From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping

Chen, Haijie; Narayan, Awadhesh; Fang, Lei; Calta, Nicholas P.; Shi, Fengyuan; Chung, Duck Young; Wagner, Lucas K.; Kwok, Wai -Kwong; Kanatzidis, Mercouri G.

doi:10.1103/PhysRevB.94.134411

Title: From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb₃ by Hole Doping

Abstract

Competing orders widely exist in many material systems, such as superconductivity, magnetism, and ferroelectricity; LaCrSb₃ is a highly anisotropic magnetic material in which the spins are aligned ferromagnetically in one direction and canted antiferromagnetically in another in the Cr-Sb chains. Hole doping with Sr²⁺ and Ca²⁺ in the La site suppresses the antiferromagnetic correlations and transforms the anisotropic magnetic order into a ferromagnetic lattice in all directions. Here, first-principles density functional theory calculations show that the canted magnetic order becomes energetically less favorable compared to the FM order upon hole doping. Doping in the La site is an effective approach to modulate the competing orders in LaCrSb₃.

Authors:

Chen, Haijie ^[1]; Narayan, Awadhesh ^[2]; Fang, Lei ^[1]; Calta, Nicholas P. ^[3]; Shi, Fengyuan ^[3]; Chung, Duck Young ^[4]; Wagner, Lucas K. ^[2]; Kwok, Wai -Kwong ^[4]; Kanatzidis, Mercouri G. ^[1]

Northwestern Univ., Evanston, IL (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Univ. of Illinois at Urbana-Champaign, Urbana, IL (United States)
Northwestern Univ., Evanston, IL (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Publication Date:: Tue Oct 11 00:00:00 EDT 2016

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; USDOE

OSTI Identifier:: 1332968

Alternate Identifier(s):: OSTI ID: 1328636

Grant/Contract Number:: AC02-06CH11357; AC02-98CH1088; NSF NNCI-1542205; NSF DMR-1121262; DEAC0298CH1088

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review, B: Condensed Matter

Additional Journal Information:: Journal Volume: 94; Journal Issue: 13; Journal ID: ISSN 0163-1829

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Chen, Haijie, Narayan, Awadhesh, Fang, Lei, Calta, Nicholas P., Shi, Fengyuan, Chung, Duck Young, Wagner, Lucas K., Kwok, Wai -Kwong, and Kanatzidis, Mercouri G. From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.94.134411.

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                    Chen, Haijie, Narayan, Awadhesh, Fang, Lei, Calta, Nicholas P., Shi, Fengyuan, Chung, Duck Young, Wagner, Lucas K., Kwok, Wai -Kwong, & Kanatzidis, Mercouri G. From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping.  United States.  https://doi.org/10.1103/PhysRevB.94.134411

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                    Chen, Haijie, Narayan, Awadhesh, Fang, Lei, Calta, Nicholas P., Shi, Fengyuan, Chung, Duck Young, Wagner, Lucas K., Kwok, Wai -Kwong, and Kanatzidis, Mercouri G. Tue .  
"From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping".  United States.  https://doi.org/10.1103/PhysRevB.94.134411.  https://www.osti.gov/servlets/purl/1332968.

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@article{osti_1332968,

  title        = {From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping},

  author       = {Chen, Haijie and Narayan, Awadhesh and Fang, Lei and Calta, Nicholas P. and Shi, Fengyuan and Chung, Duck Young and Wagner, Lucas K. and Kwok, Wai -Kwong and Kanatzidis, Mercouri G.},

  abstractNote = {Competing orders widely exist in many material systems, such as superconductivity, magnetism, and ferroelectricity; LaCrSb3 is a highly anisotropic magnetic material in which the spins are aligned ferromagnetically in one direction and canted antiferromagnetically in another in the Cr-Sb chains. Hole doping with Sr2+ and Ca2+ in the La site suppresses the antiferromagnetic correlations and transforms the anisotropic magnetic order into a ferromagnetic lattice in all directions. Here, first-principles density functional theory calculations show that the canted magnetic order becomes energetically less favorable compared to the FM order upon hole doping. Doping in the La site is an effective approach to modulate the competing orders in LaCrSb3.},

  doi          = {10.1103/PhysRevB.94.134411},

  journal      = {Physical Review, B: Condensed Matter},

  number       = 13,

  volume       = 94,

  place        = {United States},

  year         = {Tue Oct 11 00:00:00 EDT 2016},

  month        = {Tue Oct 11 00:00:00 EDT 2016}

}

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https://doi.org/10.1103/PhysRevB.94.134411

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Title: From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb3 by Hole Doping

Abstract

Citation Formats

Crystal structures of La3ZrSb5, La3HfSb5, and LaCrSb3· Structural relationships in ternary rare-earth antimonides journal, March 1997

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Title: From Complex Magnetism Ordering to Simple Ferromagnetism in Two-Dimensional LaCrSb₃ by Hole Doping

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