skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Demonstration of nitrogen-incorporated ultrananocrystalline diamond photocathodes in a RF gun environment

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/5.0029512· OSTI ID:1765464

Quantum efficiency (QE), intrinsic emittance, and robustness are the three most important figures of merit for photocathodes, the first two determine the ultimate achievable brightness of an electron beam, and the third one directly correlates with the complications of a beamline design. Nitrogen-incorporated ultrananocrystalline diamond [(N)UNCD] materials are promising candidates for photocathode applications due to their remarkable electron emission performance as well as the moderate vacuum requirement. Two (N)UNCD photocathodes have been characterized in a realistic RF gun environment with the nicely balanced performance of all three figures of merit. In this work, the QE of the first (N)UNCD cathode (stored in air for two years before the test) was found to be 3.8 x 10–4 using a 262 nm UV laser and a cathode surface field of 30MV/m. It was found that the QE of the second (N)UNCD sample (grown days before the test) was nearly the same and, therefore, demonstrates the exceptional environmental tolerance of the material. The intrinsic emittance of (N)UNCD was measured to be 1.00 μm/mm.

Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Engineering & Technology. Office of Small Business Innovation Research (SBIR) and Small Business Technology Transfer (STTR) Programs
Grant/Contract Number:
AC02-06CH11357; PHY-1403952; SC0015479; SC0013145
OSTI ID:
1765464
Alternate ID(s):
OSTI ID: 1690301
Journal Information:
Applied Physics Letters, Vol. 117, Issue 17; ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (34)

Planar ultrananocrystalline diamond field emitter in accelerator radio frequency electron injector: Performance metrics journal November 2014
Single-Shot MeV Transmission Electron Microscopy with Picosecond Temporal Resolution journal August 2014
Quantum Efficiencies of Mg Photocathode under Illumination with 3rd and 4th Harmonics Nd: LiYF 4 Laser Light in RF Gun journal March 2003
Synthesis and characterization of highly-conducting nitrogen-doped ultrananocrystalline diamond films journal September 2001
Advances in bright electron sources
  • Musumeci, P.; Giner Navarro, J.; Rosenzweig, J. B.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 907 https://doi.org/10.1016/j.nima.2018.03.019
journal November 2018
Electron Affinity of the Bare and Hydrogen Covered Single Crystal Diamond (111) Surface journal July 1998
First lasing and operation of an ångstrom-wavelength free-electron laser journal August 2010
Mean transverse energy of ultrananocrystalline diamond photocathode journal March 2019
Nanodiamond Thin Film Field Emitter Cartridge for Miniature High-Gradient Radio Frequency ${X}$ -Band Electron Injector journal March 2018
Multiwavelength Raman spectroscopy of diamond nanowires present in n -type ultrananocrystalline films journal December 2007
Cathode R&D for future light sources
  • Dowell, D. H.; Bazarov, I.; Dunham, B.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 622, Issue 3 https://doi.org/10.1016/j.nima.2010.03.104
journal October 2010
Rapid thermal emittance and quantum efficiency mapping of a cesium telluride cathode in an rf photoinjector using multiple laser beamlets journal May 2020
Breaking 50 Femtosecond Resolution Barrier in MeV Ultrafast Electron Diffraction with a Double Bend Achromat Compressor journal March 2020
Intrinsic Emittance Reduction of an Electron Beam from Metal Photocathodes journal June 2010
Overcoming the quantum efficiency-lifetime tradeoff of photocathodes by coating with atomically thin two-dimensional nanomaterials journal June 2018
Photoemission studies on niobium for superconducting photoinjectors journal August 2005
A low emittance and high efficiency visible light photocathode for high brightness accelerator-based X-ray light sources journal July 2011
The degradation of quantum efficiency in negative electron affinity GaAs photocathodes under gas exposure journal January 2014
High power conditioning and benchmarking of planar nitrogen-incorporated ultrananocrystalline diamond field emission electron source journal December 2019
Schottky-Enabled Photoemission in a rf Accelerator Photoinjector: Possible Generation of Ultralow Transverse Thermal-Emittance Electron Beam journal September 2004
In Situ Observation of Dark Current Emission in a High Gradient rf Photocathode Gun journal August 2016
Commissioning the Linac Coherent Light Source injector journal March 2008
Direct observation of electron emission from grain boundaries in CVD diamond by PeakForce-controlled tunnelling atomic force microscopy journal November 2015
Submicrometer ultrananocrystalline diamond films processed in oxygen and hydrogen plasma and analyzed by UV-vis spectroscopy: Thickness and optical constant results journal December 2020
Combined visible light photo-emission and low temperature thermionic emission from nitrogen doped diamond films journal November 2011
Overestimation of thermal emittance in solenoid scans due to coupled transverse motion journal December 2018
Bonding structure in nitrogen doped ultrananocrystalline diamond journal May 2003
Photoemission properties of nanocrystalline diamond thin films on silicon
  • Mazellier, Jean-Paul; Di Giola, Cyril; Legagneux, Pierre
  • Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 33, Issue 3 https://doi.org/10.1116/1.4904547
journal May 2015
Brightness of femtosecond nonequilibrium photoemission in metallic photocathodes at wavelengths near the photoemission threshold journal December 2018
Direct observation of electron emission from the grain boundaries of chemical vapour deposition diamond films by tunneling atomic force microscopy journal April 2014
In situ cleaning of metal cathodes using a hydrogen ion beam journal June 2006
Locally Resolved Electron Emission Area and Unified View of Field Emission from Ultrananocrystalline Diamond Films journal September 2017
Quantum efficiency and thermal emittance of metal photocathodes journal July 2009
High quantum efficiency ultrananocrystalline diamond photocathode for photoinjector applications
  • Pérez Quintero, Kenneth J.; Antipov, Sergey; Sumant, Anirudha V.
  • Applied Physics Letters, Vol. 105, Issue 12, Article No. 123103 https://doi.org/10.1063/1.4896418
journal September 2014

Similar Records

Mean transverse energy of ultrananocrystalline diamond photocathode
Journal Article · Mon Mar 04 00:00:00 EST 2019 · Applied Physics Letters · OSTI ID:1765464

High power conditioning and benchmarking of planar nitrogen-incorporated ultrananocrystalline diamond field emission electron source
Journal Article · Wed Dec 11 00:00:00 EST 2019 · Physical Review Accelerators and Beams · OSTI ID:1765464

Quantum efficiency, photoemission energy spectra, and mean transverse energy of ultrananocrystalline diamond photocathode
Journal Article · Fri Dec 09 00:00:00 EST 2022 · Journal of Applied Physics · OSTI ID:1765464

Related Subjects