Tuning the magnetic ground state of Ce1-xYbxRhIn5 by Yb valence fluctuations

Jang, S.; Pouse, N.; Keiber, T.; White, B. D.; Disseler, S. M.; Lynn, J. W.; Collini, J. C.; Janoschek, M.; Bridges, F.; Maple, M. B.

doi:10.1103/physrevb.98.195118

Title: Tuning the magnetic ground state of ${Ce}_{1 - x} {Yb}_{x} {RhIn}_{5}$ by Yb valence fluctuations

Abstract

We characterize the properties of Ce_1–x Yb_x RhIn₅ single crystals with 0 ≤ x ≤ 1 using measurements of powder x-ray diffraction, energy dispersive x-ray spectroscopy, electrical resistivity, magnetic susceptibility, specific heat, x-ray absorption near edge structure (XANES), and neutron diffraction. Here, the Yb valence v Yb , calculated from the magnetic susceptibility and measured using XANES, decreases from 3+ at x = 0 to ~2.1+ at x_act = 0.2 , where x_act is the measured Yb concentration. A transition from incommensurate to commensurate antiferromagnetism is observed in neutron diffraction measurements along Q = (0.5, 0.5, l) between 0.2 ≤ x act ≤ 0.27; this narrative is supported by specific-heat measurements in which a second robust feature appears at a temperature T_I (T_I < T_N) for the same concentration range. Magnetic susceptibility measurements also reveal features which provide additional evidence of magneticordering. The results of this study suggest that the evolution of the Yb valence plays a critical role in tuning the magnetic ground state of Ce_1–x Yb_x RhIn₅.

Authors:

Jang, S. ^[1]; Pouse, N. ^[2]; Keiber, T. ^[2]; White, B. D. ^[3]; Disseler, S. M. ^[4]; Lynn, J. W. ^[4]; Collini, J. C. ^[5]; Janoschek, M. ^[6]; Bridges, F. ^[7]; Maple, M. B. ^[2]

Univ. of California, San Diego, La Jolla, CA (United States); Univ. of California, Berkeley, CA (United States)
Univ. of California, San Diego, La Jolla, CA (United States)
Univ. of California, San Diego, La Jolla, CA (United States); Central Washington Univ., Ellensburg, WA (United States)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
Rochester Inst. of Technology, Rochester, NY (United States); Univ. of Maryland, College Park, MD (United States)
Univ. of California, San Diego, La Jolla, CA (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Univ. of California, Santa Cruz, CA (United States)

Publication Date:: Fri Nov 16 00:00:00 EST 2018

Research Org.:: Univ. of California, San Diego, CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; National Science Foundation (NSF)

OSTI Identifier:: 1609540

Alternate Identifier(s):: OSTI ID: 1482425

Grant/Contract Number:: FG02-04ER46105; DMR0802478; DMR1005568; DMR-1508249

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 98; Journal Issue: 19; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; materials science; physics; Kondo effect; magnetic order; heavy-fermion systems; strongly correlated systems

Citation Formats


                    Jang, S., Pouse, N., Keiber, T., White, B. D., Disseler, S. M., Lynn, J. W., Collini, J. C., Janoschek, M., Bridges, F., and Maple, M. B. Tuning the magnetic ground state of Ce1-xYbxRhIn5 by Yb valence fluctuations.  United States: N. p., 2018. 
Web.  doi:10.1103/physrevb.98.195118.

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                    Jang, S., Pouse, N., Keiber, T., White, B. D., Disseler, S. M., Lynn, J. W., Collini, J. C., Janoschek, M., Bridges, F., & Maple, M. B. Tuning the magnetic ground state of Ce1-xYbxRhIn5 by Yb valence fluctuations.  United States.  https://doi.org/10.1103/physrevb.98.195118

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                    Jang, S., Pouse, N., Keiber, T., White, B. D., Disseler, S. M., Lynn, J. W., Collini, J. C., Janoschek, M., Bridges, F., and Maple, M. B. Fri .  
"Tuning the magnetic ground state of Ce1-xYbxRhIn5 by Yb valence fluctuations".  United States.  https://doi.org/10.1103/physrevb.98.195118.  https://www.osti.gov/servlets/purl/1609540.

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@article{osti_1609540,

  title        = {Tuning the magnetic ground state of Ce1-xYbxRhIn5 by Yb valence fluctuations},

  author       = {Jang, S. and Pouse, N. and Keiber, T. and White, B. D. and Disseler, S. M. and Lynn, J. W. and Collini, J. C. and Janoschek, M. and Bridges, F. and Maple, M. B.},

  abstractNote = {We characterize the properties of Ce1–x Ybx RhIn5 single crystals with 0 ≤ x ≤ 1 using measurements of powder x-ray diffraction, energy dispersive x-ray spectroscopy, electrical resistivity, magnetic susceptibility, specific heat, x-ray absorption near edge structure (XANES), and neutron diffraction. Here, the Yb valence v Yb , calculated from the magnetic susceptibility and measured using XANES, decreases from 3+ at x = 0 to ~2.1+ at xact = 0.2 , where xact is the measured Yb concentration. A transition from incommensurate to commensurate antiferromagnetism is observed in neutron diffraction measurements along Q = (0.5, 0.5, l) between 0.2 ≤ x act ≤ 0.27; this narrative is supported by specific-heat measurements in which a second robust feature appears at a temperature TI (TI < TN) for the same concentration range. Magnetic susceptibility measurements also reveal features which provide additional evidence of magneticordering. The results of this study suggest that the evolution of the Yb valence plays a critical role in tuning the magnetic ground state of Ce1–x Ybx RhIn5.},

  doi          = {10.1103/physrevb.98.195118},

  journal      = {Physical Review B},

  number       = 19,

  volume       = 98,

  place        = {United States},

  year         = {Fri Nov 16 00:00:00 EST 2018},

  month        = {Fri Nov 16 00:00:00 EST 2018}

}

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Strong suppression of superconductivity by divalent ytterbium Kondo holes in CeCoIn $_{5}$
journal, October 2012

Magnetic and non-Fermi-liquid phases in ${Ce}_{1 - x} Y_{x} {RhIn}_{5}$
journal, February 2003

Electronic structure and $f$ -orbital occupancy in Yb-substituted CeCoIn $_{5}$
journal, June 2011

The Complexity of the CaF ₂ :Yb System: A Huge, Reversible, X-ray-Induced Valence Reduction
journal, December 2017

Field-induced magnetic transitions in the quasi-two-dimensional heavy-fermion antiferromagnets ${Ce}_{n} {RhIn}_{3 n + 2}$ $(n = 1$ or 2)
journal, September 2001

Neutron scattering study of crystal fields in ${CeRhIn}_{5}$
journal, November 2002

Emergent magnetic anisotropy in the cubic heavy-fermion metal CeIn3
journal, August 2017

Universal heat conduction in ${Ce}_{1 - x} {Yb}_{x} {CoIn}_{5}$ : Evidence for robust nodal $d$ -wave superconducting gap
journal, February 2016

Fermi-surface evolution in Yb-substituted CeCoIn $_{5}$
journal, June 2012

Avoided Antiferromagnetic Order and Quantum Critical Point in $C e C o I n_{5}$
journal, December 2003

Incommensurate magnetic structure of ${CeRhIn}_{5}$
journal, December 2000

Specific heat in high magnetic fields and non-Fermi-liquid behavior in $Ce M {In}_{5}$ $(M = I r, Co)$
journal, September 2001

Unconventional superconductivity in heavy-fermion compounds
journal, July 2015

Wilson ratio in Yb-substituted CeCoIn ₅
journal, November 2010

Resolution of the discrepancy between the variation of the physical properties of Ce _{1- x} Yb _x CoIn ₅ single crystals and thin films with Yb composition
journal, November 2014

Heat capacity studies of Ce and Rh site substitution in the heavy-fermion antiferromagnet ${CeRhIn}_{5} :$ Short-range magnetic interactions and non-Fermi-liquid behavior
journal, January 2004

Field-Induced Quantum Critical Point in ${C e C o I n}_{5}$
journal, December 2003

Yb valence change in Ce $_{1 - x}$ Yb $_{x}$ CoIn $_{5}$ from spectroscopy and bulk properties
journal, October 2013

Superconductivity of CeRhIn ₅ under High Pressure
journal, November 2001

Correlation between ground state and orbital anisotropy in heavy fermion materials
journal, February 2015

Low temperature magnetic structure of CeRhIn ₅ by neutron diffraction on absorption-optimized samples
journal, March 2017

Magnetic structure of CeRhIn ₅ under magnetic field
journal, May 2007

Double-Focusing Thermal Triple-Axis Spectrometer at the NCNR
journal, January 2012

Nodal to Nodeless Superconducting Energy-Gap Structure Change Concomitant with Fermi-Surface Reconstruction in the Heavy-Fermion Compound ${CeCoIn}_{5}$
journal, January 2015

A profile refinement method for nuclear and magnetic structures
journal, June 1969

Magnitude of the Magnetic Exchange Interaction in the Heavy-Fermion Antiferromagnet ${CeRhIn}_{5}$
journal, December 2014

Anisotropic three-dimensional magnetic fluctuations in heavy fermion ${CeRhIn}_{5}$
journal, February 2002

Crystalline electric field effects in $Ce M {In}_{5} (M = Co, Rh, Ir)$ : Superconductivity and the influence of Kondo spin fluctuations
journal, October 2004

Hidden magnetism and quantum criticality in the heavy fermion superconductor CeRhIn5
journal, March 2006

Electronic in-plane symmetry breaking at field-tuned quantum criticality in CeRhIn5
journal, August 2017

Compilation of x-ray cross sections UCRL-50174, sections I, II revision 1, III, IV
journal, December 1970

Competitive Coexistence of Superconductivity with Antiferromagnetism in ${CeRhIn}_{5}$
journal, July 2006

Pressure studies of the quantum critical alloy ${Ce}_{0.93} {Yb}_{0.07} {CoIn}_{5}$
journal, May 2015