Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4

Jacobsen, H.; Zaliznyak, I. A.; Savici, A. T.; Winn, B. L.; Chang, S.; Hücker, M.; Gu, G. D.; Tranquada, J. M.

doi:10.1103/PhysRevB.92.174525

Title: Neutron scattering study of spin ordering and stripe pinning in superconducting ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$

Abstract

The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$ a superconductor with a transition temperature of T_c = 20 K. At T<< T_c, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below ~ 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO₆octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO₂ planes. Moreover, we observed a weak elastic (3 ^⁻30) superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La_2-xSr_xCuO₄. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.

Authors:

Jacobsen, H. ^[1]; Zaliznyak, I. A. ^[1]; Savici, A. T. ^[2]; Winn, B. L. ^[2]; Chang, S. ^[3]; Hücker, M. ^[1]; Gu, G. D. ^[1]; Tranquada, J. M. ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)

Publication Date:: Fri Nov 20 00:00:00 EST 2015

Research Org.:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1240590

Alternate Identifier(s):: OSTI ID: 1226680; OSTI ID: 1286893

Report Number(s):: BNL-111750-2016-JA
Journal ID: ISSN 1098-0121; PRBMDO; R&D Project: PO010; KC0201060

Grant/Contract Number:: SC00112704; AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 17; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Jacobsen, H., Zaliznyak, I. A., Savici, A. T., Winn, B. L., Chang, S., Hücker, M., Gu, G. D., and Tranquada, J. M. Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.174525.

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                    Jacobsen, H., Zaliznyak, I. A., Savici, A. T., Winn, B. L., Chang, S., Hücker, M., Gu, G. D., & Tranquada, J. M. Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4.  United States.  https://doi.org/10.1103/PhysRevB.92.174525

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                    Jacobsen, H., Zaliznyak, I. A., Savici, A. T., Winn, B. L., Chang, S., Hücker, M., Gu, G. D., and Tranquada, J. M. Fri .  
"Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4".  United States.  https://doi.org/10.1103/PhysRevB.92.174525.  https://www.osti.gov/servlets/purl/1240590.

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@article{osti_1240590,

  title        = {Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4},

  author       = {Jacobsen, H. and Zaliznyak, I. A. and Savici, A. T. and Winn, B. L. and Chang, S. and Hücker, M. and Gu, G. D. and Tranquada, J. M.},

  abstractNote = {The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La1.93Sr0.07CuO4 a superconductor with a transition temperature of Tc = 20 K. At T<< Tc, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below ~ 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO6 octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO2 planes. Moreover, we observed a weak elastic (3 ⁻30) superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La2-xSrxCuO4. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.},

  doi          = {10.1103/PhysRevB.92.174525},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 17,

  volume       = 92,

  place        = {United States},

  year         = {Fri Nov 20 00:00:00 EST 2015},

  month        = {Fri Nov 20 00:00:00 EST 2015}

}

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Works referencing / citing this record:

Pairing Symmetry, Nodal and Antinodal Superconducting Gap in $$\text {La}_{2-x}\text {Sr}_x\text {CuO}_{4}$$: A Doping Scenario
journal, May 2019

Verma, Sanjeev K.; Gupta, Anushri; Kumari, Anita
Journal of Low Temperature Physics, Vol. 196, Issue 5-6
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Staging superstructures in high- $T_{c}$ Sr/O codoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4 + y}$
journal, November 2017

Ray, P. J.; Andersen, N. H.; Jensen, T. B. S.
Physical Review B, Vol. 96, Issue 17
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Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates
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Li, Yangmu; Zhong, Ruidan; Stone, M. B.
Physical Review B, Vol. 98, Issue 22
DOI: 10.1103/physrevb.98.224508

Distinct Nature of Static and Dynamic Magnetic Stripes in Cuprate Superconductors
journal, January 2018

Jacobsen, H.; Holm, S. L.; Lăcătuşu, M. -E.
Physical Review Letters, Vol. 120, Issue 3
DOI: 10.1103/physrevlett.120.037003

Pair Density Waves in Superconducting Vortex Halos
text, January 2018

Wang, Yuxuan; Edkins, Stephen D.; Hamidian, Mohammad H.
arXiv
DOI: 10.48550/arxiv.1802.01582

Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates
text, January 2018

Li, Yangmu; Zhong, Ruidan; Stone, M. B.
arXiv
DOI: 10.48550/arxiv.1806.10633

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Title: Neutron scattering study of spin ordering and stripe pinning in superconducting La 1.93 Sr 0.07 CuO 4

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Citation Formats

“Nodal Gap” Induced by the Incommensurate Diagonal Spin Density Modulation in Underdoped High- T c Superconductors journal, January 2015

Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance journal, April 2011

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The effect of collective spin-1 excitations on electronic spectra in high- T c superconductors journal, January 2006

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The geometric order of stripes and Luttinger liquids journal, October 2001

Neutron-Scattering Evidence for a Periodically Modulated Superconducting Phase in the Underdoped Cuprate La 1.905 Ba 0.095 CuO 4 journal, October 2014

Low-temperature vortex liquid in La2−xSrxCuO4 journal, March 2007

NMR study on the local structure in La-based high- T c cuprates journal, March 2008

Energy gaps in the failed high-Tc superconductor La1.875Ba0.125CuO4 journal, December 2008

Anomalous breaking of phonon softening in the superconducting state of La1.85Sr0.15CuO4 journal, February 1996

Hidden Quantum Spin-Gap State in the Static Stripe Phase of High-Temperature La 2 − x Sr x CuO 4 Superconductors journal, January 2009

Structural Instability Associated with the Tilting of CuO 6 Octahedra in La 2 - x Sr x CuO 4 journal, March 2000

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Thermal conductivity and competing orders in d-wave superconductors journal, February 2003

Charge-4e superconductivity from pair-density-wave order in certain high-temperature superconductors journal, September 2009

A model of the consecutive structural phase transitions in La2-xBaxCuO4 journal, October 1994

Mantid—Data analysis and visualization package for neutron scattering and μ SR experiments journal, November 2014

Striped superconductors: how spin, charge and superconducting orders intertwine in the cuprates journal, November 2009

Quantum Impurities in the Two-Dimensional Spin One-Half Heisenberg Antiferromagnet journal, March 2002

Emergence of Coherent Magnetic Excitations in the High Temperature Underdoped La 2 − x Sr x CuO 4 Superconductor at Low Temperatures journal, April 2009

Direct observation of a one-dimensional static spin modulation in insulating La 1.95 Sr 0.05 CuO 4 journal, February 2000

Microstructure and Tc-suppression in La-cuprates journal, August 1997

Antiferromagnetic order induced by an applied magnetic field in a high-temperature superconductor journal, January 2002

Evidence for stripe correlations of spins and holes in copper oxide superconductors journal, June 1995

From quantum matter to high-temperature superconductivity in copper oxides journal, February 2015

Spin Fluctuations in the Underdoped High- T c Cuprate La 1.93 Sr 0.07 CuO 4 journal, March 2001

Superconducting single crystals journal, January 1989

Large Bi-2212 single crystal growth by the floating-zone technique journal, April 2008

Recent progress on HYSPEC, and its polarization analysis capabilities journal, January 2015

Colloquium : Theory of intertwined orders in high temperature superconductors journal, May 2015

A common thread: The pairing interaction for unconventional superconductors journal, October 2012

Investigation of the spin dynamics in YBa2Cu3O6+x by inelastic neutron scattering journal, February 1991

Dispersive Excitations in the High-Temperature Superconductor L a 2 − x S r x C u O 4 journal, September 2004

Evidence for unusual superconducting correlations coexisting with stripe order in La 1.875 Ba 0.125 CuO 4 journal, November 2008

Stripe States with Spatially Oscillating d -Wave Superconductivity in the Two-Dimensional t − t ′ − J Model journal, February 2002

Static magnetic correlations near the insulating-superconducting phase boundary in La2-xSrxCuO4 journal, January 2002

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Incommensurate geometry of the elastic magnetic peaks in superconducting La 1.88 Sr 0.12 CuO 4 journal, June 2000

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Energy Spectrum of Spin Fluctuations in Superconducting La 2 - x Sr x CuO 4 ( 0.10 ≤ x ≤ 0.25 ) journal, April 2000

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Stripe order, depinning, and fluctuations in La 1.875 Ba 0.125 CuO 4 and La 1.875 Ba 0.075 Sr 0.050 CuO 4 journal, September 2004

Reconciliation of local and long-range tilt correlations in underdoped La 2 − x Ba x CuO 4 ( 0 ≤ x ≤ 0.155 ) journal, February 2015

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Title: Neutron scattering study of spin ordering and stripe pinning in superconducting ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$

“Nodal Gap” Induced by the Incommensurate Diagonal Spin Density Modulation in Underdoped High- $T_{c}$ Superconductors
journal, January 2015

Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance
journal, April 2011

The Ground State of the Pseudogap in Cuprate Superconductors
journal, November 2006

The effect of collective spin-1 excitations on electronic spectra in high- T _c superconductors
journal, January 2006

Competing States in the $t$ - $J$ Model: Uniform $d$ -Wave State versus Stripe State
journal, July 2014

Emergence of superconductivity from the dynamically heterogeneous insulating state in La2−xSrxCuO4
journal, November 2012

The geometric order of stripes and Luttinger liquids
journal, October 2001

Neutron-Scattering Evidence for a Periodically Modulated Superconducting Phase in the Underdoped Cuprate ${La}_{1.905} {Ba}_{0.095} {CuO}_{4}$
journal, October 2014

Low-temperature vortex liquid in La2−xSrxCuO4
journal, March 2007

NMR study on the local structure in La-based high- T _c cuprates
journal, March 2008

Energy gaps in the failed high-Tc superconductor La1.875Ba0.125CuO4
journal, December 2008

Anomalous breaking of phonon softening in the superconducting state of La1.85Sr0.15CuO4
journal, February 1996

Hidden Quantum Spin-Gap State in the Static Stripe Phase of High-Temperature ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ Superconductors
journal, January 2009

Structural Instability Associated with the Tilting of CuO ₆ Octahedra in La _{2 - x} Sr _x CuO ₄
journal, March 2000

A universal relationship between magnetic resonance and superconducting gap in unconventional superconductors
journal, October 2009

Thermal conductivity and competing orders in d-wave superconductors
journal, February 2003

Charge-4e superconductivity from pair-density-wave order in certain high-temperature superconductors
journal, September 2009

A model of the consecutive structural phase transitions in La2-xBaxCuO4
journal, October 1994

Mantid—Data analysis and visualization package for neutron scattering and $μ$ SR experiments
journal, November 2014

Striped superconductors: how spin, charge and superconducting orders intertwine in the cuprates
journal, November 2009

Quantum Impurities in the Two-Dimensional Spin One-Half Heisenberg Antiferromagnet
journal, March 2002

Emergence of Coherent Magnetic Excitations in the High Temperature Underdoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ Superconductor at Low Temperatures
journal, April 2009

Direct observation of a one-dimensional static spin modulation in insulating ${La}_{1.95} {Sr}_{0.05} {CuO}_{4}$
journal, February 2000

Microstructure and Tc-suppression in La-cuprates
journal, August 1997

Antiferromagnetic order induced by an applied magnetic field in a high-temperature superconductor
journal, January 2002

Evidence for stripe correlations of spins and holes in copper oxide superconductors
journal, June 1995

From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

Spin Fluctuations in the Underdoped High- T _c Cuprate La _1.93 Sr _0.07 CuO ₄
journal, March 2001

Superconducting single crystals
journal, January 1989

Large Bi-2212 single crystal growth by the floating-zone technique
journal, April 2008

Recent progress on HYSPEC, and its polarization analysis capabilities
journal, January 2015

Colloquium : Theory of intertwined orders in high temperature superconductors
journal, May 2015

A common thread: The pairing interaction for unconventional superconductors
journal, October 2012

Investigation of the spin dynamics in YBa2Cu3O6+x by inelastic neutron scattering
journal, February 1991

Dispersive Excitations in the High-Temperature Superconductor $L a_{2 - x} S r_{x} C u O_{4}$
journal, September 2004

Evidence for unusual superconducting correlations coexisting with stripe order in ${La}_{1.875} {Ba}_{0.125} {CuO}_{4}$
journal, November 2008

Stripe States with Spatially Oscillating $d$ -Wave Superconductivity in the Two-Dimensional $t - t^{'} - J$ Model
journal, February 2002

Static magnetic correlations near the insulating-superconducting phase boundary in La2-xSrxCuO4
journal, January 2002

Neutron-scattering study of static antiferromagnetic correlations in ${La}_{2 - x} {Sr}_{x} {Cu}_{1 - y} {Zn}_{y} O_{4}$
journal, March 1999

Incommensurate geometry of the elastic magnetic peaks in superconducting ${La}_{1.88} {Sr}_{0.12} {CuO}_{4}$
journal, June 2000

Neutron-scattering study of spin-density wave order in the superconducting state of excess-oxygen-doped ${La}_{2} {CuO}_{4 + y}$
journal, August 1999

Stripe order in superconducting La $_{2 - x}$ Ba $_{x}$ CuO $_{4}$ ( $0.095 ⩽ x ⩽ 0.155$ )
journal, March 2011

${}^{63}C u$ NQR Measurement of Stripe Order Parameter in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, May 1999

Energy Spectrum of Spin Fluctuations in Superconducting La _{2 - x} Sr _x CuO ₄ ( 0.10 ≤ x ≤ 0.25 )
journal, April 2000

Structural phase transformations and superconductivity in ${La}_{2 - x}$ ${Ba}_{x}$ ${CuO}_{4}$
journal, June 1989

Stripe order, depinning, and fluctuations in ${La}_{1.875} {Ba}_{0.125} {CuO}_{4}$ and ${La}_{1.875} {Ba}_{0.075} {Sr}_{0.050} {CuO}_{4}$
journal, September 2004

Reconciliation of local and long-range tilt correlations in underdoped ${La}_{2 - x} {Ba}_{x} {CuO}_{4} (0 \leq x \leq 0.155)$
journal, February 2015

Structural and superconducting properties of ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ as a function of Sr content
journal, February 1994

Spin susceptibility of underdoped cuprate superconductors: Insights from a stripe-ordered crystal
journal, December 2008

Probing the connections between superconductivity, stripe order, and structure in La $_{1.905}$ Ba $_{0.095}$ Cu $_{1 - y}$ Zn $_{y}$ O $_{4}$
journal, April 2012

Diamagnetism and Cooper pairing above $T_{c}$ in cuprates
journal, February 2010

Onset of the vortexlike Nernst signal above $T_{c}$ in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ and ${Bi}_{2} {Sr}_{2 - y} {La}_{y} {CuO}_{6}$
journal, November 2001

Rotated stripe order and its competition with superconductivity in ${La}_{1.88} {Sr}_{0.12} {CuO}_{4}$
journal, September 2014

Unusual Magnetic Susceptibility Anisotropy in Untwinned ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ Single Crystals in the Lightly Doped Region
journal, June 2001

Observation of Magnetic Ordering in Superconducting ${La}_{2 - x} {Sr}_{x} Cu O_{4}$ by Muon Spin Rotation
journal, January 1989

Common Phase Diagram for Antiferromagnetism in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ and $Y_{1 - x} {Ca}_{x} {Ba}_{2} {Cu}_{3} O_{6}$ as Seen by Muon Spin Rotation
journal, April 1998

Observation of incommensurate magnetic correlations at the lower critical concentration for superconductivity in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ $(x = 0.05)$
journal, July 1999

Fincher-Burke spin excitations and $ω ∕ T$ scaling in insulating ${La}_{1.95} {Sr}_{0.05} {CuO}_{4}$
journal, November 2007

Incommensurate magnetic fluctuations in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$
journal, September 1991

Charge density wave fluctuations in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ and their competition with superconductivity
journal, June 2014

Structural effects of hydrostatic pressure in orthorhombic ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$
journal, August 1994

Charge Segregation, Cluster Spin Glass, and Superconductivity in ${La}_{1.94} {Sr}_{0.06} {CuO}_{4}$
journal, July 1999

Evidence of a critical hole concentration in underdoped YBa $_{2}$ Cu $_{3}$ O $_{y}$ single crystals revealed by $^{63}$ Cu NMR
journal, December 2012

Magnetic order and superconductivity in La2$minus;xSrxCuO4: a review
journal, May 2003

Spin-Glass Behavior in L $a_{1.96}$ S $r_{0.04}$ Cu $O_{4}$
journal, September 1995

Systematic study of short-range antiferromagnetic order and the spin-glass state in lightly doped ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, August 2000

Frustrated electronic phase separation and high-temperature superconductors
journal, May 1993

Landau theory of stripe phases in cuprates and nickelates
journal, January 1998

Dimensional Crossover and Charge Order in Half-Doped Manganites and Cobaltites
journal, July 2003

Theory of Incommensurate Magnetic Correlations Across the Insulator-Superconductor Transition of Underdoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, March 2005

Spin- and Pair-Density-Wave Glasses
journal, July 2015

Magnetic, transport, and optical properties of monolayer copper oxides
journal, July 1998

Uniaxial linear resistivity of superconducting La $_{1.905}$ Ba $_{0.095}$ CuO $_{4}$ induced by an external magnetic field
journal, April 2012

Magnetic-Field-Induced Spin Excitations and Renormalized Spin Gap of the Underdoped ${La}_{1.895} {Sr}_{0.105} {CuO}_{4}$ Superconductor
journal, February 2007

Dynamical Layer Decoupling in a Stripe-Ordered High- $T_{c}$ Superconductor
journal, September 2007

Towards a Two-Dimensional Superconducting State of ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ in a Moderate External Magnetic Field
journal, April 2010

Breakdown of the universal Josephson relation in spin-ordered cuprate superconductors
journal, September 2010

Role of nematic fluctuations in the thermal melting of pair-density-wave phases in two-dimensional superconductors
journal, March 2011

Two-Dimensional Superconducting Fluctuations in Stripe-Ordered ${La}_{1.875} {Ba}_{0.125} {CuO}_{4}$
journal, August 2007