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Title: Transient GaAs plasmonic metasurfaces at terahertz frequencies

Abstract

Here we demonstrate the ultrafast formation of terahertz (THz) metasurfaces through all-optical creation of spatially modulated carrier density profiles in a deep-subwavelength GaAs film. The switch-on of the transient plasmon mode, governed by the GaAs effective electron mass and electron–phonon interactions, is revealed by structured-optical pump THz probe spectroscopy, on a time scale of 500 fs. By modulating the carrier density using different pump fluences, we observe a wide tuning of the electric dipole resonance of the transient GaAs metasurface from 0.5 THz to 1.7 THz. Furthermore, we numerically demonstrate that the metasurface presented here can be generalized to more complex architectures for realizing functionalities such as perfect absorption, leading to a 30 dB modulation depth. In conclusion, the platform also provides a pathway to achieve ultrafast manipulation of infrared beams in the linear and, potentially, nonlinear regime.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [1];  [1];  [1];  [1];  [3];  [1]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Indian Institute of Science Education and Research, Mohanpur (India)
  3. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1338393
Report Number(s):
SAND-2016-12650J
Journal ID: ISSN 2330-4022; 649940
Grant/Contract Number:  
AC04-94AL85000
Resource Type:
Accepted Manuscript
Journal Name:
ACS Photonics
Additional Journal Information:
Journal Volume: 4; Journal Issue: 1; Journal ID: ISSN 2330-4022
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; metasurface; perfect absorber; semiconductor; ultrafast plasmonics

Citation Formats

Yang, Yuanmu, Kamaraju, N., Campione, Salvatore, Liu, Sheng, Reno, John L., Sinclair, Michael B., Prasankumar, Rohit P., and Brener, Igal. Transient GaAs plasmonic metasurfaces at terahertz frequencies. United States: N. p., 2016. Web. doi:10.1021/acsphotonics.6b00735.
Yang, Yuanmu, Kamaraju, N., Campione, Salvatore, Liu, Sheng, Reno, John L., Sinclair, Michael B., Prasankumar, Rohit P., & Brener, Igal. Transient GaAs plasmonic metasurfaces at terahertz frequencies. United States. https://doi.org/10.1021/acsphotonics.6b00735
Yang, Yuanmu, Kamaraju, N., Campione, Salvatore, Liu, Sheng, Reno, John L., Sinclair, Michael B., Prasankumar, Rohit P., and Brener, Igal. Fri . "Transient GaAs plasmonic metasurfaces at terahertz frequencies". United States. https://doi.org/10.1021/acsphotonics.6b00735. https://www.osti.gov/servlets/purl/1338393.
@article{osti_1338393,
title = {Transient GaAs plasmonic metasurfaces at terahertz frequencies},
author = {Yang, Yuanmu and Kamaraju, N. and Campione, Salvatore and Liu, Sheng and Reno, John L. and Sinclair, Michael B. and Prasankumar, Rohit P. and Brener, Igal},
abstractNote = {Here we demonstrate the ultrafast formation of terahertz (THz) metasurfaces through all-optical creation of spatially modulated carrier density profiles in a deep-subwavelength GaAs film. The switch-on of the transient plasmon mode, governed by the GaAs effective electron mass and electron–phonon interactions, is revealed by structured-optical pump THz probe spectroscopy, on a time scale of 500 fs. By modulating the carrier density using different pump fluences, we observe a wide tuning of the electric dipole resonance of the transient GaAs metasurface from 0.5 THz to 1.7 THz. Furthermore, we numerically demonstrate that the metasurface presented here can be generalized to more complex architectures for realizing functionalities such as perfect absorption, leading to a 30 dB modulation depth. In conclusion, the platform also provides a pathway to achieve ultrafast manipulation of infrared beams in the linear and, potentially, nonlinear regime.},
doi = {10.1021/acsphotonics.6b00735},
journal = {ACS Photonics},
number = 1,
volume = 4,
place = {United States},
year = {Fri Dec 09 00:00:00 EST 2016},
month = {Fri Dec 09 00:00:00 EST 2016}
}

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Works referenced in this record:

Plasmonics for extreme light concentration and manipulation
journal, February 2010

  • Schuller, Jon A.; Barnard, Edward S.; Cai, Wenshan
  • Nature Materials, Vol. 9, Issue 3
  • DOI: 10.1038/nmat2630

Plasmonic meta-atoms and metasurfaces
journal, November 2014


Frontiers in terahertz sources and plasmonics
journal, August 2013


Widely Tunable Infrared Antennas Using Free Carrier Refraction
journal, November 2015


Reconfigurable Semiconductor Phased-Array Metasurfaces
journal, July 2015


Epsilon-Near-Zero Mode for Active Optoelectronic Devices
journal, December 2012


Epsilon-Near-Zero Strong Coupling in Metamaterial-Semiconductor Hybrid Structures
journal, October 2013

  • Jun, Young Chul; Reno, John; Ribaudo, Troy
  • Nano Letters, Vol. 13, Issue 11
  • DOI: 10.1021/nl402939t

Theory of epsilon-near-zero modes in ultrathin films
journal, March 2015

  • Campione, Salvatore; Brener, Igal; Marquier, Francois
  • Physical Review B, Vol. 91, Issue 12, Article No. 121408(R)
  • DOI: 10.1103/PhysRevB.91.121408

Epsilon-near-zero Al-doped ZnO for ultrafast switching at telecom wavelengths
journal, January 2015


Electrically Tunable Epsilon-Near-Zero (ENZ) Metafilm Absorbers
journal, November 2015

  • Park, Junghyun; Kang, Ju-Hyung; Liu, Xiaoge
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep15754

Ultrafast switching of tunable infrared plasmons in indium tin oxide nanorod arrays with large absolute amplitude
journal, February 2016

  • Guo, Peijun; Schaller, Richard D.; Ketterson, John B.
  • Nature Photonics, Vol. 10, Issue 4
  • DOI: 10.1038/nphoton.2016.14

Graphene plasmonics for tunable terahertz metamaterials
journal, September 2011


Electrically tunable graphene anti-dot array terahertz plasmonic crystals exhibiting multi-band resonances
journal, January 2015


Induced transparency by coupling of Tamm and defect states in tunable terahertz plasmonic crystals
journal, September 2013


Two Two-Dimensional Materials Are Better than One
journal, June 2013


Photo-designed terahertz devices
journal, October 2011

  • Okada, Takanori; Tanaka, Koichiro
  • Scientific Reports, Vol. 1, Issue 1
  • DOI: 10.1038/srep00121

One- and two-dimensional photo-imprinted diffraction gratings for manipulating terahertz waves
journal, July 2013

  • Chatzakis, Ioannis; Tassin, Philippe; Luo, Liang
  • Applied Physics Letters, Vol. 103, Issue 4
  • DOI: 10.1063/1.4813620

Subcycle control of terahertz waveform polarization using all-optically induced transient metamaterials
journal, February 2014

  • Kamaraju, N.; Rubano, Andrea; Jian, Linke
  • Light: Science & Applications, Vol. 3, Issue 2
  • DOI: 10.1038/lsa.2014.36

All-photoinduced terahertz optical activity
journal, January 2014

  • Kanda, Natsuki; Konishi, Kuniaki; Kuwata-Gonokami, Makoto
  • Optics Letters, Vol. 39, Issue 11
  • DOI: 10.1364/OL.39.003274

Photo-generated THz antennas
journal, January 2014

  • Georgiou, G.; Tyagi, H. K.; Mulder, P.
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep03584

Carrier dynamics in self-assembled ErAs nanoislands embedded in GaAs measured by optical-pump terahertz-probe spectroscopy
journal, May 2005

  • Prasankumar, R. P.; Scopatz, A.; Hilton, D. J.
  • Applied Physics Letters, Vol. 86, Issue 20
  • DOI: 10.1063/1.1923174

Ultrafast carrier dynamics in III-V semiconductors grown by molecular-beam epitaxy at very low substrate temperatures
journal, January 1992

  • Gupta, S.; Whitaker, J. F.; Mourou, G. A.
  • IEEE Journal of Quantum Electronics, Vol. 28, Issue 10
  • DOI: 10.1109/3.159553

Ultrafast optical switching of terahertz metamaterials fabricated on ErAs/GaAs nanoisland superlattices
journal, January 2007

  • Chen, Hou-Tong; Padilla, Willie J.; Zide, Joshua M. O.
  • Optics Letters, Vol. 32, Issue 12
  • DOI: 10.1364/OL.32.001620

Ultrafast thermalization of photoexcited carriers in polar semiconductors
journal, February 1993


Nonparabolicity of the conduction band in GaAs
journal, May 1990


Ultrafast relaxation dynamics of photoexcited carriers in GaAs and related compounds
journal, January 1985

  • Taylor, A. J.; Erskine, D. J.; Tang, C. L.
  • Journal of the Optical Society of America B, Vol. 2, Issue 4
  • DOI: 10.1364/JOSAB.2.000663

Effective Wavelength Scaling for Optical Antennas
journal, June 2007


Surface plasmons enhance optical transmission through subwavelength holes
journal, September 1998

  • Ghaemi, H. F.; Thio, Tineke; Grupp, D. E.
  • Physical Review B, Vol. 58, Issue 11, p. 6779-6782
  • DOI: 10.1103/PhysRevB.58.6779

Direct Observation of a Transition of a Surface Plasmon Resonance from a Photonic Crystal Effect
journal, May 2007


Experimental demonstration of frequency-agile terahertz metamaterials
journal, April 2008


Terahertz metamaterials with semiconductor split-ring resonators for magnetostatic tunability
journal, January 2008

  • Han, Jiaguang; Lakhtakia, Akhlesh; Qiu, Cheng-Wei
  • Optics Express, Vol. 16, Issue 19
  • DOI: 10.1364/OE.16.014390

Thermal tunability in terahertz metamaterials fabricated on strontium titanate single-crystal substrates
journal, January 2011

  • Singh, Ranjan; Azad, Abul K.; Jia, Q. X.
  • Optics Letters, Vol. 36, Issue 7
  • DOI: 10.1364/OL.36.001230

Perfect Metamaterial Absorber
journal, May 2008


Interference theory of metamaterial perfect absorbers
journal, January 2012


Nonlinear Terahertz Metamaterials via Field-Enhanced Carrier Dynamics in GaAs
journal, May 2013


Works referencing / citing this record:

Epsilon-Near-Zero Photonics: A New Platform for Integrated Devices
journal, March 2018

  • Niu, Xinxiang; Hu, Xiaoyong; Chu, Saisai
  • Advanced Optical Materials, Vol. 6, Issue 10
  • DOI: 10.1002/adom.201701292

High-efficiency and low-loss gallium nitride dielectric metasurfaces for nanophotonics at visible wavelengths
journal, November 2017

  • Emani, Naresh Kumar; Khaidarov, Egor; Paniagua-Domínguez, Ramón
  • Applied Physics Letters, Vol. 111, Issue 22
  • DOI: 10.1063/1.5007007

Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber
journal, May 2017


Semiconductor infrared plasmonics
journal, May 2019


Accelerating terahertz all-optical modulation by hot carriers effects of silver nanorods in PVA film
journal, July 2019

  • Yu, Jian-Ping; Chen, Sai; Fan, Fei
  • AIP Advances, Vol. 9, Issue 7
  • DOI: 10.1063/1.5098386

A Review of THz Modulators with Dynamic Tunable Metasurfaces
journal, July 2019

  • Wang, Lan; Zhang, Yaxin; Guo, Xiaoqing
  • Nanomaterials, Vol. 9, Issue 7
  • DOI: 10.3390/nano9070965

All‐Optical and Ultrafast Tuning of Terahertz Plasmonic Metasurfaces
journal, May 2018

  • Cai, Honglei; Huang, Qiuping; Hu, Xiang
  • Advanced Optical Materials, Vol. 6, Issue 14
  • DOI: 10.1002/adom.201800143