X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules
Abstract
Proof-of-principle measurements of the electron densities, temperatures, and ionization states of spherically compressed multi-shocked CH (polystyrene) capsules have been achieved using spectrally resolved x-ray Thomson scattering. A total energy of 13.5 kJ incident on target is used to compress a 70 μm thick CH shell above solid-mass density using three coalescing shocks. Separately, a laser-produced zinc He-α x-ray source at 9 keV delayed 200 ps-800 ps after maximum compression is used to probe the plasma in the non-collective scattering regime. The data show that x-ray Thomson scattering enables a complete description of the time-dependent hydrodynamic evolution of shock-compressed CH capsules, with a maximum measured density of ρ > 6 g cm–3. Additionally, the results demonstrate that accurate measurements of x-ray scattering from bound-free transitions in the CH plasma demonstrate strong evidence that continuum lowering is the primary ionization mechanism of carbon L-shell electrons.
- Authors:
-
- Univ. of California, Berkeley, CA (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Los Angeles, CA (United States)
- Univ. of Warwick, Coventry (United Kingdom)
- Univ. of Warwick, Coventry (United Kingdom); AWE plc, Aldermaston (United Kingdom)
- Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Univ. of California, Berkeley, CA (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1334509
- Alternate Identifier(s):
- OSTI ID: 1240054
- Report Number(s):
- LLNL-JRNL-611992
Journal ID: ISSN 1070-664X; PHPAEN
- Grant/Contract Number:
- FG52-06NA26212; AC52-07NA27344
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physics of Plasmas
- Additional Journal Information:
- Journal Volume: 20; Journal Issue: 5; Journal ID: ISSN 1070-664X
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY; x-ray scattering; ionization; electron scattering; inelastic scattering; carbon; 42 ENGINEERING; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Fletcher, L. B., Kritcher, A., Pak, A., Ma, T., Doppner, T., Fortmann, C., Divol, L., Landen, O. L., Vorberger, J., Chapman, D. A., Gericke, D. O., Falcone, R. W., and Glenzer, S. H. X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules. United States: N. p., 2013.
Web. doi:10.1063/1.4807032.
Fletcher, L. B., Kritcher, A., Pak, A., Ma, T., Doppner, T., Fortmann, C., Divol, L., Landen, O. L., Vorberger, J., Chapman, D. A., Gericke, D. O., Falcone, R. W., & Glenzer, S. H. X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules. United States. https://doi.org/10.1063/1.4807032
Fletcher, L. B., Kritcher, A., Pak, A., Ma, T., Doppner, T., Fortmann, C., Divol, L., Landen, O. L., Vorberger, J., Chapman, D. A., Gericke, D. O., Falcone, R. W., and Glenzer, S. H. Fri .
"X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules". United States. https://doi.org/10.1063/1.4807032. https://www.osti.gov/servlets/purl/1334509.
@article{osti_1334509,
title = {X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules},
author = {Fletcher, L. B. and Kritcher, A. and Pak, A. and Ma, T. and Doppner, T. and Fortmann, C. and Divol, L. and Landen, O. L. and Vorberger, J. and Chapman, D. A. and Gericke, D. O. and Falcone, R. W. and Glenzer, S. H.},
abstractNote = {Proof-of-principle measurements of the electron densities, temperatures, and ionization states of spherically compressed multi-shocked CH (polystyrene) capsules have been achieved using spectrally resolved x-ray Thomson scattering. A total energy of 13.5 kJ incident on target is used to compress a 70 μm thick CH shell above solid-mass density using three coalescing shocks. Separately, a laser-produced zinc He-α x-ray source at 9 keV delayed 200 ps-800 ps after maximum compression is used to probe the plasma in the non-collective scattering regime. The data show that x-ray Thomson scattering enables a complete description of the time-dependent hydrodynamic evolution of shock-compressed CH capsules, with a maximum measured density of ρ > 6 g cm–3. Additionally, the results demonstrate that accurate measurements of x-ray scattering from bound-free transitions in the CH plasma demonstrate strong evidence that continuum lowering is the primary ionization mechanism of carbon L-shell electrons.},
doi = {10.1063/1.4807032},
journal = {Physics of Plasmas},
number = 5,
volume = 20,
place = {United States},
year = {Fri May 24 00:00:00 EDT 2013},
month = {Fri May 24 00:00:00 EDT 2013}
}
Web of Science
Works referenced in this record:
Observations of Plasmons in Warm Dense Matter
journal, February 2007
- Glenzer, S. H.; Landen, O. L.; Neumayer, P.
- Physical Review Letters, Vol. 98, Issue 6
X-Ray Scattering Measurements of Radiative Heating and Cooling Dynamics
journal, July 2008
- Gregori, G.; Glenzer, S. H.; Fournier, K. B.
- Physical Review Letters, Vol. 101, Issue 4
HELIOS-CR – A 1-D radiation-magnetohydrodynamics code with inline atomic kinetics modeling
journal, May 2006
- MacFarlane, J. J.; Golovkin, I. E.; Woodruff, P. R.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 99, Issue 1-3
Screening of ionic cores in partially ionized plasmas within linear response
journal, June 2010
- Gericke, D. O.; Vorberger, J.; Wünsch, K.
- Physical Review E, Vol. 81, Issue 6
Pressure ionization in laser-fusion target simulation
journal, May 1980
- Zimmerman, G. B.; More, R. M.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 23, Issue 5
X-ray scattering from solid density plasmas
journal, June 2003
- Glenzer, S. H.; Gregori, G.; Rogers, F. J.
- Physics of Plasmas, Vol. 10, Issue 6
Electronic structure measurements of dense plasmas
journal, May 2004
- Gregori, G.; Glenzer, S. H.; Rogers, F. J.
- Physics of Plasmas, Vol. 11, Issue 5
High-precision measurements of the equation of state of hydrocarbons at 1–10 Mbar using laser-driven shock waves
journal, May 2010
- Barrios, M. A.; Hicks, D. G.; Boehly, T. R.
- Physics of Plasmas, Vol. 17, Issue 5
Measurement of carbon ionization balance in high-temperature plasma mixtures by temporally resolved X-ray scattering
journal, May 2006
- Gregori, G.; Glenzer, S. H.; Chung, H. -K.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 99, Issue 1-3
Experimental astrophysics with high power lasers and pinches
journal, August 2006
- Remington, Bruce A.; Drake, R. Paul; Ryutov, Dmitri D.
- Reviews of Modern Physics, Vol. 78, Issue 3
Interiors of Giant Planets Inside and Outside the Solar System
journal, October 1999
- Guillot, T.
- Science, Vol. 286, Issue 5437
Measurement of Short-Range Correlations in Shock-Compressed Plastic by Short-Pulse X-Ray Scattering
journal, April 2009
- Barbrel, B.; Koenig, M.; Benuzzi-Mounaix, A.
- Physical Review Letters, Vol. 102, Issue 16
Lowering of Ionization Potentials in Plasmas
journal, April 1966
- Stewart, John C.; Pyatt, Kedar D. , Jr.
- The Astrophysical Journal, Vol. 144
Comparison of methods for calculating atomic shielding factors
journal, October 1975
- Bloch, Benjamin J.; Mendelsohn, Lawrence B.
- Physical Review A, Vol. 12, Issue 4
X-ray scattering as a probe for warm dense mixtures and high-pressure miscibility
journal, March 2011
- Wünsch, K.; Vorberger, J.; Gregori, G.
- EPL (Europhysics Letters), Vol. 94, Issue 2
Absolute Equation-of-State Data in the 10–40 Mbar (1–4 TPa) Regime
journal, February 1998
- Cauble, R.; Perry, T. S.; Bach, D. R.
- Physical Review Letters, Vol. 80, Issue 6
Cryogenic thermonuclear fuel implosions on the National Ignition Facility
journal, May 2012
- Glenzer, S. H.; Callahan, D. A.; MacKinnon, A. J.
- Physics of Plasmas, Vol. 19, Issue 5
Theoretical model of x-ray scattering as a dense matter probe
journal, February 2003
- Gregori, G.; Glenzer, S. H.; Rozmus, W.
- Physical Review E, Vol. 67, Issue 2
Compton Scattering of X Rays from Bound Electrons
journal, August 1970
- Eisenberger, P.; Platzman, P. M.
- Physical Review A, Vol. 2, Issue 2
Electronic energy-levels in dense plasmas
journal, March 1982
- More, Richard M.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 27, Issue 3
Difference in X-ray scattering between metallic and non-metallic liquids due to conduction electrons
journal, February 1987
- Chihara, J.
- Journal of Physics F: Metal Physics, Vol. 17, Issue 2
X-ray Thomson scattering in high energy density plasmas
journal, December 2009
- Glenzer, Siegfried H.; Redmer, Ronald
- Reviews of Modern Physics, Vol. 81, Issue 4
Equation-of-state measurements for polystyrene at multi-TPa pressures in laser direct-drive experiments
journal, December 2005
- Ozaki, N.; Ono, T.; Takamatsu, K.
- Physics of Plasmas, Vol. 12, Issue 12
Lowering of the Ionization Energy for a Plasma in Thermodynamic Equilibrium
journal, January 1963
- Ecker, G.; Kröll, W.
- Physics of Fluids, Vol. 6, Issue 1
Interaction of photons with plasmas and liquid metals - photoabsorption and scattering
journal, December 1999
- Chihara, Junzo
- Journal of Physics: Condensed Matter, Vol. 12, Issue 3
Dense matter characterization by X-ray Thomson scattering
journal, October 2001
- Landen, O. L.; Glenzer, S. H.; Edwards, M. J.
- Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 71, Issue 2-6
Probing warm dense lithium by inelastic X-ray scattering
journal, October 2008
- García Saiz, E.; Gregori, G.; Gericke, D. O.
- Nature Physics, Vol. 4, Issue 12
High Density Plasma Effects on Atomic and Ionic Spectra
journal, November 1982
- Burgess, D. D.; Lee, R. W.
- Le Journal de Physique Colloques, Vol. 43, Issue C2
Compton Scattering and Electron Momentum Density in Beryllium
journal, January 1971
- Currat, R.; DeCicco, P. D.; Kaplow, Roy
- Physical Review B, Vol. 3, Issue 2
X-Ray Thomson-Scattering Measurements of Density and Temperature in Shock-Compressed Beryllium
journal, March 2009
- Lee, H. J.; Neumayer, P.; Castor, J.
- Physical Review Letters, Vol. 102, Issue 11
Atomic -shell Compton profiles and incoherent scattering factors: Theory
journal, January 1974
- Bloch, Benjamin J.; Mendelsohn, Lawrence B.
- Physical Review A, Vol. 9, Issue 1
Direct Measurements of the Ionization Potential Depression in a Dense Plasma
journal, August 2012
- Ciricosta, O.; Vinko, S. M.; Chung, H. -K.
- Physical Review Letters, Vol. 109, Issue 6
Design and simulations of indirect drive ignition targets for NIF
journal, November 2004
- Haan, S. W.; Amendt, P. A.; Dittrich, T. R.
- Nuclear Fusion, Vol. 44, Issue 12
Three-dimensional HYDRA simulations of National Ignition Facility targets
journal, May 2001
- Marinak, M. M.; Kerbel, G. D.; Gentile, N. A.
- Physics of Plasmas, Vol. 8, Issue 5
Works referencing / citing this record:
Density functional theory calculations of continuum lowering in strongly coupled plasmas
journal, March 2014
- Vinko, S. M.; Ciricosta, O.; Wark, J. S.
- Nature Communications, Vol. 5, Issue 1