:: Physical Review Letters, Vol. 127, Issue 5; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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