Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge

Zhou, Guangmin; Paek, Eunsu; Hwang, Gyeong S.; Manthiram, Arumugam

doi:10.1038/ncomms8760

Title: Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge

Abstract

Lithium–sulphur batteries with a high theoretical energy density are regarded as promising energy storage devices for electric vehicles and large-scale electricity storage. However, the low active material utilization, low sulphur loading and poor cycling stability restrict their practical applications. Herein, we present an effective strategy to obtain Li/polysulphide batteries with high-energy density and long-cyclic life using three-dimensional nitrogen/sulphur codoped graphene sponge electrodes. The nitrogen/sulphur codoped graphene sponge electrode provides enough space for a high sulphur loading, facilitates fast charge transfer and better immobilization of polysulphide ions. The hetero-doped nitrogen/sulphur sites are demonstrated to show strong binding energy and be capable of anchoring polysulphides based on first-principles calculations. As a result, a high specific capacity of 1,200 mAh g^–1 at 0.2C rate, a high-rate capacity of 430 mAh g^–1 at 2C rate and excellent cycling stability for 500 cycles with ~0.078% capacity decay per cycle are achieved.

Authors:

Zhou, Guangmin ^[1]; Paek, Eunsu ^[1]; Hwang, Gyeong S. ^[1]; Manthiram, Arumugam ^[1]

Univ. of Texas, Austin, TX (United States)

Publication Date:: Fri Jul 17 00:00:00 EDT 2015

Research Org.:: Ceramatec, Inc., West Valley City, UT (United States

Sponsoring Org.:: USDOE Advanced Research Projects Agency - Energy (ARPA-E); Robert A. Welch Foundation

OSTI Identifier:: 1623994

Grant/Contract Number:: AR0000377; F-1535

Resource Type:: Accepted Manuscript

Journal Name:: Nature Communications

Additional Journal Information:: Journal Volume: 6; Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 36 MATERIALS SCIENCE; 25 ENERGY STORAGE; science & technology - other topics; batteries; chemical physics; graphene

Citation Formats


                    Zhou, Guangmin, Paek, Eunsu, Hwang, Gyeong S., and Manthiram, Arumugam. Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge.  United States: N. p., 2015. 
Web.  doi:10.1038/ncomms8760.

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                    Zhou, Guangmin, Paek, Eunsu, Hwang, Gyeong S., & Manthiram, Arumugam. Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge.  United States.  https://doi.org/10.1038/ncomms8760

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                    Zhou, Guangmin, Paek, Eunsu, Hwang, Gyeong S., and Manthiram, Arumugam. Fri .  
"Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge".  United States.  https://doi.org/10.1038/ncomms8760.  https://www.osti.gov/servlets/purl/1623994.

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@article{osti_1623994,

  title        = {Long-life Li/polysulphide batteries with high sulphur loading enabled by lightweight three-dimensional nitrogen/sulphur-codoped graphene sponge},

  author       = {Zhou, Guangmin and Paek, Eunsu and Hwang, Gyeong S. and Manthiram, Arumugam},

  abstractNote = {Lithium–sulphur batteries with a high theoretical energy density are regarded as promising energy storage devices for electric vehicles and large-scale electricity storage. However, the low active material utilization, low sulphur loading and poor cycling stability restrict their practical applications. Herein, we present an effective strategy to obtain Li/polysulphide batteries with high-energy density and long-cyclic life using three-dimensional nitrogen/sulphur codoped graphene sponge electrodes. The nitrogen/sulphur codoped graphene sponge electrode provides enough space for a high sulphur loading, facilitates fast charge transfer and better immobilization of polysulphide ions. The hetero-doped nitrogen/sulphur sites are demonstrated to show strong binding energy and be capable of anchoring polysulphides based on first-principles calculations. As a result, a high specific capacity of 1,200 mAh g–1 at 0.2C rate, a high-rate capacity of 430 mAh g–1 at 2C rate and excellent cycling stability for 500 cycles with ~0.078% capacity decay per cycle are achieved.},

  doi          = {10.1038/ncomms8760},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 6,

  place        = {United States},

  year         = {Fri Jul 17 00:00:00 EDT 2015},

  month        = {Fri Jul 17 00:00:00 EDT 2015}

}

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Sulfiphilic Nickel Phosphosulfide Enabled Li ₂ S Impregnation in 3D Graphene Cages for Li-S Batteries
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More Reliable Lithium-Sulfur Batteries: Status, Solutions and Prospects
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Integration of Graphene, Nano Sulfur, and Conducting Polymer into Compact, Flexible Lithium-Sulfur Battery Cathodes with Ultrahigh Volumetric Capacity and Superior Cycling Stability for Foldable Devices
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Polymeric Graphene Bulk Materials with a 3D Cross-Linked Monolithic Graphene Network
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Chen, Wangqiao; Xiao, Peishuang; Chen, Honghui
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Long-Life Lithium-Sulfur Batteries with a Bifunctional Cathode Substrate Configured with Boron Carbide Nanowires
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Luo, Liu; Chung, Sheng-Heng; Yaghoobnejad Asl, Hooman
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Single Nickel Atoms on Nitrogen‐Doped Graphene Enabling Enhanced Kinetics of Lithium–Sulfur Batteries
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High-Performance Lithium-Sulfur Batteries with a Self-Supported, 3D Li ₂ S-Doped Graphene Aerogel Cathodes
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From Hollow Carbon Spheres to N-Doped Hollow Porous Carbon Bowls: Rational Design of Hollow Carbon Host for Li-S Batteries
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Emergent Pseudocapacitance of 2D Nanomaterials
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Double-Shelled Nanocages with Cobalt Hydroxide Inner Shell and Layered Double Hydroxides Outer Shell as High-Efficiency Polysulfide Mediator for Lithium-Sulfur Batteries
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Bi ₂ S ₃ /Ketjen Black as a Highly Efficient Bifunctional Catalyst for Long‐Cycle Lithium‐Oxygen Batteries
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Dual Heteroatom-Doped Carbon Nanofoam-Wrapped Iron Monosulfide Nanoparticles: An Efficient Cathode Catalyst for Li-O ₂ Batteries
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Plasma Treatment for Nitrogen-Doped 3D Graphene Framework by a Conductive Matrix with Sulfur for High-Performance Li-S Batteries
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Balancing surface adsorption and diffusion of lithium-polysulfides on nonconductive oxides for lithium–sulfur battery design
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Chen, Liang; Shi, Mengting; He, Binhong
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3D Ferroconcrete-Like Aminated Carbon Nanotubes Network Anchoring Sulfur for Advanced Lithium–Sulfur Battery
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Yan, M.; Chen, H.; Yu, Y.
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Sandwich-Type Nitrogen and Sulfur Codoped Graphene-Backboned Porous Carbon Coated Separator for High Performance Lithium-Sulfur Batteries
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Chen, Feng; Ma, Lulu; Ren, Jiangang
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Chem-Bonding and Phys-Trapping Se Electrode for Long-Life Rechargeable Batteries
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Wu, Tianjing; Ding, Zhiying; Jing, Mingjun
Advanced Functional Materials, Vol. 29, Issue 9
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Mutually Exclusive p‐Type and n‐Type Hybrid Electrode of MoS ₂ and Graphene for Artificial Soft Touch Fingers
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Manzoor, Muhammad Taha; Nguyen, Van Hiep; Umrao, Sima
Advanced Functional Materials, Vol. 29, Issue 48
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Rational Design of Binders for Stable Li‐S and Na‐S Batteries
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Guo, Qianyi; Zheng, Zijian
Advanced Functional Materials, Vol. 30, Issue 6
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A Cooperative Interface for Highly Efficient Lithium-Sulfur Batteries
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Peng, Hong-Jie; Zhang, Ze-Wen; Huang, Jia-Qi
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Recent Progress in the Design of Advanced Cathode Materials and Battery Models for High-Performance Lithium-X (X = O ₂ , S, Se, Te, I ₂ , Br ₂ ) Batteries
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Xu, Jiantie; Ma, Jianmin; Fan, Qinghua
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A Top-Down Strategy toward SnSb In-Plane Nanoconfined 3D N-Doped Porous Graphene Composite Microspheres for High Performance Na-Ion Battery Anode
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Qin, Jian; Wang, Tianshuai; Liu, Dongye
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Simultaneous Suppression of the Dendrite Formation and Shuttle Effect in a Lithium-Sulfur Battery by Bilateral Solid Electrolyte Interface
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Fan, Ling; Chen, Suhua; Zhu, Jingyi
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Polysulfide-Shuttle Control in Lithium-Sulfur Batteries with a Chemically/Electrochemically Compatible NaSICON-Type Solid Electrolyte
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Yu, Xingwen; Bi, Zhonghe; Zhao, Feng
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Hierarchical Structures Based on Two-Dimensional Nanomaterials for Rechargeable Lithium Batteries
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Bi ₂ S ₃ /Ketjen Black as a Highly Efficient Bifunctional Catalyst for Long‐Cycle Lithium‐Oxygen Batteries
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Xu, Peng; Zhu, Jiajia; Chen, Congdi
ChemElectroChem, Vol. 6, Issue 15
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Few‐Layer Boron Nitride with Engineered Nitrogen Vacancies for Promoting Conversion of Polysulfide as a Cathode Matrix for Lithium–Sulfur Batteries
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Yi, Yikun; Li, Hongping; Chang, Honghong
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Electrospun zeolitic imidazolate framework-derived nitrogen-doped carbon nanofibers with high performance for lithium-sulfur batteries
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N-doped Mesoporous Carbon/Graphene Aerogels as Sulfur Hosts for High-Performance Lithium-Sulfur Batteries
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Chemical Confinement and Utility of Lithium Polysulfides in Lithium Sulfur Batteries
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The dual actions of modified polybenzimidazole in taming the polysulfide shuttle for long-life lithium–sulfur batteries
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Sandwich-Type Nitrogen and Sulfur Codoped Graphene-Backboned Porous Carbon Coated Separator for High Performance Lithium-Sulfur Batteries
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Three-dimensional Fe₃O₄/N-graphene sponge as an efficient organosulfide host for high-performance lithium-organosulfur batteries

Journal Article He, Jiarui ; Bhargav, Amruth ; Manthiram, Arumugam - Energy Storage Materials

The rapid capacity decay and unclear mechanism for the capacity fade limit the practical application of lithium-organosulfur batteries. Herein, we employ dimethyl trisulfide (DMTS) as a model compound to investigate the capacity fading mechanism and propose a solution to improve its cycling stability. Our results reveal that both DMTS and its discharge products (e.g., LiSCH₃, LiSSCH₃) are soluble in the electrolyte, leading to severe active material migration and loss, which becomes the predominant capacity fading mechanism. A three-dimensional nitrogen-doped graphene sponge decorated with Fe₃O₄ nanoparticles (3DFNG) is designed as a host for DMTS, which effectively confine the active material, enablingmore »« less
Cited by 30
https://doi.org/10.1016/j.ensm.2019.05.027

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Citation Formats

Issues and challenges facing rechargeable lithium batteries journal, November 2001

Electrical Energy Storage for the Grid: A Battery of Choices journal, November 2011

Li–O2 and Li–S batteries with high energy storage journal, January 2012

Nanostructured sulfur cathodes journal, January 2013

Rechargeable Lithium–Sulfur Batteries journal, July 2014

Sulfur Cathodes with Hydrogen Reduced Titanium Dioxide Inverse Opal Structure journal, April 2014

Challenges and Prospects of Lithium–Sulfur Batteries journal, June 2012

Carbon–sulfur composites for Li–S batteries: status and prospects journal, January 2013

Preparation of N-doped activated carbons for electric double-layer capacitors from waste fiberboard by K2CO3 activation journal, April 2014

A highly ordered nanostructured carbon–sulphur cathode for lithium–sulphur batteries journal, May 2009

Amphiphilic Surface Modification of Hollow Carbon Nanofibers for Improved Cycle Life of Lithium Sulfur Batteries journal, February 2013

Lithium-Sulfur Batteries: Electrochemistry, Materials, and Prospects journal, November 2013

Tailoring Microstructure of Graphene-Based Membrane by Controlled Removal of Trapped Water Inspired by the Phase Diagram journal, February 2014

Insight into the Electrode Mechanism in Lithium-Sulfur Batteries with Ordered Microporous Carbon Confined Sulfur as the Cathode journal, November 2013

Sulphur–TiO2 yolk–shell nanoarchitecture with internal void space for long-cycle lithium–sulphur batteries journal, January 2013

Polydopamine-Coated, Nitrogen-Doped, Hollow Carbon–Sulfur Double-Layered Core–Shell Structure for Improving Lithium–Sulfur Batteries journal, August 2014

Phosphorous Pentasulfide as a Novel Additive for High-Performance Lithium-Sulfur Batteries journal, June 2012

Dendrite-Free Lithium Deposition via Self-Healing Electrostatic Shield Mechanism journal, March 2013

Nitrogen-Doped Mesoporous Carbon Promoted Chemical Adsorption of Sulfur and Fabrication of High-Areal-Capacity Sulfur Cathode with Exceptional Cycling Stability for Lithium-Sulfur Batteries journal, October 2013

Fibrous Hybrid of Graphene and Sulfur Nanocrystals for High-Performance Lithium–Sulfur Batteries journal, May 2013

Strongly Coupled Interfaces between a Heterogeneous Carbon Host and a Sulfur-Containing Guest for Highly Stable Lithium-Sulfur Batteries: Mechanistic Insight into Capacity Degradation journal, July 2014

Enhancing lithium–sulphur battery performance by strongly binding the discharge products on amino-functionalized reduced graphene oxide journal, September 2014

Development and costs calculation of lithium–sulfur cells with high sulfur load and binder free electrodes journal, February 2013

Key Parameters Governing the Energy Density of Rechargeable Li/S Batteries journal, February 2014

A Facile Layer-by-Layer Approach for High-Areal-Capacity Sulfur Cathodes journal, January 2015

Lithium-Ion Textile Batteries with Large Areal Mass Loading journal, October 2011

Very High Surface Capacity Observed Using Si Negative Electrodes Embedded in Copper Foam as 3D Current Collectors journal, February 2014

A lithium–sulfur cathode with high sulfur loading and high capacity per area: a binder-free carbon fiber cloth–sulfur material journal, January 2014

Three-Dimensional Sulfur/Graphene Multifunctional Hybrid Sponges for Lithium-Sulfur Batteries with Large Areal Mass Loading journal, April 2014

Hierarchical Free-Standing Carbon-Nanotube Paper Electrodes with Ultrahigh Sulfur-Loading for Lithium-Sulfur Batteries journal, July 2014

A graphene foam electrode with high sulfur loading for flexible and high energy Li-S batteries journal, January 2015

Highly Reversible Lithium/Dissolved Polysulfide Batteries with Carbon Nanotube Electrodes journal, May 2013

A membrane-free lithium/polysulfide semi-liquid battery for large-scale energy storage journal, January 2013

Liquid-Type Cathode Enabled by 3D Sponge-Like Carbon Nanotubes for High Energy Density and Long Cycling Life of Li-S Batteries journal, October 2014

Carbonized Eggshell Membrane as a Natural Polysulfide Reservoir for Highly Reversible Li-S Batteries journal, November 2013

Sulfur-Functionalized Mesoporous Carbons as Sulfur Hosts in Li–S Batteries: Increasing the Affinity of Polysulfide Intermediates to Enhance Performance journal, February 2014

A pH-sensitive graphene oxide composite hydrogel journal, January 2010

An ice-templated, pH-tunable self-assembly route to hierarchically porous graphene nanoscroll networks journal, January 2014

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage journal, January 2008

Monolithic Fe2O3/graphene hybrid for highly efficient lithium storage and arsenic removal journal, February 2014

The reduction of graphene oxide journal, August 2012

BCN Graphene as Efficient Metal-Free Electrocatalyst for the Oxygen Reduction Reaction journal, March 2012

Three-Dimensional Nitrogen and Boron Co-doped Graphene for High-Performance All-Solid-State Supercapacitors journal, July 2012

Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide journal, June 2007

Graphene sponge for efficient and repeatable adsorption and desorption of water contaminations journal, January 2012

Cathode Composites for Li–S Batteries via the Use of Oxygenated Porous Architectures journal, October 2011

Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells journal, November 2011

Lithium/Sulfur Cell Discharge Mechanism: An Original Approach for Intermediate Species Identification journal, April 2012

Free-Standing Nitrogen-doped Graphene Paper as Electrodes for High-Performance Lithium/Dissolved Polysulfide Batteries journal, July 2014

Free-standing TiO2 nanowire-embedded graphene hybrid membrane for advanced Li/dissolved polysulfide batteries journal, March 2015

Improved lithium–sulfur cells with a treated carbon paper interlayer journal, January 2013

New insight into the discharge process of sulfur cathode by electrochemical impedance spectroscopy journal, April 2009

A Soft Approach to Encapsulate Sulfur: Polyaniline Nanotubes for Lithium-Sulfur Batteries with Long Cycle Life journal, January 2012

On the Surface Chemical Aspects of Very High Energy Density, Rechargeable Li–Sulfur Batteries journal, January 2009

Role of LiNO3 in rechargeable lithium/sulfur battery journal, May 2012

A Graphene-Pure-Sulfur Sandwich Structure for Ultrafast, Long-Life Lithium-Sulfur Batteries journal, November 2013

Formation of Large Polysulfide Complexes during the Lithium-Sulfur Battery Discharge journal, September 2014

Toward a Molecular Understanding of Energetics in Li–S Batteries Using Nonaqueous Electrolytes: A High-Level Quantum Chemical Study journal, May 2014

A quantum-chemical study on the discharge reaction mechanism of lithium-sulfur batteries journal, January 2013

Efficient Preparation of Large-Area Graphene Oxide Sheets for Transparent Conductive Films journal, August 2010

Generalized Gradient Approximation Made Simple journal, October 1996

Semiempirical GGA-type density functional constructed with a long-range dispersion correction journal, January 2006

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage journal, February 2009

Preparation of N-doped activated carbons for electric double-layer capacitors from waste fiberboard by K2CO3 activation journal, September 2014

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage journal, February 2009

BCN Graphene as Efficient Metal-Free Electrocatalyst for the Oxygen Reduction Reaction journal, March 2012

Highly Reversible Lithium/Dissolved Polysulfide Batteries with Carbon Nanotube Electrodes journal, May 2013

Lithium/Sulfur Cell Discharge Mechanism: An Original Approach for Intermediate Species Identification journal, April 2012

Issues and challenges facing rechargeable lithium batteries journal, November 2001

Phase Inversion: A Universal Method to Create High-Performance Porous Electrodes for Nanoparticle-Based Energy Storage Devices journal, October 2016

Functional Carbons Remedy the Shuttling of Polysulfides in Lithium-Sulfur Batteries: Confining, Trapping, Blocking, and Breaking up journal, March 2018

Manipulation of Edge‐Site Fe–N 2 Moiety on Holey Fe, N Codoped Graphene to Promote the Cycle Stability and Rate Capacity of Li–S Batteries journal, December 2018

3D Interconnected Electrode Materials with Ultrahigh Areal Sulfur Loading for Li-S Batteries journal, March 2016

Dendrite-Free Lithium Deposition Induced by Uniformly Distributed Lithium Ions for Efficient Lithium Metal Batteries journal, February 2016

The Regulating Role of Carbon Nanotubes and Graphene in Lithium-Ion and Lithium-Sulfur Batteries journal, July 2018

Current Status and Future Prospects of Metal–Sulfur Batteries journal, May 2019

Defect Engineering on Electrode Materials for Rechargeable Batteries journal, November 2019

Issues and challenges facing rechargeable lithium batteries
journal, November 2001

Electrical Energy Storage for the Grid: A Battery of Choices
journal, November 2011

Li–O₂ and Li–S batteries with high energy storage
journal, January 2012

Nanostructured sulfur cathodes
journal, January 2013

Rechargeable Lithium–Sulfur Batteries
journal, July 2014

Sulfur Cathodes with Hydrogen Reduced Titanium Dioxide Inverse Opal Structure
journal, April 2014

Challenges and Prospects of Lithium–Sulfur Batteries
journal, June 2012

Carbon–sulfur composites for Li–S batteries: status and prospects
journal, January 2013

Preparation of N-doped activated carbons for electric double-layer capacitors from waste fiberboard by K2CO3 activation
journal, April 2014

A highly ordered nanostructured carbon–sulphur cathode for lithium–sulphur batteries
journal, May 2009

Amphiphilic Surface Modification of Hollow Carbon Nanofibers for Improved Cycle Life of Lithium Sulfur Batteries
journal, February 2013

Lithium-Sulfur Batteries: Electrochemistry, Materials, and Prospects
journal, November 2013

Tailoring Microstructure of Graphene-Based Membrane by Controlled Removal of Trapped Water Inspired by the Phase Diagram
journal, February 2014

Insight into the Electrode Mechanism in Lithium-Sulfur Batteries with Ordered Microporous Carbon Confined Sulfur as the Cathode
journal, November 2013

Sulphur–TiO₂ yolk–shell nanoarchitecture with internal void space for long-cycle lithium–sulphur batteries
journal, January 2013

Polydopamine-Coated, Nitrogen-Doped, Hollow Carbon–Sulfur Double-Layered Core–Shell Structure for Improving Lithium–Sulfur Batteries
journal, August 2014

Phosphorous Pentasulfide as a Novel Additive for High-Performance Lithium-Sulfur Batteries
journal, June 2012

Dendrite-Free Lithium Deposition via Self-Healing Electrostatic Shield Mechanism
journal, March 2013

Nitrogen-Doped Mesoporous Carbon Promoted Chemical Adsorption of Sulfur and Fabrication of High-Areal-Capacity Sulfur Cathode with Exceptional Cycling Stability for Lithium-Sulfur Batteries
journal, October 2013

Fibrous Hybrid of Graphene and Sulfur Nanocrystals for High-Performance Lithium–Sulfur Batteries
journal, May 2013

Strongly Coupled Interfaces between a Heterogeneous Carbon Host and a Sulfur-Containing Guest for Highly Stable Lithium-Sulfur Batteries: Mechanistic Insight into Capacity Degradation
journal, July 2014

Enhancing lithium–sulphur battery performance by strongly binding the discharge products on amino-functionalized reduced graphene oxide
journal, September 2014

Development and costs calculation of lithium–sulfur cells with high sulfur load and binder free electrodes
journal, February 2013

Key Parameters Governing the Energy Density of Rechargeable Li/S Batteries
journal, February 2014

A Facile Layer-by-Layer Approach for High-Areal-Capacity Sulfur Cathodes
journal, January 2015

Lithium-Ion Textile Batteries with Large Areal Mass Loading
journal, October 2011

Very High Surface Capacity Observed Using Si Negative Electrodes Embedded in Copper Foam as 3D Current Collectors
journal, February 2014

A lithium–sulfur cathode with high sulfur loading and high capacity per area: a binder-free carbon fiber cloth–sulfur material
journal, January 2014

Three-Dimensional Sulfur/Graphene Multifunctional Hybrid Sponges for Lithium-Sulfur Batteries with Large Areal Mass Loading
journal, April 2014

Hierarchical Free-Standing Carbon-Nanotube Paper Electrodes with Ultrahigh Sulfur-Loading for Lithium-Sulfur Batteries
journal, July 2014

A graphene foam electrode with high sulfur loading for flexible and high energy Li-S batteries
journal, January 2015

Highly Reversible Lithium/Dissolved Polysulfide Batteries with Carbon Nanotube Electrodes
journal, May 2013

A membrane-free lithium/polysulfide semi-liquid battery for large-scale energy storage
journal, January 2013

Liquid-Type Cathode Enabled by 3D Sponge-Like Carbon Nanotubes for High Energy Density and Long Cycling Life of Li-S Batteries
journal, October 2014

Carbonized Eggshell Membrane as a Natural Polysulfide Reservoir for Highly Reversible Li-S Batteries
journal, November 2013

Sulfur-Functionalized Mesoporous Carbons as Sulfur Hosts in Li–S Batteries: Increasing the Affinity of Polysulfide Intermediates to Enhance Performance
journal, February 2014

A pH-sensitive graphene oxide composite hydrogel
journal, January 2010

An ice-templated, pH-tunable self-assembly route to hierarchically porous graphene nanoscroll networks
journal, January 2014

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage
journal, January 2008

Monolithic Fe2O3/graphene hybrid for highly efficient lithium storage and arsenic removal
journal, February 2014

The reduction of graphene oxide
journal, August 2012

BCN Graphene as Efficient Metal-Free Electrocatalyst for the Oxygen Reduction Reaction
journal, March 2012

Three-Dimensional Nitrogen and Boron Co-doped Graphene for High-Performance All-Solid-State Supercapacitors
journal, July 2012

Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide
journal, June 2007

Graphene sponge for efficient and repeatable adsorption and desorption of water contaminations
journal, January 2012

Cathode Composites for Li–S Batteries via the Use of Oxygenated Porous Architectures
journal, October 2011

Graphene Oxide as a Sulfur Immobilizer in High Performance Lithium/Sulfur Cells
journal, November 2011

Lithium/Sulfur Cell Discharge Mechanism: An Original Approach for Intermediate Species Identification
journal, April 2012

Free-Standing Nitrogen-doped Graphene Paper as Electrodes for High-Performance Lithium/Dissolved Polysulfide Batteries
journal, July 2014

Free-standing TiO2 nanowire-embedded graphene hybrid membrane for advanced Li/dissolved polysulfide batteries
journal, March 2015

Improved lithium–sulfur cells with a treated carbon paper interlayer
journal, January 2013

New insight into the discharge process of sulfur cathode by electrochemical impedance spectroscopy
journal, April 2009

A Soft Approach to Encapsulate Sulfur: Polyaniline Nanotubes for Lithium-Sulfur Batteries with Long Cycle Life
journal, January 2012

On the Surface Chemical Aspects of Very High Energy Density, Rechargeable Li–Sulfur Batteries
journal, January 2009

Role of LiNO3 in rechargeable lithium/sulfur battery
journal, May 2012

A Graphene-Pure-Sulfur Sandwich Structure for Ultrafast, Long-Life Lithium-Sulfur Batteries
journal, November 2013

Formation of Large Polysulfide Complexes during the Lithium-Sulfur Battery Discharge
journal, September 2014

Toward a Molecular Understanding of Energetics in Li–S Batteries Using Nonaqueous Electrolytes: A High-Level Quantum Chemical Study
journal, May 2014

A quantum-chemical study on the discharge reaction mechanism of lithium-sulfur batteries
journal, January 2013

Efficient Preparation of Large-Area Graphene Oxide Sheets for Transparent Conductive Films
journal, August 2010

Generalized Gradient Approximation Made Simple
journal, October 1996

Semiempirical GGA-type density functional constructed with a long-range dispersion correction
journal, January 2006

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage
journal, February 2009

Preparation of N-doped activated carbons for electric double-layer capacitors from waste fiberboard by K2CO3 activation
journal, September 2014

3D Aperiodic Hierarchical Porous Graphitic Carbon Material for High-Rate Electrochemical Capacitive Energy Storage
journal, February 2009

BCN Graphene as Efficient Metal-Free Electrocatalyst for the Oxygen Reduction Reaction
journal, March 2012

Highly Reversible Lithium/Dissolved Polysulfide Batteries with Carbon Nanotube Electrodes
journal, May 2013

Lithium/Sulfur Cell Discharge Mechanism: An Original Approach for Intermediate Species Identification
journal, April 2012

Issues and challenges facing rechargeable lithium batteries
journal, November 2001

Phase Inversion: A Universal Method to Create High-Performance Porous Electrodes for Nanoparticle-Based Energy Storage Devices
journal, October 2016

Functional Carbons Remedy the Shuttling of Polysulfides in Lithium-Sulfur Batteries: Confining, Trapping, Blocking, and Breaking up
journal, March 2018

Manipulation of Edge‐Site Fe–N ₂ Moiety on Holey Fe, N Codoped Graphene to Promote the Cycle Stability and Rate Capacity of Li–S Batteries
journal, December 2018

3D Interconnected Electrode Materials with Ultrahigh Areal Sulfur Loading for Li-S Batteries
journal, March 2016

Dendrite-Free Lithium Deposition Induced by Uniformly Distributed Lithium Ions for Efficient Lithium Metal Batteries
journal, February 2016

The Regulating Role of Carbon Nanotubes and Graphene in Lithium-Ion and Lithium-Sulfur Batteries
journal, July 2018

Current Status and Future Prospects of Metal–Sulfur Batteries
journal, May 2019

Defect Engineering on Electrode Materials for Rechargeable Batteries
journal, November 2019

A Nacre-Like Carbon Nanotube Sheet for High Performance Li-Polysulfide Batteries with High Sulfur Loading
journal, April 2018

Double-Shelled Phosphorus and Nitrogen Codoped Carbon Nanospheres as Efficient Polysulfide Mediator for High-Performance Lithium-Sulfur Batteries
journal, September 2018

Graphene-Based Nanocomposites for Energy Storage
journal, June 2016