Crystal fields and magnetic structure of the Ising antiferromagnet Er3Ga5O12

Cai, Y.; Wilson, M. N.; Beare, J.; Lygouras, C.; Thomas, G.; Yahne, D. R.; Ross, K.; Taddei, Keith M.; Sala, Gabriele; Dabkowska, H. A.; Aczel, Adam A.; Luke, G. M.

doi:10.1103/PhysRevB.100.184415

Title: Crystal fields and magnetic structure of the Ising antiferromagnet Er₃Ga₅O₁₂

Journal Article · Mon Nov 18 00:00:00 EST 2019 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.100.184415· OSTI ID:1607071

^[1]; Wilson, M. N. ^[1]; Beare, J. ^[1]; Lygouras, C. ^[1]; Thomas, G. ^[1]; Yahne, D. R. ^[2]; Ross, K. ^[3];

^[4];

^[4]; Dabkowska, H. A. ^[1];

^[5]; Luke, G. M. ^[6]

McMaster Univ., Hamilton, ON (Canada)
Colorado State Univ., Fort Collins, CO (United States). Physics Dept.
Colorado State Univ., Fort Collins, CO (United States). Physics Dept.; Canadian Inst. for Advanced Research, Toronto, Ontario, Canada
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division; Univ. of Tennessee, Knoxville, TN (United States). Dept. of Physics and Astronomy
McMaster Univ., Hamilton, ON (Canada); Canadian Inst. for Advanced Research, Toronto, ON (Canada); TRIUMF, Vancouver, BC (Canada)

Rare-earth garnets are an exciting playground for studying the exotic magnetic properties of the frustrated hyperkagome lattice. In this paper we present a comprehensive study of the single ion and collective magnetic properties of the garnet ${Er}_{3} {Ga}_{5} O_{12}$ . Using inelastic neutron scattering, we find a crystal-field ground-state doublet for ${Er}^{3 +}$ with strong Ising anisotropy along local [100] axes. Magnetic susceptibility and heat-capacity measurements provide evidence for long-range magnetic ordering with $T_{N} = 0.8 K$ , and no evidence for residual entropy is found when cooling through the ordering transition. Neutron powder diffraction reveals that the ground-state spin configuration corresponds to the six-sublattice, Ising antiferromagnetic state ( $Γ_{3}$ ) common to many of the rare-earth garnets. However, we also found that $μ SR$ appears to be insensitive to the ordering transition in this material, in which a low-temperature relaxation plateau was observed with no evidence of spontaneous muon precession. The combined muon and neutron results may be indicative of a dynamical ground state with a relatively long correlation time. Despite this potential complication, our work indicates that ${Er}_{3} {Ga}_{5} O_{12}$ is an excellent model system for studying the complex metamagnetism expected for a multiaxis antiferromagnet.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS) and High Flux Isotope Reactor (HFIR)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); Natural Sciences and Engineering Research Council of Canada (NSERC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1607071

Journal Information:: Physical Review B, Vol. 100, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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Title: Crystal fields and magnetic structure of the Ising antiferromagnet Er₃Ga₅O₁₂