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Title: Performance of a palladium membrane reactor using a Ni catalyst for fusion fuel impurities processing

Conference ·
OSTI ID:10162691
;  [1];  [2]
  1. Los Alamos National Lab., NM (United States)
  2. Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan)

The palladium membrane reactor (PNM) provides a means to recover hydrogen isotopes from impurities expected to be present in fusion reactor exhaust. This recovery is based on reactions such as water-gas shift and steam reforming for which conversion is equilibrium limited. By including a selectively permeable membrane such as Pd/Ag in the catalyst bed, hydrogen isotopes can be removed from the reacting environment, thus promoting the reaction to complete conversion. Such a device has been built and operated at the Tritium Systems Test Assembly (TSTA) at Los Alamos National Laboratory (LANL). For the reactions listed above, earlier study with this unit has shown that hydrogen single-pass recoveries approaching 100% can be achieved. It was also determined that a nickel catalyst is a feasible choice for use with a PMR appropriate for fusion fuel impurities processing. The purpose of this study was to systematically assess the performance of the PMR using a nickel catalyst over a range of temperatures, feed compositions and flowrates. Reactions which were studied are the water-gas shift reaction and steam reforming.

Research Organization:
Los Alamos National Lab., NM (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States); Japan Atomic Energy Research Inst., Tokyo (Japan)
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
10162691
Report Number(s):
LA-UR-94-2108; CONF-940664-16; ON: DE94014476; TRN: 94:013651
Resource Relation:
Conference: ISFNT-3: international symposium on fusion nuclear technology,Los Angeles, CA (United States),27 Jun - 1 Jul 1994; Other Information: PBD: [1994]
Country of Publication:
United States
Language:
English