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Title: Experimental demonstration of broadband solar absorption beyond the lambertian limit in certain thin silicon photonic crystals

Abstract

The tantalizing possibility of 31% solar-to-electric power conversion efficiency in thin film crystalline silicon solar cell architectures relies essentially on solar absorption well beyond the Lambertian light trapping limit (Bhattacharya and John in Nat Sci Rep 9:12482, 2019). Up to now, no solar cell architecture has exhibited above-Lambertian solar absorption, integrated over the broad solar spectrum. In this work, we experimentally demonstrate two types of photonic crystal (PhC) solar cells architectures that exceed Lambertian light absorption, integrated over the entire 300–1,200 nm wavelength band. These measurements confirm theoretically predicted wave-interference-based optical resonances associated with long lifetime, slow-light modes and parallel-to-interface refraction. These phenomena are beyond the realm of ray optics. Using two types of 10-μm thick PhC’s, first an Inverted Pyramid PhC with lattice constant a= 2,500 nm and second a Teepee PhC with a = 1,200 nm, we observe solar absorption well beyond the Lambertian limit over λ = 950–1,200 nm. Our absorption measurements correspond to the maximum-achievable-photocurrent-density (MAPD), under AM1.5G illumination at 4-degree incident angle, 41.29 and 41.52 mA/cm2 for the Inverted Pyramid and Teepee PhC, respectively, in agreement with wave-optics, numerical simulations. Both of these values exceed the MAPD (= 39.63 mA/cm2) corresponding to the Lambertian limitmore » for a 10-μm thick silicon for solar absorption over the 300–1,200 nm band.« less

Authors:
 [1];  [2];  [3];  [4];  [1]
  1. Rensselaer Polytechnic Inst., Troy, NY (United States). Center for Future Energy System (CFES); National Chiao-Tung Univ., Hsinchu (Taiwan)
  2. Rensselaer Polytechnic Inst., Troy, NY (United States). Center for Future Energy System (CFES)
  3. Univ. of Toronto, ON (Canada); Indraprastha Inst. of Information Technology, New Delhi (India)
  4. Univ. of Toronto, ON (Canada)
Publication Date:
Research Org.:
Rensselaer Polytechnic Inst., Troy, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Natural Science Foundation (NSF)
OSTI Identifier:
1647330
Grant/Contract Number:  
FG02-06ER46347; ECCS-1840673-NOA
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Energy science and technology; materials science; nanoscience and technology; optics and photonics

Citation Formats

Hsieh, Mei-Li, Kaiser, Alex, Bhattacharya, Sayak, John, Sajeev, and Lin, Shawn-Yu. Experimental demonstration of broadband solar absorption beyond the lambertian limit in certain thin silicon photonic crystals. United States: N. p., 2020. Web. doi:10.1038/s41598-020-68704-w.
Hsieh, Mei-Li, Kaiser, Alex, Bhattacharya, Sayak, John, Sajeev, & Lin, Shawn-Yu. Experimental demonstration of broadband solar absorption beyond the lambertian limit in certain thin silicon photonic crystals. United States. https://doi.org/10.1038/s41598-020-68704-w
Hsieh, Mei-Li, Kaiser, Alex, Bhattacharya, Sayak, John, Sajeev, and Lin, Shawn-Yu. Thu . "Experimental demonstration of broadband solar absorption beyond the lambertian limit in certain thin silicon photonic crystals". United States. https://doi.org/10.1038/s41598-020-68704-w. https://www.osti.gov/servlets/purl/1647330.
@article{osti_1647330,
title = {Experimental demonstration of broadband solar absorption beyond the lambertian limit in certain thin silicon photonic crystals},
author = {Hsieh, Mei-Li and Kaiser, Alex and Bhattacharya, Sayak and John, Sajeev and Lin, Shawn-Yu},
abstractNote = {The tantalizing possibility of 31% solar-to-electric power conversion efficiency in thin film crystalline silicon solar cell architectures relies essentially on solar absorption well beyond the Lambertian light trapping limit (Bhattacharya and John in Nat Sci Rep 9:12482, 2019). Up to now, no solar cell architecture has exhibited above-Lambertian solar absorption, integrated over the broad solar spectrum. In this work, we experimentally demonstrate two types of photonic crystal (PhC) solar cells architectures that exceed Lambertian light absorption, integrated over the entire 300–1,200 nm wavelength band. These measurements confirm theoretically predicted wave-interference-based optical resonances associated with long lifetime, slow-light modes and parallel-to-interface refraction. These phenomena are beyond the realm of ray optics. Using two types of 10-μm thick PhC’s, first an Inverted Pyramid PhC with lattice constant a= 2,500 nm and second a Teepee PhC with a = 1,200 nm, we observe solar absorption well beyond the Lambertian limit over λ = 950–1,200 nm. Our absorption measurements correspond to the maximum-achievable-photocurrent-density (MAPD), under AM1.5G illumination at 4-degree incident angle, 41.29 and 41.52 mA/cm2 for the Inverted Pyramid and Teepee PhC, respectively, in agreement with wave-optics, numerical simulations. Both of these values exceed the MAPD (= 39.63 mA/cm2) corresponding to the Lambertian limit for a 10-μm thick silicon for solar absorption over the 300–1,200 nm band.},
doi = {10.1038/s41598-020-68704-w},
journal = {Scientific Reports},
number = 1,
volume = 10,
place = {United States},
year = {Thu Jul 16 00:00:00 EDT 2020},
month = {Thu Jul 16 00:00:00 EDT 2020}
}

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