Role of Tartaric Acid in Chemical, Mechanical and Self-Healing Behaviors of a Calcium-Aluminate Cement Blend with Fly Ash F under Steam and Alkali Carbonate Environments at 270°C

Pyatina, Tatiana; Sugama, Toshifumi

doi:10.3390/ma10040342

Title: Role of Tartaric Acid in Chemical, Mechanical and Self-Healing Behaviors of a Calcium-Aluminate Cement Blend with Fly Ash F under Steam and Alkali Carbonate Environments at 270°C

Journal Article · Sat Mar 25 00:00:00 EDT 2017 · Materials

DOI:https://doi.org/10.3390/ma10040342· OSTI ID:1392214

Pyatina, Tatiana ^[1]; Sugama, Toshifumi ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States)

Tartaric acid (TA) changes short-term mechanical behavior and phase composition of sodium-metasilicate activated calcium-aluminate cement blend with fly ash, type F, when used as a set control additive to allow sufficient pumping time for underground well placement. The present work focuses on TA effect on self-healing properties of the blend under steam or alkali carbonate environments at 270°C applicable to geothermal wells. Compressive strength recoveries and cracks sealing were examined to evaluate self-healing of the cement after repeated crush tests followed by two consecutive healing periods of 10 and 5 days at 270°C. Optical and scanning electron microscopes, X-ray diffraction, Fourier Transform infrared and EDX measurements along with thermal gravimetric analyses were used to identify phases participating in the healing processes. Samples with 1% mass fraction of TA by weight of blend demonstrated improved strength recoveries and crack plugging properties, especially in alkali carbonate environment. This effect was attributed to silicon-rich (C,N)-A-S-H amorphous phase predominant in TA-modified samples, high-temperature stable zeolite phases along with the formation of tobermorite-type crystals in the presence of tartaric acid.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Geothermal Technologies Office; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; AC02-98CH10886

OSTI ID:: 1392214

Report Number(s):: BNL-114134-2017-JA; MATEG9; R&D Project: 22444

Journal Information:: Materials, Vol. 10, Issue 4; ISSN 1996-1944

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 5 works

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Title: Role of Tartaric Acid in Chemical, Mechanical and Self-Healing Behaviors of a Calcium-Aluminate Cement Blend with Fly Ash F under Steam and Alkali Carbonate Environments at 270°C

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