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Title: An innovative method for extracting isotopic information from low-resolution gamma spectra

Technical Report ·
DOI:https://doi.org/10.2172/296760· OSTI ID:296760

A method is described for the extraction of isotopic information from attenuated gamma ray spectra using the gross-count material basis set (GC-MBS) model. This method solves for the isotopic composition of an unknown mixture of isotopes attenuated through an absorber of unknown material. For binary isotopic combinations the problem is nonlinear in only one variable and is easily solved using standard line optimization techniques. Results are presented for NaI spectrum analyses of various binary combinations of enriched uranium, depleted uranium, low burnup Pu, {sup 137}Cs, and {sup 133}Ba attenuated through a suite of absorbers ranging in Z from polyethylene through lead. The GC-MBS method results are compared to those computed using ordinary response function fitting and with a simple net peak area method. The GC-MBS method was found to be significantly more accurate than the other methods over the range of absorbers and isotopic blends studied.

Research Organization:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
296760
Report Number(s):
LA-UR-98-1899; CONF-980545-; ON: DE99000666; TRN: 99:003051
Resource Relation:
Conference: 9. symposium on radiation measurements and applications, Ann Arbor, MI (United States), 11-14 May 1998; Other Information: PBD: [1998]
Country of Publication:
United States
Language:
English