Why ionizing radiation enhances surface wettability

Seshadri, Arunkumar; Forrest, Eric C.; Shirvan, Koroush

doi:10.1016/j.apsusc.2020.145935

Title: Why ionizing radiation enhances surface wettability

Journal Article · Fri Feb 28 00:00:00 EST 2020 · Applied Surface Science

DOI:https://doi.org/10.1016/j.apsusc.2020.145935· OSTI ID:1605721

^[1]; Forrest, Eric C. ^[1];

^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Radiation-Induced Surface Activation is an inherent phenomenon where surfaces that are exposed to gamma irradiation are observed to undergo an increase in wettability. This increase in wettability as a result of the ionizing radiation exposure has so far been demonstrated to have a pronounced impact on Leidenfrost temperature and two-phase fluid dynamics. Test results from previous experiments have shown that incorporation of this effect on heat transfer equipment design may increase the thermal-hydraulic margin leading to higher thermal efficiency. However, the mechanism behind the increased wettability is not clearly understood. In the present work, three different materials (Zircaloy-4, 316 stainless steel, and copper) were exposed at two different dose rates with use of two different gamma irradiation facilities. A detailed surface characterization on the post-irradiated samples is carried out to understand the changes in surface chemistry, wettability and surface morphology. It is observed from the experiments that the increase in wettability upon irradiation depended on the total dose and not on the dose rate. Moreover, localized oxidation and porosity induced by radiolysis was seen to be the predominant mechanism behind increased wettability which leads to improved Leidenfrost temperature.

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE Office of Nuclear Energy (NE)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1605721

Alternate ID(s):: OSTI ID: 1776967

Report Number(s):: SAND-2020-2747J; 684509

Journal Information:: Applied Surface Science, Vol. 514, Issue C; ISSN 0169-4332

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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